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We theoretically propose a family of $f$-electron based magnets that realizes Kitaev-type bond-dependent anisotropic interactions. Based on {\it ab initio} calculations, we show that $A_2$PrO$_3$ ($A$: alkali metals) crystalize in a…

Strongly Correlated Electrons · Physics 2020-11-03 Seong-Hoon Jang , Ryoya Sano , Yasuyuki Kato , Yukitoshi Motome

The recently discovered three-dimensional hyperhoneycomb iridate, $\beta$-Li$_2$IrO$_3$, has raised hopes for the realization of dominant Kitaev interaction between spin-orbit entangled local moments due to its near-ideal lattice structure.…

Strongly Correlated Electrons · Physics 2016-01-15 Heung-Sik Kim , Eric Kin-Ho Lee , Yong Baek Kim

Quantum spin liquids have fascinated condensed matter physicists for decades because of their unusual properties such as spin fractionalization and long-range entanglement. Unlike conventional symmetry breaking the topological order…

Strongly Correlated Electrons · Physics 2018-03-22 Maria Hermanns , Itamar Kimchi , Johannes Knolle

Kitaev's honeycomb lattice spin model is a remarkable exactly solvable model, which has a particular type of spin liquid (Kitaev spin liquid) as the ground state. Although its possible realization in iridates and $\alpha$-RuCl$_3$ has been…

Strongly Correlated Electrons · Physics 2017-08-07 Masahiko G. Yamada , Hiroyuki Fujita , Masaki Oshikawa

In the field of quantum magnetism, the exactly solvable Kitaev honeycomb model serves as a paradigm for the fractionalization of spin degrees of freedom and the formation of $\mathbb{Z}_2$ quantum spin liquids. An intense experimental…

Strongly Correlated Electrons · Physics 2019-02-07 Ciarán Hickey , Simon Trebst

Kitaev's honeycomb spin-liquid model and its proposed realization in materials such as $\alpha$-RuCl$_3$, Li$_2$IrO$_3$ and Na$_2$IrO$_3$ continue to present open questions about how the dynamics of a spin-liquid are modified in the…

Strongly Correlated Electrons · Physics 2020-02-12 R. Sarkar , Z. Mei , A. Ruiz , G. Lopez , H. -H. Klauss , J. G. Analytis , I. Kimchi , N. J. Curro

The Kitaev model, a honeycomb network of spins with bond-dependent anisotropic interactions, is a rare example of having a quantum spin liquid ground state. Although most Kitaev model candidate materials eventually order magnetically due to…

Strong spin-orbital-coupling magnetic systems with the honeycomb structure can provide bond-directional interactions which may result in Kitaev quantum spin liquids and exotic anyonic excitations. However, one of the key ingredients in real…

We point out that the Kitaev materials may not necessarily support Kitaev spin liquid. It is well-known that having a Kitaev term in the spin interaction is not the sufficient condition for the Kitaev spin liquid ground state. Many other…

Strongly Correlated Electrons · Physics 2019-05-22 Yao Dong Li , Xu Yang , Yi Zhou , Gang Chen

The physics of spin-orbit entangled magnetic moments of $4d$ and $5d$ transition metal ions on a honeycomb lattice has been much explored in search for unconventional magnetic orders or quantum spin liquids expected for compass spin models,…

Strongly Correlated Electrons · Physics 2024-10-15 Ryutaro Okuma , Kylie MacFarquharson , Roger D. Johnson , David Voneshen , Pascal Manuel , Radu Coldea

Quantum spin liquids (QSLs) represent a novel state of matter in which quantum fluctuations prevent conventional magnetic order from being established, and the spins remain disordered even at zero temperature. There have been many…

Strongly Correlated Electrons · Physics 2018-10-11 Zhen Ma , Kejing Ran , Jinghui Wang , Song Bao , Zhengwei Cai , Shichao Li , Jinsheng Wen

The 5d-electron honeycomb compound H$_3$LiIr$_2$O$_3$ [K. Kitagawa $et$ $al.$, Nature 554, 341-345 (2018)] exhibits an apparent quantum spin liquid (QSL) state. In this intercalated spin-orbital compound, a remarkable pile up of low-energy…

Strongly Correlated Electrons · Physics 2019-02-07 Johannes Knolle , Roderich Moessner , Natalia B. Perkins

We discuss magnetically ordered states, arising in Heisenberg-Kitaev and related spin models, on three-dimensional (3D) harmonic honeycomb lattices. For large classes of ordered states, we show that they can be mapped onto two-dimensional…

Strongly Correlated Electrons · Physics 2020-01-29 Wilhelm G. F. Krüger , Matthias Vojta , Lukas Janssen

Quantum spin liquids, a highly topologically entangled, dynamically correlated state where quantum fluctuations preclude any long-range ordering down to absolute zero. In the search for a topologically robust qubit, the scientific community…

Strongly Correlated Electrons · Physics 2026-02-11 Vivek Kumar , Pradeep Kumar

We have investigated the magnetic properties and mapped out the phase diagram of the honeycomb magnet Na2Co2TeO6 with Co 3d7 in out-of-plane magnetic fields. This material has previously been proposed to show nearest-neighbor Kitaev…

Strongly Correlated Electrons · Physics 2024-06-03 Shengzhi Zhang , Sangyun Lee , Eric Brosha , Qing Huang , Haidong Zhou , Vivien S. Zapf , Minseong Lee

Metastable states with surprising properties abound in Hilbert space. We study unfrustrated isotropic spin-\half Heisenberg models in honeycomb lattice and find emergence of \textit{metastable Kitaev spin liquids having a 2-spin nematic…

Strongly Correlated Electrons · Physics 2023-09-14 Ganapathy Baskaran

In the quest for materials hosting Kitaev spin liquids, much of the efforts have been focused on the fourth- and fifth-row transition metal compounds, which are spin-orbit coupling assisted Mott insulators. Here, we study the structural and…

Strongly Correlated Electrons · Physics 2022-12-20 Shishir Kumar Pandey , Ji Feng

Kitaev iridates have been proposed as candidates for realizing an elusive quantum spin liquid (QSL) state, in which strong spin-orbit coupling and bond-directional exchange generate a highly frustrated and entangled ground state. However,…

Quantum spin liquids (QSLs) host a variety of fractionalized particles. In Kitaev's paradigmatic honeycomb model a spin-$\tfrac{1}{2}$ fractionalizes into $Z_2$ flux due to emergent $Z_2$ gauge field and matter Majorana fermions. Although…

Strongly Correlated Electrons · Physics 2026-01-22 Shi Feng , Nandini Trivedi

Rare-earth materials hold promise to realize exotic magnetic states owing to synergy between electron correlations and spin-orbit coupling. Recently, quasi-two-dimensional honeycomb magnets $A_2$PrO$_3$ ($A$ = alkali metals) were predicted…

Strongly Correlated Electrons · Physics 2024-10-11 Seong-Hoon Jang , Yukitoshi Motome
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