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It is now well established that the Kitaev honeycomb model in a magnetic field along the $[111]$-direction harbors an intermediate gapless quantum spin liquid (QSL) phase sandwiched between a gapped non-abelian QSL at low fields $H< H_{c1}$…

Strongly Correlated Electrons · Physics 2020-05-13 Subhasree Pradhan , Niravkumar D. Patel , Nandini Trivedi

BaCo$_2$(AsO$_4$)$_2$ (BCAO), a honeycomb cobaltate, is considered a promising candidate for materials displaying the Kitaev quantum spin liquid state. This assumption is based on the distinctive characteristics of Co$^{2+}$ ions (3$d^7$)…

Strongly Correlated Electrons · Physics 2024-08-02 Sangyun Lee , Shengzhi Zhang , S. M. Thomas , L. Pressley , C. A. Bridges , Eun Sang Choi , Vivien S. Zapf , Stephen M. Winter , Minseong Lee

Despite the exciting implications of the Kitaev spin-Hamiltonian, finding and confirming the quantum spin liquid state has proven incredibly difficult. Recently the applicability of the model has been expanded through the development of a…

Strongly Correlated Electrons · Physics 2022-09-23 K. M. Taddei , V. O. Garlea , A. M. Samarakoon , L. D. Sanjeewa , J. Xing , T. W. Heitmann , C. dela Cruz , A. S. Sefat , D. Parker

Na$_2$IrO$_3$, a honeycomb 5$d^5$ oxide, has been recently identified as a potential realization of the Kitaev spin lattice. The basic feature of this spin model is that for each of the three metal-metal links emerging out of a metal site,…

Kitaev interactions, arising from the interplay of frustration and bond anisotropy, can lead to strong quantum fluctuations and, in an ideal case, to a quantum-spin-liquid state. However, in many nonideal materials, spurious non-Kitaev…

Recently, honeycomb cobaltates with 3$d^7$ were proposed to display Kitaev physics despite weak spin-orbit coupling. However, other theoretical and experimental works found leading XXZ Heisenberg and negligible Kitaev interactions in…

Strongly Correlated Electrons · Physics 2023-03-01 Xiaoyu Liu , Hae-Young Kee

In the search for realizations of Quantum Spin Liquids (QSL), it is essential to understand the interplay between inherent disorder and the correlated fluctuating spin ground state. H$_3$LiIr$_2$O$_6$ is regarded as a spin liquid proximate…

Strongly Correlated Electrons · Physics 2024-07-11 A. de la Torre , B. Zager , F. Bahrami , M. H. Upton , J. Kim , G. Fabbris , G. -H. Lee , W. Yang , D. Haskel , F. Tafti , K. W. Plumb

Using quantum chemistry calculations we shed fresh light on the electronic structure and magnetic properties of RuCl3, a proposed realization of the honeycomb Kitaev spin model. It is found that the nearest-neighbor Kitaev exchange K is…

Strongly Correlated Electrons · Physics 2017-01-19 Ravi Yadav , Nikolay A. Bogdanov , Vamshi M. Katukuri , Satoshi Nishimoto , Jeroen van den Brink , Liviu Hozoi

The honeycomb iridates A2IrO3 (A=Na, Li) constitute promising candidate materials to realize the Heisenberg-Kitaev model (HKM) in nature, hosting unconventional magnetic as well as spin liquid phases. Recent experiments suggest, however,…

Strongly Correlated Electrons · Physics 2015-06-19 Johannes Reuther , Ronny Thomale , Stephan Rachel

We investigate the ground state properties of the spin S=1 Kitaev honeycomb model under a magnetic field based on the density matrix renormalization group (DMRG) calculation. With the time reversal symmetry breaking due to the magnetic…

Strongly Correlated Electrons · Physics 2020-09-23 Zheng Zhu , Zheng-Yu Weng , D. N. Sheng

Magnetic materials are composed of the simple building blocks of magnetic moments on a crystal lattice that interact via magnetic exchange. Yet from this simplicity emerges a remarkable diversity of magnetic states. Some reveal the deep…

A range of honeycomb-lattice compounds has been proposed and investigated in the search for a topological Kitaev spin liquid. However, sizable Heisenberg interactions and additional symmetry-allowed exchange anisotropies in the magnetic…

Strongly Correlated Electrons · Physics 2018-10-18 Ravi Yadav , Stephan Rachel , Liviu Hozoi , Jeroen van den Brink , George Jackeli

One of the most important issues in modern condensed matter physics is the realization of fractionalized excitations, such as the Majorana excitations in the Kitaev quantum spin liquid. To this aim, the 3d-based Kitaev material Na2Co2TeO6…

We explore the potential experimental realization of the mixed-spin Kitaev model in materials such as Zr$_{0.5}$Ru$_{0.5}$Cl$_3$, where spin-1/2 and spin-3/2 ions occupy distinct sublattices of a honeycomb lattice. By developing a…

Strongly Correlated Electrons · Physics 2025-05-09 Willian Natori , Yang Yang , Hui-Ke Jin , Johannes Knolle , Natalia B. Perkins

Cobaltates with 3$d$ based layered honeycomb structure were recently proposed as Kitaev magnets and putative candidates to host the long-sought Kitaev spin liquid. Here we present inelastic neutron scattering results down to 50 mK for…

Strongly Correlated Electrons · Physics 2023-01-18 Alaric L. Sanders , Richard A. Mole , Jiatu Liu , Alex J. Brown , Dehong Yu , Chris D. Ling , Stephan Rachel

We report a $^{35}$Cl nuclear magnetic resonance study in the honeycomb lattice, $\alpha$-RuCl$_3$, a material that has been suggested to potentially realize a Kitaev quantum spin liquid (QSL) ground state. Our results provide direct…

Strongly Correlated Electrons · Physics 2017-07-26 S. -H. Baek , S. -H. Do , K. -Y. Choi , Y. S. Kwon , A. U. B. Wolter , S. Nishimoto , Jeroen van den Brink , B. Büchner

Finding new materials with antiferromagnetic (AFM) Kitaev interaction is an urgent issue to broaden and enrich the quantum magnetism research significantly. By carrying out inelastic neutron scattering experiments and subsequent analysis,…

There have been tremendous experimental and theoretical efforts toward discovery of quantum spin liquid phase in honeycomb-based-lattice materials with strong spin-orbit coupling. Here the bond-dependent Kitaev interaction between local…

Strongly Correlated Electrons · Physics 2016-12-23 Heung-Sik Kim , Yong Baek Kim , Hae-Young Kee

H3LiIr2O6 is the first honeycomb-lattice system without any signs of long-range magnetic order down to the lowest temperatures, raising the hope for the realization of an ideal Kitaev quantum spin liquid. Its honeycomb layers are coupled by…

Strongly Correlated Electrons · Physics 2020-05-13 K. Geirhos , P. Lunkenheimer , M. Blankenhorn , R. Claus , Y. Matsumoto , K. Kitagawa , T. Takayama , H. Takagi , I. Kézsmárki , A. Loidl

The 3$d^7$ Co$^{2+}$-based insulating magnet \NCTO{} has recently been reported to have strong Kitaev interactions on a honeycomb lattice, and is thus being considered as a Kitaev quantum spin liquid candidate. However, due to the existence…