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In the quest for realizations of quantum spin liquids, the exploration of Kitaev materials - spin-orbit entangled Mott insulators with strong bond-directional exchanges - has taken center stage. However, in these materials the local…

Despite exhibiting magnetic long-range order below $T_\mathrm{N} = 26.7\,\mathrm{K}$, the honeycomb cobaltate Na$_2$Co$_2$TeO$_6$ is predicted to enter a Kitaev spin liquid state when subjected to small external perturbations. While most of…

Strongly Correlated Electrons · Physics 2026-03-04 J. Arneth , R. Kalaivanan , R. Sankar , K. -Y. Choi , R. Klingeler

The honeycomb magnet $\alpha-$RuCl$_3$ is a prime candidate material for realizing the Kitaev quantum spin liquid (QSL), but it shows long-range magnetic order at low temperature. Nevertheless, its broad inelastic neutron scattering (INS)…

Strongly Correlated Electrons · Physics 2022-11-23 Oliver Franke , Dumitru Călugăru , Andreas Nunnenkamp , Johannes Knolle

The layered honeycomb magnet $\alpha$-RuCl$_3$ has attracted intense scrutiny as a prime candidate for realizing the Kitaev quantum spin liquid, yet a consensus on its microscopic Hamiltonian remains elusive due to the material's extreme…

The search for Kitaev quantum spin liquids (Kitaev-QSLs) in real materials has mainly focused on $4d$- and $5d$-electron honeycomb systems. A recent experimental study on the $4f^5$ honeycomb iodide $\mathrm{SmI}_3$ reported the absence of…

Strongly Correlated Electrons · Physics 2025-09-09 Li-Hao Xia , Yi-Peng Gao , Zhao-Yang Dong , Jian-Xin Li

Kitaev materials are of great interest due to their potential in realizing quantum spin liquid (QSL) states and applications in topological quantum computing. In the pursuit of realizing Kitaev QSL, a Mott insulator with strong…

Materials Science · Physics 2025-12-30 Yaozhenghang Ma , Ke Yang , Yuxuan Zhou , Hua Wu

When spin-orbit-entangled $d$-electrons reside on a honeycomb lattice, rich quantum states are anticipated to emerge, as exemplified by the $d^5$ Kitaev materials. Distinct yet equally intriguing physics may be realized with a $d$-electron…

A polycrystalline sample of the hyperhoneycomb iridate $\beta$-ZnIrO$_3$ was synthesized via a topochemical reaction, and its structural, magnetic, and thermodynamic properties were investigated. The magnetization and heat capacity data…

Strongly Correlated Electrons · Physics 2022-02-17 Yuya Haraguchi , Akira Matsuo , Koichi Kindo , Hiroko Aruga Katori

The Kitaev spin liquid, stabilized as the ground state of the Kitaev honeycomb model, is a paradigmatic example of a topological $\mathbb{Z}_2$ quantum spin liquid. The fate of the Kitaev spin liquid in presence of an external magnetic…

Strongly Correlated Electrons · Physics 2026-05-04 Will Holdhusen , Daniel Huerga , Gerardo Ortiz

The spin liquid phase is one of the prominent strongly interacting topological phases of matter whose unambiguous confirmation is yet to be reached despite intensive experimental efforts on numerous candidate materials. Recently, a new…

Strongly Correlated Electrons · Physics 2018-05-10 Andrei Catuneanu , Youhei Yamaji , Gideon Wachtel , Yong Baek Kim , Hae-Young Kee

We study the emergence of magnetic order in localized spins that interact solely through their coupling to a Kitaev-type spin liquid. Using three toy models -- the Kitaev model, the Yao-Lee model, and a square-lattice generalization of the…

Strongly Correlated Electrons · Physics 2025-07-09 M. A. Keskiner , M. Ö. Oktel , Natalia B. Perkins , Onur Erten

Kitaev magnets are materials with bond-dependent Ising interactions between localized spins on a honeycomb lattice. Such interactions could lead to a quantum spin-liquid (QSL) ground state at zero temperature. Recent theoretical studies…

In this computational study, we explore a viable route to access the Kitaev-Quantum Spin Liquid (QSL) state in recently synthesized monolayer of a so-called spin-orbit assisted Mott insulator OsCl$_3$. In addition to other magnetic ground…

Strongly Correlated Electrons · Physics 2025-01-14 Qiangqiang Gu , Shishir Kumar Pandey , Yihao Lin

Topological states of matter such as quantum spin liquids (QSLs) are of great interest because of their remarkable predicted properties including protection of quantum information and the emergence of Majorana fermions. Such QSLs, however,…

We discuss the discovery by variational Monte Carlo (VMC) methods of a series of multinode quantum spin liquids (QSLs) in extended Kitaev models on the honeycomb lattice. Like the gapless Kitaev spin liquid with its two nodes at K and…

Strongly Correlated Electrons · Physics 2024-12-03 Jiucai Wang , B. Normand , Zheng-Xin Liu

We investigate an S=3/2 quantum spin model on a two-dimensional honeycomb lattice that continuously interpolates between two paradigmatic quantum disordered states with distinct entanglement structures: the Kitaev quantum spin liquid and…

Strongly Correlated Electrons · Physics 2026-04-28 Sogen Ikegami , Kiyu Fukui , Rico Pohle , Yukitoshi Motome

While phase transitions between magnetic analogs of three states of matter --- a long-range ordered state, paramagnet, and spin liquid --- have been extensively studied, the possibility of "liquid-liquid" transitions, namely, between…

Strongly Correlated Electrons · Physics 2017-04-05 Joji Nasu , Yasuyuki Kato , Junki Yoshitake , Yoshitomo Kamiya , Yukitoshi Motome

Recent interest in honeycomb lattice materials has focused on their potential to host quantum spin liquid (QSL) states. Variations in bond angles and spin allow a range of interesting behaviors on this lattice, from the predicted QSL ground…

Strongly Correlated Electrons · Physics 2021-09-15 Veronica J. Stewart , Juan R. Chamorro , Tyrel M. McQueen

Motivated by the largely unexplored domain of multi-polar ordered spin states in the Kitaev-Heisenberg (KH) systems we investigate the ground state dynamics of the spin-$\frac{1}{2}$ KH model, focusing on quadrupolar (QP) order in 2-leg…

Strongly Correlated Electrons · Physics 2025-03-28 Manodip Routh , Sayan Ghosh , Jeroen van den Brink , Satoshi Nishimoto , Manoranjan Kumar

The $S=3/2$ Kitaev honeycomb model (KHM) is unique among the spin-$S$ Kitaev models due to a massive ground state quasi-degeneracy that hampered previous numerical and analytical studies. In a recent work~\cite{jin2022unveiling}, we showed…

Strongly Correlated Electrons · Physics 2023-08-15 Willian M. H. Natori , Hui-Ke Jin , Johannes Knolle