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The equilibrium phase behaviour of hard spheres with size polydispersity is studied theoretically. We solve numerically the exact phase equilibrium equations that result from accurate free energy expressions for the fluid and solid phases,…

Soft Condensed Matter · Physics 2007-05-23 M. Fasolo , P. Sollich

We report a numerical study, covering a wide range of packing fraction $\phi$ and temperature $T$, for a system of particles interacting via a square well potential supplemented by an additional constraint on the maximum number $n_{\rm…

Soft Condensed Matter · Physics 2009-11-10 E. Zaccarelli , S. V. Buldyrev , E. La Nave , A. J. Moreno , I. Saika-Voivod , F. Sciortino , P. Tartaglia

The physical mechanism of elasticity of liquid surfaces coated with colloidal particles is proposed. It is suggested that particles are separated by water clearings and the capillary interaction between them is negligible. The case is…

Soft Condensed Matter · Physics 2015-03-12 Edward Bormashenko , Gene Whyman , Oleg Gendelman

Creating amorphous solid states by randomly bonding an ensemble of dense liquid monomers is a common procedure which is applied to create a variety of materials such as epoxy resins, colloidal gels, and vitrimers. The properties of the…

Soft Condensed Matter · Physics 2024-01-26 Misaki Ozawa , Jean-Louis Barrat , Walter Kob , Francesco Zamponi

Polymer microgels exhibit intriguing macroscopic flow properties arising from their unique microscopic structure. Microgel colloids usually comprise a crosslinked polymer network with a radially decaying density profile, resulting in a…

Soft Condensed Matter · Physics 2025-02-10 Maxime Bergman , Yixuan Xu , José Muñéton Díaz , Zhang Chi , Thomas G. Mason , Frank Scheffold

Motivated by the idea that intrinsically disordered proteins (IDPs) condense into liquid-like droplets within cells, we carry out Monte Carlo simulations of a polymer lattice model to study the relationship between charge patterning and…

Soft Condensed Matter · Physics 2019-12-11 Nicholas A. S. Robichaud , Ivan Saika-Voivod , Stefan Wallin

We use large-scale computer simulations to explore the non-equilibrium aging dynamics in a microscopic model for colloidal gels. We find that gelation resulting from a kinetically-arrested phase separation is accompanied by `anomalous'…

Soft Condensed Matter · Physics 2017-06-21 Pinaki Chaudhuri , Ludovic Berthier

Polypeptide-based diblock copolymers forming either well-defined self-assembled micelles or vesicles after direct dissolution in water or in dichloromethane, have been studied combining light and neutron scattering with electron microscopy…

The transport properties of colloidal particles in active liquids have been studied extensively. It has led to a deeper understanding of the interactions between passive and active particles. However, the phase behavior of colloidal…

Soft Condensed Matter · Physics 2023-01-30 Pragya Kushwaha , Vivek Semwal , Sayan Maity , Shraddha Mishra , Vijayakumar Chikkadi

In this thesis the formation and properties of a polymer gel on and at a surface are investigated. The gel under investigation is defined as a three-dimensional network of "phantom" macromolecules that form permanent links with one another…

Disordered Systems and Neural Networks · Physics 2007-05-23 WL Vandoolaeghe

Colloidal particles are considered ideal building blocks to produce materials with enhanced physical properties. The state-of-the-art techniques for synthesizing these particles provide control over shape, size, and directionality of the…

Soft Condensed Matter · Physics 2016-12-21 N. A. M. Araújo , C. S. Dias , M. M. Telo da Gama

Experimental results have shown that the kinetics of bond formation in chemical crosslinking of gelatin solutions is strongly affected not only by gelatin and reactant concentrations but also by the solution pH. We present an extended…

Soft Condensed Matter · Physics 2009-11-13 T. Abete , E. Del Gado , L. de Arcangelis , D. Hellio Serughetti , M. Djabourov

Colloidal patchy particles with divalent attractive interaction can self-assemble into linear polymer chains. Their equilibrium properties in 2D and 3D are well described by Wertheim's thermodynamic perturbation theory which predicts a…

Soft Condensed Matter · Physics 2022-09-21 H. J. Jonas , P. Schall , P. G. Bolhuis

A simple model of an active colloid consisting of dumbbell-shaped particles that cyclically change their length without propelling themselves is proposed and analyzed. At nanoscales, it represents an idealization for bacterial cytoplasm or…

Adaptation and Self-Organizing Systems · Physics 2020-01-28 Yuki Koyano , Hiroyuki Kitahata , Alexander S. Mikhailov

We construct a three-dimensional lattice model for biological gels in which straight lines of bonds correspond to filamentous semi-flexible polymers and lattice sites, which are exactly four-fold coordinated, to crosslinks. With only…

Soft Condensed Matter · Physics 2011-08-23 Olaf Stenull , T. C. Lubensky

We report an extensive numerical study of a charged colloidal system with competing short-range depletion attraction and long-range electrostatic repulsion. By analizing the cluster properties, we identify two distinct regions in the phase…

Soft Condensed Matter · Physics 2009-03-18 Juan Carlos Fernandez Toledano , Francesco Sciortino , Emanuela Zaccarelli

Lateral microsegregation in a monolayer of a binary mixture of particles or macromolecules is studied by MD simulations in a generic model with the interacting potentials inspired by effective interactions in biological or soft-matter…

Soft Condensed Matter · Physics 2025-05-26 M. Litniewski , W. T. Gozdz nd A. Ciach

We study the phase ordering dynamics of a two dimensional model colloidal solid using molecular dynamics simulations. The colloid particles interact with each other with a Hamaker potential modified by the presence of equatorial "patches"…

Disordered Systems and Neural Networks · Physics 2014-12-30 Chandana Mondal , Smarajit Karmakar , Surajit Sengupta

We examine nonequilibrium features of collapse behavior in model polymers with competing crystallization and glass transitions using extensive molecular dynamics simulations. By comparing to "colloidal" systems with no covalent bonds but…

Soft Condensed Matter · Physics 2015-03-19 Robert S. Hoy , Corey S. O'Hern

Recent studies aimed at investigating artificial analogs of bacterial colonies have shown that low-density suspensions of self-propelled particles confined in two dimensions can assemble into finite aggregates that merge and split, but have…

Soft Condensed Matter · Physics 2015-06-17 B. M. Mognetti , A. Šarić , S. Angioletti-Uberti , A. Cacciuto , C. Valeriani , D. Frenkel