English
Related papers

Related papers: Laser-coolable polyatomic molecules with heavy nuc…

200 papers

The particular advantages of using the diatomic molecule radium monofluoride (RaF) as a versatile molecular probe for physics beyond the Standard Model are highlighted. i) RaF was previously suggested as being potentially amenable to direct…

Chemical Physics · Physics 2020-05-25 T. A. Isaev , R. Berger

We have studied a general technique for laser cooling a cloud of polarized trapped atoms down to the Doppler temperature. A one-dimensional optical molasses using polarized light cools the axial motional degree of freedom of the atoms in…

Quantum Physics · Physics 2016-08-16 Piet O. Schmidt , Sven Hensler , Jörg Werner , Thomas Binhammer , Axel Görlitz , Tilman Pfau

We demonstrate direct cooling of gaseous formaldehyde (H2CO) to the microkelvin regime. Our approach, optoelectrical Sisyphus cooling, provides a simple dissipative cooling method applicable to electrically trapped dipolar molecules. By…

Atomic Physics · Physics 2016-02-19 Alexander Prehn , Martin Ibrügger , Rosa Glöckner , Gerhard Rempe , Martin Zeppenfeld

We investigate cooling mechanisms in magneto-optically and magnetically trapped erbium. We find efficient sub-Doppler cooling in our trap, which can persist even in large magnetic fields due to the near degeneracy of two Lande g factors.…

Atomic Physics · Physics 2009-09-29 Andrew J. Berglund , Siu Au Lee , Jabez J. McClelland

We propose a method for laser cooling and trapping a substantial class of polar molecules, and in particular titanium (II) oxide (TiO). This method uses pulsed electric fields to nonadiabatically remix the ground-state magnetic sublevels of…

Atomic Physics · Physics 2008-12-13 Benjamin K. Stuhl , Brian C. Sawyer , Dajun Wang , Jun Ye

Analogous to the extension of laser cooling techniques from two-level to three-level atoms, Doppler cooling of molecules with an intermediate electronic state is considered. In particular, we use a rate-equation approach to simulate cooling…

Atomic Physics · Physics 2015-03-17 J. H. V. Nguyen , B. Odom

We present the first experimental demonstration of radiation pressure force deflection and direct laser cooling for barium monohydride (BaH) molecules resulting from multiple photon scattering. Despite a small recoil velocity (2.7 mm/s) and…

We present a robust, continuous molecular decelerator that employs high magnetic fields and few optical pumping steps. CaOH molecules are slowed, accumulating at low velocities in a range sufficient for loading both magnetic and…

Cooling of molecules via free-space dissipative scattering of photons is thought not to be practicable due to the inherently large number of Raman loss channels available to molecules and the prohibitive expense of building multiple…

We propose to sympathetically slow and cool polar molecules in a cold, low-density beam using laser-cooled Rydberg atoms. The elastic collision cross sections between molecules and Rydberg atoms are large enough to efficiently thermalize…

Recent work with laser-cooled molecules in attractive optical traps has shown that the differential AC Stark shifts arising from the trap light itself can become problematic, limiting collisional shielding efficiencies, rotational coherence…

Atomic Physics · Physics 2022-06-08 Yukai Lu , Connor M. Holland , Lawrence W. Cheuk

The development of laser cooling coupled with the ability to trap atoms and ions in electromagnetic fields, has revolutionised atomic and optical physics, leading to the development of atomic clocks, high-resolution spectroscopy and…

We present a magnetically enhanced laser cooling scheme applicable to multi-level type-II transitions and further diatomic molecules with adiabatic transfer. An angled magnetic field is introduced to not only remix the dark states, but also…

Atomic Physics · Physics 2019-05-07 Qian Liang , Tao Chen , Wenhao Bu , Yuhe Zhang , Bo Yan

Laser cooling of alkali atoms typically requires time-varying magnetic fields, introducing unwanted coupling between atom preparation and coherent operations. Here we demonstrate sub-Doppler laser cooling and optical transport of alkali…

We present an opto-electrical cooling scheme for polar molecules based on a Sisyphus-type cooling cycle in suitably tailored electric trapping fields. Dissipation is provided by spontaneous vibrational decay in a closed level scheme found…

Quantum Physics · Physics 2009-10-07 M. Zeppenfeld , M. Motsch , P. W. H. Pinkse , G. Rempe

Current dual-frequency magneto-optical traps for ultracold molecules are plagued by sub-Doppler heating effects, making them vastly inferior to standard atomic MOTs. Here we demonstrate theoretically that the sub-Doppler effects in such a…

Atomic Physics · Physics 2023-04-06 S. Xu , P. Kaebert , M. Stepanova , T. Poll , M. Siercke , S. Ospelkaus

The general idea that optical radiation may cool matter was put forward by Pringsheim already in 1929. Doppler cooling of dilute atomic gases is an extremely successful application of this concept, and more recently anti-Stokes cooling in…

Quantum Gases · Physics 2015-05-13 Ulrich Vogl , Martin Weitz

Ultracold atoms at temperatures close to the recoil limit have been achieved by extending Doppler cooling to forbidden transitions. A cloud of ^40Ca atoms has been cooled and trapped to a temperature as low as 6 \mu K by operating a…

Atomic Physics · Physics 2015-11-30 T. Binnewies , G. Wilpers , U. Sterr , F. Riehle , J. Helmcke , T. E. Mehlstäubler , E. M. Rasel , W. Ertmer

We propose a general method to cool the translational motion of molecules. Our method is an extension of single photon atomic cooling which was successfully implemented in our laboratory. Requiring a single event of absorption followed by a…

Chemical Physics · Physics 2015-05-13 Edvardas Narevicius , S. Travis Bannerman , Mark G. Raizen

There is substantial interest in producing samples of ultracold molecules for possible applications in quantum computation, quantum simulation of condensed matter systems, precision measurements, controlled chemistry, and high precision…

Atomic Physics · Physics 2013-05-30 J. F. Barry , E. S. Shuman , E. B. Norrgard , D. DeMille