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Related papers: Laser-coolable polyatomic molecules with heavy nuc…

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When laser radiation is skilfully applied, atoms and molecules can be cooled allowing precise measurements and control of quantum systems. This is essential in fundamental studies of physics as well as practical applications such as…

We suggest a protocol for the sympathetic cooling of a molecular asymmetric top rotor co-trapped with laser-cooled atomic ions, based on resonant coupling between the molecular ion's electric dipole moment and a common normal mode of the…

Quantum Physics · Physics 2026-02-04 Monika Leibscher , Alexander Blech , Christiane P. Koch

Recent experiments have demonstrated direct cooling and trapping of diatomic and triatomic molecules in magneto-optical traps (MOTs). However, even the best molecular MOTs to date still have density $10^{-5}$ times smaller than in typical…

Atomic Physics · Physics 2023-04-19 Thomas K. Langin , David DeMille

We propose a generic approach to nonresonant laser cooling of atoms/molecules in a bistable optical cavity. The method exemplifies a photonic version of Sisyphus cooling, in which the matter-dressed cavity extracts energy from the particles…

Quantum Physics · Physics 2009-11-13 Mark Y. Vilensky , Yehiam Prior , Ilya Sh. Averbukh

Barium monohydride (BaH) is an attractive candidate for extending laser cooling and trapping techniques to diatomic hydrides. The apparatus and high-resolution optical spectroscopy presented here demonstrate progress toward this goal. A…

Atomic Physics · Physics 2017-08-08 G. Z. Iwata , R. L. McNally , T. Zelevinsky

We demonstrate a scheme for magneto-optically trapping strontium monofluoride (SrF) molecules at temperatures one order of magnitude lower and phase space densities three orders of magnitude higher than obtained previously with laser-cooled…

Atomic Physics · Physics 2016-02-17 E. B. Norrgard , D. J. McCarron , M. H. Steinecker , M. R. Tarbutt , D. DeMille

Since the advent of atom laser-cooling, trapping or cooling natural molecules has been a long standing and challenging goal. Here, we demonstrate a method for laser-trapping molecules that is radically novel in its configuration, in its…

Optics · Physics 2015-06-04 M. Alharbi , A. Husakou , B. Debord , F. Gerome , F. Benabid

We present a rigorous theoretical study of low-temperature collisions of polyatomic molecular radicals with ^1S_0 atoms in the presence of an external magnetic field. Accurate quantum scattering calculations based on ab initio and scaled…

Atomic Physics · Physics 2011-03-07 T. V. Tscherbul , H-G. Yu , A. Dalgarno

Only bosonic molecular species have been directly laser cooled to date, primarily due to an abundance of bosonic isotopes in nature and to their simpler hyperfine structure. Fermionic molecules provide new opportunities for ultracold…

Atomic Physics · Physics 2024-08-07 Jinyu Dai , Qi Sun , Benjamin C. Riley , Debayan Mitra , Tanya Zelevinsky

Laser cooling of translational motion of small molecules is performed by addressing transitions that ensure spontaneous emission cannot cause net rotational excitation. This will not be possible once the rotational splitting becomes…

Quantum Physics · Physics 2022-03-08 W. C. Campbell , B. L. Augenbraun

Single-photon cooling is a recently introduced method to cool atoms and molecules for which standard methods might not be applicable. We numerically examine this method in a two-dimensional wedge trap as well as in a two-dimensional…

Quantum Physics · Physics 2014-03-25 V. P. Singh , A. Ruschhaupt

We demonstrate laser cooling of barium monofluoride (138BaF) molecules. We use serrodynes to synthesize time-sequenced optical spectra that can be precisely tailored to the hyperfine structure of this heaviest non-radioactive alkaline earth…

It is shown that the translational degrees of freedom of a large variety of molecules, from light diatomic to heavy organic ones, can be cooled sympathetically and brought to rest (crystallized) in a linear Paul trap. The method relies on…

Quantum Physics · Physics 2009-11-10 S. Schiller , C. Laemmerzahl

We show that it is possible to cool interacting pairs of atoms by a lin $\perp$ lin Sisyphus-like laser cooling scheme using counter-propagating photoassociation (PA) lasers. It is shown that the center-of-mass motion (c.m.) of atom pairs…

Atomic and Molecular Clusters · Physics 2016-09-12 Subrata Saha , Somnath Naskar , Bimalendu Deb

In this work we investigate the theory for three different uni-directional population transfer schemes in trapped multilevel systems which can be utilized to cool molecular ions. The approach we use exploits the laser-induced coupling…

Quantum Physics · Physics 2010-01-27 C. Lazarou , M. Keller , B. M. Garraway

Laser cooling of large, complex molecules is a long-standing goal, instrumental for enabling new quantum technology and precision measurements. A primary consideration for the feasibility of laser cooling, which determines the efficiency…

The extension of laser cooling and trapping techniques to polyatomic molecular ions would have advanced scientific applications such as search of physics outside of the Standard Model, ultracold chemistry etc. We apply the Fock space…

We present a scheme for laser cooling applicable for an extremely dilute sample of magnetically trapped antihydrogen atoms($\bar{H}$). Exploiting and controlling the dynamical coupling between the $\bar{H}$'s motional degrees of freedom in…

Atomic Physics · Physics 2015-06-11 P. H. Donnan , M. C. Fujiwara , F. Robicheaux

Optical cycling transitions and direct laser cooling have recently been demonstrated for a number of alkaline-earth dimers and trimer molecules. This is made possible by diagonal Franck-Condon factors between the vibrational modes of the…

Chemical Physics · Physics 2020-04-08 Jacek Kłos , Svetlana Kotochigova

Following the bichromatic sub-Doppler cooling scheme on the D1 line of 40K recently demonstrated in (Fernandes et al. 2012), we introduce a similar technique for 7Li atoms and obtain temperatures of 60 uK while capturing all of the 5x10^8…

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