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The role of defects in solids of mixed ionic-covalent bonds such as ferroelectric oxides is complex. Current understanding of defects on ferroelectric properties at the single-defect level remains mostly at the empirical level, and the…

Materials Science · Physics 2017-09-13 Shi Liu , R. E. Cohen

We present results of an extensive set of first-principles density functional theory calculations of point defect formation, binding and clustering energies in austenitic Fe with dilute concentrations of Cr and Ni solutes.

Materials Science · Physics 2012-09-13 T. P. C. Klaver , D. J. Hepburn , G. J. Ackland

In this work we undertake the problem of a transition metal impurity in an oxide. We present an ab-initio study of the relaxations introduced in TiO2 when a Cd impurity replaces substitutionally a Ti atom. Using the Full-Potential…

Soft Condensed Matter · Physics 2009-11-10 L. Errico , G. Fabricius , M. Renteria

It is important to understand whether $\alpha$-clustering structures can leave traces in ultra-relativistic heavy ion collisions. Using the modified AMPT model, we simulate three $\alpha$ + core configurations of $^{44}$Ti in…

Nuclear Theory · Physics 2024-04-05 Yu-Xuan Zhang , Song Zhang , Yu-Gang Ma

X-ray diffraction studies showed that the structure of (Sr$_{1-x}$Pr$_x$)TiO$_3$ solid solutions at 300 K changes from the cubic $Pm3m$ to the tetragonal $I4/mcm$ with increasing $x$. The analysis of XANES and EXAFS spectra of the solid…

Materials Science · Physics 2012-07-26 I. A. Sluchinskaya , A. I. Lebedev , A. Erko

Dispersed impurities in diamond present a flourishing platform for research in quantum informatics, spintronics and single phonon emitters. Based on the vast pool of experimental and theoretical work describing impurity atoms in diamond, we…

Materials Science · Physics 2023-08-31 D. Propst , J. Kotakoski , E. H. Åhlgren

A theoretical study of the newly identified Ti5Al2C3 belonging to the MAX phases has been performed by using the first-principles pseudopotential plane-wave method within the generalized gradient approximation (GGA). The energy band…

Materials Science · Physics 2012-06-19 M. S. Ali , A. K. M. A. Islam , M. A. Hossain

The 3D ternary Li_4Ti_5O_12, the Li+-based battery anode, presents the unusual lattice symmetry (a triclinic crystal), band structure, charge density, and density of states, under the first-principles calculations. It belongs to a large…

Materials Science · Physics 2019-12-06 Thi Dieu Hien Nguyen , Hai Duong Pham , Shih-Yang Lin , Ming-Fa Lin

We study by means of first-principles pseudopotential method the coordination defects in a-Si and a-Si:H, also in their formation and their evolution upon hydrogen interaction. An accurate analysis of the valence charge distribution and of…

Materials Science · Physics 2009-10-31 M. Peressi , M. Fornari , S. de Gironcoli , L. De Santis , A. Baldereschi

We perform total energy calculations based on the tight-binding Hamiltonian scheme (i) to study the structural properties and energetics of the extended {311} defects depending upon their dimensions and interstitial concentrations and (ii)…

Materials Science · Physics 2009-10-28 Jeongnim Kim , John W. Wilkins , Furrukh S. Khan , Andrew Canning

The formation and electronic properties of nitrogen-related defect complexes in $\beta-Ga_2O_3$ are investigated using first-principles calculations. Starting from the energetically favorable $N_{i9}-N_{OI}$ configuration, nitrogen atoms…

Materials Science · Physics 2026-05-13 Asiyeh Shokri , Yevgen Melikhov , Yevgen Syryanyy , Maryna Chernyshova , Iraida N. Demchenko

Correlated band theory is employed to investigate the magnetic and electronic properties of different arrangements of oxygen di- and tri-vacancy clusters in SrTiO$_3$. Hole and electron doping of oxygen deficient SrTiO$_3$ yields various…

Materials Science · Physics 2016-03-30 Alejandro Lopez-Bezanilla , P. Ganesh , Peter B. Littlewood

One of the main sources of error associated with the calculation of defect formation energies using plane-wave Density Functional Theory (DFT) is finite size error resulting from the use of relatively small simulation cells and periodic…

Materials Science · Physics 2015-06-15 Samuel T. Murphy , Nicholas D. M. Hine

Increasing attention is being paid to $\alpha$$_2$ Ti$_3$(Al,Sn) precipitation from the $\alpha$ phase of titanium alloys owing to its effect on slip band formation, localisation and the implications for fatigue performance in jet engine…

Materials Science · Physics 2022-11-22 Felicity F. Worsnop , Susannah L. M. Lea , Jan Ilavsky , David Rugg , David Dye

Multi-principal-element alloys, including high-entropy alloys, experience segregation or partially-ordering as they are cooled to lower temperatures. For Ti$_{0.25}$CrFeNiAl$_{x}$, experiments suggest a partially-ordered B2 phase, whereas…

Materials Science · Physics 2021-05-11 Prashant Singh , A. V. Smirnov , Aftab Alam , Duane D. Johnson

The energetic cost of creating a defect within a host material is given by the formation energy. Here we present a formulation allowing the calculation of formation energies in one-dimensional nanostructures, which overcomes the…

Materials Science · Physics 2015-05-13 Riccardo Rurali , Xavier Cartoixa

The structure and thermodynamic properties of Ti$_x$(HfNbTaZr)$_{(1-x)/4}$ from Refractory High Entropy multicomponent Alloys to pure titanium are investigated employing comprehensive MCSQS realizations of the disordered atomic structure…

Materials Science · Physics 2024-07-18 Asif I. Bhatti , Marwa Al-Houcine , David Tingaud , Sylvain Queyreau

We employed density functional theory-based ab initio molecular dynamics simulations to examine the hydration structure of several common alkali and alkali earth metal cations. We found that the commonly used atom pairwise dispersion…

Chemical Physics · Physics 2023-09-08 Vojtech Kostal , Philip E. Mason , Hector Martinez-Seara , Pavel Jungwirth

There is growing evidence that the unconventional spatial inhomogeneities in the doped high-Tc superconductors are accompanied by the pairing of electrons, subsequent quantum phase transitions (QPTs), and condensation in coherent states. We…

Strongly Correlated Electrons · Physics 2012-11-12 Kun Fang , G. W. Fernando , A. V. Balatsky , A. N. Kocharian , Kalum Palandage

Point defect complexes in crystalline silicon composed of hydrogen, nitrogen, and oxygen atoms are studied within density-functional theory (DFT). Ab initio Random Structure Searching (AIRSS) is used to find low-energy defect structures. We…

Materials Science · Physics 2010-02-11 Andrew J. Morris , Chris J. Pickard , R. J. Needs