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Laser-driven high-order harmonic generation (HHG) provides tabletop sources of broadband extreme-ultraviolet (XUV) light with excellent spatial and temporal coherence. These sources are typically operated at low repetition rates,…

We present spatial coherence measurements of extreme-ultraviolet light generated using the process of high-harmonic upconversion of a femtosecond laser. Using a phase-matched hollow-fiber geometry, the generated beam is found to exhibit…

We applied a tabletop, ultrafast, high-harmonic generation (HHG) source to measure the element-specific ferromagnetic resonance (FMR) in ultra-thin magnetic alloys and multilayers on an opaque Si substrate. We demonstrate a continuous wave…

Materials Science · Physics 2024-04-25 Michael Tanksalvala , Anthony Kos , Jacob Wisser , Scott Diddams , Hans T. Nembach , Justin M. Shaw

Recent demonstrations of high-harmonic generation (HHG) at very high repetition frequencies (~100 MHz) may allow for the revolutionary transfer of frequency combs to the vacuum ultraviolet (VUV). This advance necessitates unifying optical…

The efficiency of a coherent VUV source at 125 nm, based on 2-photon resonant four-wave mixing in mercury vapor, has been enhanced by up to 2 orders of magnitude. This enhancement was obtained by locally heating a liquid Hg surface with a…

Coherent ultraviolet (UV) light has many uses, for example in the study of molecular species relevant in biology and chemistry. Very few if any laser materials offer UV transparency along with damage-free operation at high photon energies…

Dual Comb Spectroscopy proved its versatile capabilities in molecular fingerprinting in different spectral regions, but not yet in the ultraviolet (UV). Unlocking this spectral window would expand fingerprinting to the electronic energy…

We propose to generate continuous-wave vacuum ultraviolet (VUV) laser light at 148.4 nm using four-wave mixing in cadmium vapor for precision spectroscopy of the Th-229 isomer transition. Due to the large transition matrix elements of…

Development of the optical frequency comb has revolutionised metrology and precision spectroscopy due to its ability to provide a precise and direct link between microwave and optical frequencies. A novel application of frequency comb…

The exceptionally low-energy isomeric transition in $^{229}$Th at around 148.4 nm offers a unique opportunity for coherent nuclear control and the realisation of a nuclear clock. Recent advances, most notably the incorporation of large…

Ultraviolet (UV) diode lasers are widely used in many photonics applications. But their frequency stabilization schemes are not as mature as frequency-doubling lasers, mainly due to some limitations in the UV spectral region. Here we…

We report the generation of the 5th harmonic of Ti:sapphire, at 160 nm, with more than 4~$\mu$J of pulse energy, and a pulse length of 37 fs with a 1 kHz repetition rate. The VUV pulses are produced using Four-Wave Difference Frequency…

Optics · Physics 2024-04-01 Ruaridh Forbes , Paul Hockett , Quentin Leterrier , Rune Lausten

Vibrational sum- and difference-frequency generation (SFG and DFG) spectroscopy probes the nonlinear response of interfaces at mid-infrared (MIR) wavelengths while detecting upconverted signals in the visible. Recent work has moved from…

In the last few decades the development of ultrafast lasers has revolutionized our ability to gain insight into light-matter interactions. The appearance of few-cycle light sources available from the visible to the mid-infrared spectral…

Coherent extreme ultraviolet (XUV) radiation produced by table-top high-harmonic generation (HHG) sources provides a wealth of possibilities in research areas ranging from attosecond physics to high resolution coherent imaging. However, it…

Optics · Physics 2016-10-28 G. S. M. Jansen , D. Rudolf , L. Freisem , K. S. E. Eikema , S. Witte

Laser-Induced Fluorescence (LIF) spectroscopy is an essential tool for probing ion and atom velocity distribution functions (VDFs) in complex plasmas. VDFs carry information about kinetic properties of the species critical for plasma…

Plasma Physics · Physics 2024-03-19 Ivan Romadanov , Yevgeny Raitses , Andrei Smolyakov

The remarkable progress in the field of laser spectroscopy induced by the invention of the frequency-comb laser has enabled many new high-precision tests of fundamental theory and searches for new physics. Extending frequency-comb based…

Atomic Physics · Physics 2021-01-20 L. S. Dreissen , C. Roth , E. L. Gründeman , J. J. Krauth , M. G. J. Favier , K. S. E. Eikema

We present the general properties of the far-ultraviolet (FUV; 1370-1720A) continuum background over most of the sky, obtained with the Spectroscopy of Plasma Evolution from Astrophysical Radiation instrument (SPEAR, also known as FIMS),…

Astrophysics of Galaxies · Physics 2015-05-19 K. -I. Seon , J. Edelstein , E. Korpela , A. Witt , K. -W. Min , W. Han , J. Shinn , I. -J. Kim , J. -W. Park

Laser spectroscopy of the $^{\mathrm{229m}}$Th nuclear clock transition is necessary for the future construction of a nuclear-based optical clock. Precision laser sources with broad spectral coverage in the vacuum ultraviolet are needed for…

Deep Ultraviolet (DUV) Photolithography is currently used to fabricate mass-scale integrated circuits (ICs). Its high throughput and resolution could benefit large-scale RF MEMS production for the telecommunication market. We present a…

Systems and Control · Electrical Eng. & Systems 2024-07-23 Marco Liffredo , Federico Peretti , Nan Xu , Silvan Stettler , Luis Guillermo Villanueva