Related papers: Laser-coolable polyatomic molecules with heavy nuc…
We report on a cycling scheme for Doppler cooling of trapped OH$^+$ ions using transitions between the electronic ground state $X^3\Sigma^-$ and the first excited triplet state $A^3\Pi$. We have identified relevant transitions for photon…
We present a novel optical cooling scheme that relies on hyperfine dark states to enhance loading and cooling atoms inside deep optical dipole traps. We demonstrate a seven-fold increase in the number of atoms loaded in the conservative…
The helium dimer in its metastable triplet state is a promising candidate to be the first laser-cooled homonuclear molecule. An ultracold gas of He$_2^*$ would enable a new generation of precision measurements to test quantum…
Polyatomic molecules have rich structural features that make them uniquely suited to applications in quantum information science, quantum simulation, ultracold chemistry, and searches for physics beyond the Standard Model. However, a key…
We introduce a scheme for deep laser cooling of molecules based on robust dark states at zero velocity. By simulating this scheme, we show it to be a widely applicable method that can reach the recoil limit or below. We demonstrate and…
Atoms in spatially dependent light fields are attracted to local intensity maxima or minima depending on the sign of the frequency difference between the light and the atomic resonance. For light fields confined in open high-Q optical…
Molecular predissociation is the spontaneous, nonradiative bond breaking process that can occur upon excitation. In the context of laser cooling, predissociation is an unwanted consequence of molecular structure that limits the ability to…
Polyatomic molecules are projected to be powerful tools in searches for physics beyond the Standard Model (BSM), including new CP-violating (CPV) interactions and ultralight dark matter (UDM) particles. Certain degrees of freedom present in…
Molecules and atomic highly charged ions provide powerful low-energy probes of the fundamental laws of physics: Polar molecules possess internal fields suitable to enhance fundamental symmetry violation by several orders of magnitudes,…
We propose a new laser cooling method for atomic species whose level structure makes traditional laser cooling difficult. For instance, laser cooling of hydrogen requires single-frequency vacuum-ultraviolet light, while multielectron atoms…
We report on an apparatus for cooling and trapping of neutral dysprosium. We characterize and optimize the performance of our Zeeman slower and 2D molasses cooling of the atomic beam by means of Doppler spectroscopy on a 136 kHz broad…
Laser cooled atoms are central to modern precision measurements. They are also increasingly important as an enabling technology for experimental cavity quantum electrodynamics, quantum information processing and matter wave interferometry.…
We consider the use of pulse-shaped broadband femtosecond lasers to optically cool rotational and vibrational degrees of freedom of molecules. Since this approach relies on cooling rotational and vibrational quanta by exciting an electronic…
Doppler cooling with lasers is essential to ions' trapping and also a preliminary step towards achievement of ultracold ions. Due to lack of effective tools, experimentally monitoring the ions' temperature and the laser-ion coupling is…
We present a practical roadmap to achieve optical cycling and laser cooling of asymmetric top molecules (ATMs). Our theoretical analysis describes how reduced molecular symmetry, as compared to diatomic and symmetric non-linear molecules,…
We describe an approach to optically trapping small, chemically stable molecules at cryogenic temperatures by buffer-gas loading a deep optical dipole trap. The ~10 K trap depth will be produced by a tightly-focused, 1064-nm cavity capable…
Laser cooling is a powerful method to control molecules for applications in precision measurement, as well as quantum information, many-body physics, and fundamental chemistry. However, many optically-active metal centers in valence states…
Large, 3D trapped ion crystals offer improved sensitivity in quantum sensing protocols, and are expected to be implemented as platforms in near-future experiments. However, numerical techniques used to study the laser cooling of such…
Laser cooling is a key ingredient for quantum control of atomic systems in a variety of settings. In divalent atoms, two-stage Doppler cooling is typically used to bring atoms to the uK regime. Here, we implement a pulsed radial cooling…
We demonstrate rotational and vibrational cooling of cesium dimers by optical pumping techniques. We use two laser sources exciting all the populated rovibrational states, except a target state that thus behaves like a dark state where…