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Self-assembly of colloidal particles is a promising avenue to control the shape and dynamics of larger aggregates. However, achieving the necessary fine control over the dynamics and specificity of the bonds between such particles remains a…

Soft Condensed Matter · Physics 2024-09-26 Muraleedharapai Mayarani , Justine Laurent , Martin Lenz , Olivia du Roure , Julien Heuvingh

Transitions in structural heterogeneity of colloidal depletion gels formed through short-range attractive interactions are correlated with their dynamical arrest. The system is a density and refractive index matched suspension of 0.20…

Soft Condensed Matter · Physics 2009-11-11 C. J. Dibble , M. Kogan , M. J. Solomon

We examine the structure and dynamics of small isolated $N$-particle clusters interacting via short-ranged Morse potentials. "Ideally preprared ensembles" obtained via exact enumeration studies of sticky hard sphere packings serve as…

Soft Condensed Matter · Physics 2015-06-22 Robert S. Hoy

Mixtures of several macromolecular species can lead to the formation of higher-order structures that often display non-ideal mixing behavior. In this work, we propose a minimal model of a quaternary system which considers the formation of a…

Soft Condensed Matter · Physics 2022-12-14 Ruoyao Zhang , Sheng Mao , Mikko Haataja

At low temperatures, colloidal particles with short-range attractive and long-range repulsive interactions can form various periodic microphases in bulk.In this paper, we investigate the self-assembly behaviour of colloids with competing…

Soft Condensed Matter · Physics 2023-12-12 Ningyi Li , Junhong Li , Lijingting Qing , Shicheng Ma , Yao Li , Baohui Li

Microgels are soft colloidal particles constituted by cross-linked polymer networks with a high potential for applications. In particular, after adsorption at a fluid interface, interfacial tension provides two-dimensional (2D) confinement…

Soft Condensed Matter · Physics 2021-09-03 Jacopo Vialetto , Natalie Nussbaum , Jotam Bergfreund , Peter Fischer , Lucio Isa

The theory of elastic interaction of micron size axially symmetric colloidal particles immersed into confined nematic liquid crystal has been proposed. General formulas are obtained for the self energy of one colloidal particle and…

Soft Condensed Matter · Physics 2015-05-14 S. B. Chernyshuk , B. I. Lev

We introduce a model gel system in which colloidal forces, structure, and rheology are measured by balancing the requirements of rheological and microscopy techniques with those of optical tweezers. Sterically stabilized poly(methyl…

Soft Condensed Matter · Physics 2015-06-18 Lilian C. Hsiao , Kathryn A. Whitaker , Michael J. Solomon , Eric M. Furst

Colloidal gels are out-of-equilibrium structures, made up of a rarefied network of colloidal particles. Comparing experiments to numerical simulations, with hydrodynamic interactions switched off, we demonstrate the crucial role of the…

Soft Condensed Matter · Physics 2015-09-17 C. Patrick Royall , Jens Eggers , Akira Furukawa , Hajime Tanaka

The binodals and the non-ergodicity lines of a binary mixture of hard sphere-like particles with large size ratio are computed for studying the interplay between dynamic arrest and phase separation in depletion-driven colloidal mixtures.…

Soft Condensed Matter · Physics 2009-11-13 Ph. Germain , S. Amokrane

We report a molecular dynamics simulation study of a model gel whose interaction potential is obtained by modifying the three body Stillinger-Weber model potential for silicon. The modification reduces the average coordination number, and…

Soft Condensed Matter · Physics 2015-05-14 Shibu Saw , Niels L. Ellegaard , Walter Kob , Srikanth Sastry

Strong particulate gels are widely believed to behave poroelastically in compression, e.g. in sedimentation, even though they consolidate irreversibly because of the stickiness of the particles. Particulate gels are usually adhesive as well…

Soft Condensed Matter · Physics 2009-03-06 Richard Buscall

We study gelation in suspensions of model colloidal particles with short-ranged attractive and long-ranged repulsive interactions by means of three-dimensional fluorescence confocal microscopy. At low packing fractions, particles form…

Soft Condensed Matter · Physics 2009-11-10 Andrew I. Campbell , Valerie J. Anderson , Jeroen S. van Duijneveldt , Paul Bartlett

Recently developed linker-mediated vitrimers based on metathesis of dioxaborolanes with various commercially available polymers have shown both good processability and outstanding performance, such as mechanical, thermal, and chemical…

Soft Condensed Matter · Physics 2020-11-10 Qun-Li Lei , Xiuyang Xia , Juan Yang , Massimo Pica Ciamarra , Ran Ni

We investigated the formation of cocontinuous structures in polymer blends. These polymeric bijels (bicontinuous interfacially jammed emulsion gels) were composed of polystyrene oligomer, polybutene and fluorescent hydrophobic silica…

Soft Condensed Matter · Physics 2015-02-03 Lian Bai , John Fruehwirth , Xiang Cheng , Christopher W. Macosko

We study the phase ordering colloids suspended in a thermotropic nematic liquid crystal below the clearing point Tni and the resulting aggregated structure. Small (150nm) PMMA particles are dispersed in a classical liquid crystal matrix,…

Soft Condensed Matter · Physics 2007-05-23 V. J. Anderson , E. M. Terentjev , S. P. Meeker , J. Crain , W. C. K. Poon

All liquids (except helium due to quantum effects) crystallize at low temperatures, forming ordered structures. The competition between disorder, which stabilizes the liquid phase, and energy, which favors the ordered crystalline structure,…

Soft Condensed Matter · Physics 2013-07-09 Frank Smallenburg , Francesco Sciortino

Colloidal gels are elasto-plastic materials composed of an out-of-equilibrium, self-assembled network of micron-sized (solid) particles suspended in a fluid. Recent work has shown that far-field hydrodynamic interactions do not change gel…

Soft Condensed Matter · Physics 2023-06-21 Kim William Torre , Joost de Graaf

In order to study the viscoelastic properties of certain complex fluids which are described in terms of a multiconnected transient network we have developed a convenient model system composed of microemulsion droplets linked by telechelic…

Soft Condensed Matter · Physics 2007-05-23 Mohammed Filali , Mohamed J. Ouazzani , Erir Michel , Raymond Aznar , Gregoire Porte , Jacqueline Appell

The possibility to induce demixing in a colloidal mixture by adding small polymers, or other equivalent depletant agents, is theoretically investigated. By use of Mean Field Theory, suitably generalized to deal with short range effective…

Soft Condensed Matter · Physics 2015-10-28 Alberto Parola , Luciano Reatto
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