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Defects on surfaces of semiconductors have a strong effect on their reactivity and catalytic properties. The concentration of different charge states of defects is determined by their formation energies. First-principles calculations are an…

Mesoscale and Nanoscale Physics · Physics 2017-07-05 Dmitry Vinichenko , M. Gokhan Sensoy , Cynthia M. Friend , Efthimios Kaxiras

A combination of Scanning Tunneling Microscopy/Spectroscopy and Density Functional Theory (DFT+U) is used to characterize excess electrons in TiO$_2$ rutile and anatase, two prototypical materials with identical chemical composition but…

We present a comprehensive first-principles investigation of carbon self-interstitial defects in diamond, ranging from mono- to hexa-interstitial complexes. By quantum mechanical density functional theory, empowered by interatomic potential…

Materials Science · Physics 2026-05-01 Nima Ghafari Cherati , Arsalan Hashemi , Ádám Gali

An influence of Mg and Si dopants on the formation energies and the concentration of point defects in yttrium aluminum garnet (YAG) is studied using the density functional approach. The formation energies of Mg and Si substitutional and…

Materials Science · Physics 2023-01-16 L. Yu. Kravchenko , D. V. Fil

We calculate the upper critical field, Hc2(T), due to the orbital pair breaking in disordered superconductors without inversion symmetry. Differences from the usual centrosymmetric case are highlighted. The linearized gap equations in…

Superconductivity · Physics 2009-11-13 K. V. Samokhin

In this work an overall electronic structure including the position and formation energies of various intrinsic defects are computed for anatase using Density Functional Theory aided by Hubbard correction (DFT+U). The intrinsic point…

We perform first-principles calculations of the quasiparticle defect states, charge transition levels, and formation energies of oxygen vacancies in rutile titanium dioxide. The calculations are done within the recently developed combined…

Materials Science · Physics 2014-07-23 Andrei Malashevich , Manish Jain , Steven G. Louie

Surface-states of topological insulators are assumed to be robust against non-magnetic defects in the crystal. However, recent theoretical models and experiments indicate that even non-magnetic defects can perturb these states. Our…

Materials Science · Physics 2022-07-25 Sharmila N. Shirodkar , Pratibha Dev

The dependence of the electrical conductivity on the oxygen partial pressure is calculated for the prototypical perovskite $\Ba\Ti\O_3$ based on data obtained from first-principles calculations within density functional theory. The…

Materials Science · Physics 2012-01-19 Paul Erhart , Karsten Albe

Lattice defects affect the long-term stability of halide perovskite solar cells. Whereas simple point defects, i.e., atomic interstitials and vacancies, have been studied in great detail, here we focus on compound defects that are more…

Materials Science · Physics 2022-09-09 Haibo Xue , José Manuel Vicent-Luna , Shuxia Tao , Geert Brocks

The phase separation behaviors from the single B2 ordered phase into the two separate B2 and L2$_1$ ordered phases in the X-Al-Ti (X: Fe, Co, and Ni) alloys are analyzed using the cluster variation method (CVM) with the interaction energies…

Materials Science · Physics 2019-10-23 Ryo Yamada , Tetsuo Mohri

Radiation defects in barium fluoride single crystals doped with cadmium have been investigated by luminescence and absorption spectroscopy, as well as by electron spin resonance spectroscopy. Three types of Cd$^+$ centers differing by the…

Materials Science · Physics 2015-10-28 A. V. Egranov

The binary Bi-chalchogenides, Bi2Ch3, are widely regarded as model examples of a recently discovered new form of quantum matter, the three-dimensional topological insulator (TI) [1-4]. These compounds host a single spin-helical surface…

Mixtures of bare atomic nuclei on a nearly uniform degenerate electron background are a realistic model of matter in the interior of white dwarfs. Despite tremendous progress in understanding their phase diagrams achieved mainly via…

Solar and Stellar Astrophysics · Physics 2025-04-17 D. A. Baiko

Recent experimental work has realized a new insulating state of samarium nickelate (SmNiO$_3$), accessible in a reversible manner via high-density electron doping. To elucidate this behavior, we use the first-principles density functional…

Mesoscale and Nanoscale Physics · Physics 2019-11-27 Michele Kotiuga , Karin M. Rabe

We investigate the mechanism of the resonant X-ray scattering on the Ti $K$ edge region of YTiO$_3$ using the band structure calculation combined with the local density approximation. A large intensity is obtained for the orbital…

Strongly Correlated Electrons · Physics 2007-05-23 Manabu Takahashi , Jun-ichi Igarashi

We report a comprehensive first-principles study of the thermodynamics and transport of intrinsic point defects in layered oxide cathode materials LiMO$_2$ (M=Co, Ni), using density-functional theory and the Heyd-Scuseria-Ernzerhof screened…

Materials Science · Physics 2014-12-17 Khang Hoang , Michelle D. Johannes

The electron dephasing time $\tau_{\phi}$ in a diffusive quantum dot is calculated by considering the interaction between the electron and dynamical defects, modelled as two-level system. Using the standard tunneling model of glasses, we…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Kang-Hun Ahn , Pritiraj Mohanty

Cobalt-related impurity centers in diamond have been studied using first principles calculations. We computed the symmetry, formation and transition energies, and hyperfine parameters of cobalt impurities in isolated configurations and in…

Computational Physics · Physics 2013-07-11 R. Larico , L. V. C. Assali , W. V. M. Machado , J. F. Justo

A large number of published experimental works suggest that when the Fe ions in orthorhombic LaFeO3 are substituted, band gap reduction is expected. However, recent experimental works observe band gap enhancement with increasing Ti ions…

Materials Science · Physics 2024-01-23 Jesaya Situmeang , Djoko Triyono , Muhammad Aziz Majidi
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