Related papers: Vacuum-ultraviolet frequency-modulation spectrosco…
The highly energetic photons of ultraviolet light drive electronic and rovibronic transitions in all molecular species. This radiation is thus a prime tool for strongly selective spectroscopic fingerprinting and real-time environmental…
We present a 100 kHz broadband vibrational sum-frequency generation (VSFG) spectrometer operating in the 5.5-10.5 $\mu$m (950-1750 cm$^{-1}$) wavelength range. The mid-infrared beam of the system is obtained from a collinear, type-I…
New near- and far-ultraviolet (NUV and FUV) HST spectra of Mrk 231, the nearest quasar known, are combined with ground-based optical spectra to study the remarkable dichotomy between the FUV and NUV-optical spectral regions in this object.…
We describe an electro-optic dual-comb system that operates in the near-infrared (near-IR) region to generate optical frequency combs in the near-UV by sum frequency generation in two configurations. The near-IR frequency combs are…
Moving the detection wavelength in vibrational sum-frequency generation (VSFG) spectroscopy to the near-infrared (> 700 nm) can potentially enable the study of molecular interfaces absorbing in the visible and give access to buried…
VUV radiation around 159 nm is obtained toward direct excitation of a single trapped $^{115}$In$^{+}$ ion. An efficient fluoride-based VUV output-coupler is employed for intracavity high-harmonic generation of a Ti:S oscillator. Using this…
Using a mid-infrared quantum cascade laser and wavelength modulation absorption spectroscopy, we measure the frequencies of ro-vibrational transitions of N$_2$O in the 17 $\mu$m region with uncertainties below 5 MHz. These lines,…
We report here a detailed study of the four-wave mixing process in the extreme ultraviolet (XUV) region around 30 nm by using two collinear incommensurate frequency laser pulses. The experimental results reveal evidence of the coherent…
A femtosecond frequency comb provides a vast number of equidistantly spaced narrow band laser modes that can be simultaneously tuned and frequency calibrated with 15 digits accuracy. Our Vernier spectrometer utilizes all of theses modes in…
We investigate whether the far-UV continuum of nearby radio galaxies reveals evidence for the presence of star forming or non-stellar components. If a UV excess due to an extra radiation component exists we compare this with other…
Controlling the quantum field statistics of confined light is a long-standing goal in integrated photonics. We show that by coupling molecular vibrations with a confined mid-infrared cavity vacuum, the photocount and quadrature field…
We investigate the generation of ultraviolet (UV) second-harmonic radiation on the boundary of a UV transparent crystal, which is derived from the automatic partial phase matching of the incident wave and the total internal reflection. By…
A comprehensive study of interstellar medium phases and the nature of their boundaries or connections requires comparing abundances and velocity profiles from tracers of the different phases. In the UV, studies of a wealth of absorption…
We report here experimental results of perturbative nonlinear optical wave-mixing processes in the extreme ultraviolet region by using two-color and three-color laser fields. Besides the usual odd-harmonic spectrum of high harmonic…
A full spectral characterization of carbonaceous dust analogs is necessary to understand their potential as carriers of observed astronomical spectral signatures such as the ubiquitous UV bump at 217.5 nm and the far-ultraviolet (FUV) rise…
We present an approach for improving spatial frequency sampling in active incoherent millimeter-wave (AIM) imaging systems using frequency diversity. AIM imaging relies on active transmission of spatio-temporally incoherent signals to…
There are several mechanisms by which the frequency spectrum of a laser broadens when it propagates at near-relativistic-intensity in tenuous plasma. Focusing on one dimensional effects, we identify two strong optical nonlinearities,…
We introduce a novel ultra-broadband ultraviolet and visible frequency comb light source covering more than 240 THz by resonant dispersive wave emission in a gas-filled hollow-core fiber waveguide. The light source allows tuning from ~340…
Extreme ultraviolet (XUV) lasers are essential for the investigation of fundamental physics. Especially high repetition rate, high photon flux sources are of major interest for reducing acquisition times and improving signal to noise ratios…
Ultraviolet spectroscopy provides unique insights into the structure of matter with applications ranging from fundamental tests to photochemistry in the earth's atmosphere and astronomical observations from space telescopes. At longer…