Related papers: Vacuum-ultraviolet frequency-modulation spectrosco…
The recent development of ultrafast extreme ultraviolet (XUV) coherent light sources bears great potential for a better understanding of the structure and dynamics of matter. Promising routes are advanced coherent control and nonlinear…
A narrow-bandwidth actively mode-locked laser using a Cr:ZnS gain medium has been successfully demonstrated. A free-space electro-optic phase modulator is employed in the solid-state laser resonator to achieve frequency-modulation (FM)…
One of the essential goals of molecular spectroscopy is to measure all fundamental molecular vibrations simultaneously. To this end, one needs to measure broadband infrared (IR) absorption and Raman scattering spectra, which provide…
Many fields such as bio-spectroscopy and photochemistry often require sources of vacuum ultraviolet (VUV) pulses featuring a narrow linewidth and tunable over a wide frequency range. However, the majority of available VUV light sources do…
The generation of shaped laser beams, or structured light, is of interest in a wide range of fields, from microscopy to fundamental physics. There are several ways to make shaped beams, most commonly using spatial light modulators comprised…
Self-diffraction is a non-collinear four-wave mixing technique well-known in optics. We explore self-diffraction in the extreme ultraviolet (EUV) range, taking advantage of intense femtosecond EUV pulses produced by a free electron laser.…
High-intensity laser pulses covering the ultraviolet to terahertz spectral regions are nowadays routinely generated in a large number of laboratories. In contrast, intense extreme-ultraviolet (XUV) pulses have only been demonstrated using a…
Non-collinear four-wave mixing (FWM) techniques at near-infrared (NIR), visible, and ultraviolet frequencies have been widely used to map vibrational and electronic couplings, typically in complex molecules. However, correlations between…
High harmonics generation (HHG) of coherent extreme ultraviolet (EUV) radiation enables ultrafast pump-probe spectroscopy with attosecond-scale timing resolutions. Yet beam control of generated EUV radiation remains a major challenge for…
Although supercontinuum sources are readily available for the visible and near infrared, and recently also for the mid-IR, many areas of biology, chemistry and physics would benefit greatly from the availability of compact, stable and…
We present a new technique using a frequency comb laser and optical cavities for performing ultrafast transient absorption spectroscopy with improved sensitivity. Resonantly enhancing the probe pulses, we demonstrate a sensitivity of…
We demonstrate a 1.4 W continuous wavelength (CW) laser at 243.1 nm. The radiation is generated through frequency quadrupling the output of a ytterbium-doped fiber amplifier system which produces $>$ 10 W of CW power at 972.5 nm. We…
Frequency modulation of a continuous wave laser source enables generation of photons at multiple frequencies from a single pump laser. Such multiple closely spaced laser lines are important for high data rate QAM in dense-WDM networks. In…
A chirped-pulse electro-optic (EO) dual comb system operating near 821 nm is used to generate cavity enhanced dual combs in the ultraviolet (UV) region near 323 nm with an optical bandwidth of up to 90 GHz. The UV combs result from…
We combine different wavelengths from an intense high-order harmonics source with variable delay at the focus of a split-mirror interferometer to conduct pump-probe experiments on gas-phase molecules. We report measurements of the time…
The operation of a frequency comb at extreme ultraviolet (XUV) wavelengths based on pair-wise amplification and nonlinear upconversion to the 15th harmonic of pulses from a frequency comb laser in the near-infrared range is reported.…
High harmonic generation (HHG) in solids has emerged as a powerful spectroscopic method for resolving ultrafast electron dynamics and band structure properties across a wide range of materials. However, quantitative HHG studies require…
Supercontinuum generation in the ultraviolet spectral region is challenging in solid-core optical fibres due to solarization and photodarkening. Antiresonant hollow-core fibres have overcome this limitation and have been shown to guide…
We present a novel high-power, frequency-stabilized UV laser source at 326.2~nm, resonant with the Cd $^{1}$S$_{0}$ - $^{3}$P$_{1}$ narrow intercombination transition. We have achieved a maximum produced power of 1~W at 326.2~nm by two…
We analyze the spectral properties of high-order harmonic radiation with photon energies extending beyond the regular cutoff energy in standard high-order harmonic generation. The extension of the regular harmonic cutoff results from…