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This paper reviews and summarizes the recent first-principles theoretical studies of the structural stability, electronic structure, optical and magnetic properties of nonmetal-doped TiO$_2$. The first section presents a comparison study of…

Materials Science · Physics 2020-09-10 Kesong Yang , Ying Dai , Baibiao Huang

Many mixed ionic/electronic conductors (MIECs) applied in fuel cell electrodes can be considered as alloys between perovskite oxides and ordered oxygen vacancy compounds. For example, in the model MIEC (STF), low oxygen diffusion barrier…

Materials Science · Physics 2018-08-14 Bin Ouyang , Tim Mueller , Nicola H. Perry , Narayana R Aluru , Elif Ertekin

Quartz is extensively used for luminescence and ESR dosimetry as well as dating. These techniques use inherent defects introduced in quartz crystal during its crystallization in nature. The defect comprises both intrinsic as well as…

Materials Science · Physics 2025-04-28 Jalaja Pandya , Malika Singhal , Navinder Singh , Naveen Chauhan

We present a comprehensive study of the energetics and magnetic properties of ZnO clusters doped with 3d transition metals (TM) using ab initio density functional calculations in the framework of generalized gradient approximation + Hubbard…

Materials Science · Physics 2015-05-20 Nirmal Ganguli , Indra Dasgupta , Biplab Sanyal

Defects in crystalline silicon consisting of a silicon self-interstitial atom and one, two, three, or four hydrogen atoms are studied within density-functional theory (DFT). We search for low-energy defects by starting from an ensemble of…

Materials Science · Physics 2010-02-11 Andrew J. Morris , Chris J. Pickard , R. J. Needs

Semi-empirical interatomic potentials have been developed for Al, alpha-Ti, and gamma-TiAl within the embedded atomic method (EAM) by fitting to a large database of experimental as well as ab-initio data. The ab-initio calculations were…

Materials Science · Physics 2009-11-10 Rajendra R. Zope , Y. Mishin

We investigate the behavior of oxygen vacancies in three different metal-oxide semiconductors (rutile and anatase TiO2, monoclinic WO3, and tetragonal ZrO2) using a recently proposed hybrid density-functional method in which the fraction of…

Density functional theory (DFT) and DFT corrected for on-site Coulomb interactions (DFT+U) calculations are presented on Aluminium doping in bulk TiO$_2$ and the anatase (101) surface. Particular attention is paid to the mobility of oxygen…

Materials Science · Physics 2014-03-24 Conn O'Rourke , David R. Bowler

Dimer vacancy (DV) defect complexes in the Si(001)2x1 surface were investigated using high-resolution scanning tunneling microscopy and first principles calculations. We find that under low bias filled-state tunneling conditions, isolated…

The formation of heterogeneous lanthanide-ion clusters in CaF$_2$ was investigated experimentally and computationally. CaF$_2$ nanoparticles co-doped with 20~mol\% Yb$^{3+}$ and 2~mol\% Ln$^{3+}$ (Ln$^{3+}$ = Ce$^{3+}$, Pr$^{3+}$,…

Ab-initio density functional theory (DFT) calculations of the relative stability of anatase and rutile polymorphs of TiO2 were carried using all-electron atomic orbitals methods with local density approximation (LDA). The rutile phase…

Materials Science · Physics 2012-10-30 Dorian A. H. Hanaor , Mohammed H. N. Assadi , Sean Li , Aibing Yu , Charles C. Sorrell

Ab initio molecular dynamics simulations are used to investigate the structure and electronic properties of the liquid Ag-Se system at three compositions. The realism of the simulations is demonstrated by comparison with diffraction data…

mtrl-th · Physics 2009-10-28 F. Kirchhoff , J. M. Holender , M. J. Gillan

The phase diagram of Al-Li-Cu system in the Al-rich region was determined by means of first-principles calculations and statistical mechanics. The mixing enthalpies of many configurations for different lattices in the whole Al-Li-Cu system…

Materials Science · Physics 2022-06-29 S. Liu , J. S. Wróbel , J. LLorca

Optimising the photoelectrochemical performance of hematite photoanodes for solar water splitting requires better understanding of the relationships between dopant distribution, structural defects and photoelectrochemical properties. Here,…

Erbium (Er) doped GaN has been studied extensively for optoelectronic applications, yet its defect physics is still not well understood. In this work, we report a first-principles hybrid density functional study of the structure,…

Materials Science · Physics 2017-10-30 Khang Hoang

Topological insulators are a class of band insulators with non-trivial topology, a result of band inversion due to the strong spin-orbit coupling. The transition between topological and normal insulator can be realized by tuning the…

Strongly Correlated Electrons · Physics 2018-03-29 Wenhan Zhang , M. X. Chen , Jixia Dai , Xueyun Wang , Zhicheng Zhong , Sang-Wook Cheong , Weida Wu

Quantum technologies would benefit from the development of high performance quantum defects acting as single-photon emitters or spin-photon interface. Finding such a quantum defect in silicon is especially appealing in view of its favorable…

Materials Science · Physics 2024-05-09 Yihuang Xiong , Jiongzhi Zheng , Shay McBride , Xueyue Zhang , Sinéad M. Griffin , Geoffroy Hautier

We perform full-potential screened-hybrid density-functional theory (DFT) calculations to compare the thermodynamic stability of neutral and charged states of the surface oxygen vacancy at the rutile TiO$_2$(110) surface. Solid-state…

Materials Science · Physics 2015-08-19 Daniel Berger , Harald Oberhofer , Karsten Reuter

We carried out a first principles investigation on the microscopic properties of nickel-related defect centers in diamond. Several configurations, involving substitutional and interstitial nickel impurities, have been considered either in…

Materials Science · Physics 2012-08-17 R. Larico , J. F. Justo , W. V. M. Machado , L. V. C. Assali

Elastic properties of Ti based \beta-alloy were studied by the method of the model structure first principle calculations. Concentrational dependence of Young modulus for the binary \beta-alloy Ti-Nb was discovered. It is shown that…

Atomic and Molecular Clusters · Physics 2011-12-01 A. N. Timoshevskii , S. O. Yablonovskii , O. M. Ivasishin