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Starting from weakly bound Feshbach molecules, we demonstrate a two-photon pathway to the dipolar ground state of bi-alkali molecules that involves only singlet-to-singlet optical transitions. This pathway eliminates the search for a…

We present a systematic investigation of the antiferromagnetic ordering and structural distortion for the series of Ba(Fe{1-x}Ru{x})2As2 compounds (0 <= x <= 0.246). Neutron and x-ray diffraction measurements demonstrate that, unlike for…

We calculate the microwave spectra of ultracold KRb alkali metal dimers, including hyperfine interactions and in the presence of electric and magnetic fields. We show that microwave transitions may be used to transfer molecules between…

Chemical Physics · Physics 2015-05-13 J. Aldegunde , Hong Ran , Jeremy M. Hutson

We present a combined high-resolution x-ray diffraction and x-ray resonant magnetic scattering (XRMS) study of as-grown BaFe2As2. The structural/magnetic transitions must be described as a two-step process. At T_S = 134.5 K we observe the…

Relativistic coupled-cluster calculations of the ionization potential, dissociation energy, and excited electronic states under 35,000 cm$^{-1}$ are presented for the actinium monofluoride (AcF) molecule. The ionization potential is…

Complex molecular structure demands customized solutions to laser cooling by extending its general set of principles and practices. Yttrium monoxide (YO) has unique intramolecular interactions. The Fermi-contact interaction dominates over…

Atomic Physics · Physics 2020-06-18 Shiqian Ding , Yewei Wu , Ian A. Finneran , Justin J. Burau , Jun Ye

In this research paper, we investigated the structural, electronic, and magnetic features of titanium atom substituting calciumatom in rock salt structure of CaS to explore the new dilute magnetic semiconductor compounds. The calculations…

Materials Science · Physics 2022-02-16 Meryem Ziati , Hamid Ez-Zahraouy

A model for determining the hyperfine structure of the excited electronic states of diatomic bialkali heteronuclear molecules is formulated from the atomic hyperfine interactions, and is applied to the case of bosonic $^{39}$KCs and…

The electronic structure of fluorite crystals are studied by means of density functional theory within the local density approximation for the exchange correlation energy. The ground-state electronic properties, which have been calculated…

Materials Science · Physics 2011-08-01 Emiliano Cadelano , Giancarlo Cappellini

Conventional theoretical studies on the ground-state laser cooling of a trapped ion have mostly focused on the weak sideband coupling (WSC) regime, where the cooling rate is inverse proportional to the linewidth of the excited state. In a…

Quantum Physics · Physics 2022-11-17 Shuo Zhang , Zhuo-Peng Huang , Tian-Ci Tian , Zheng-Yang Wu , Jian-Qi Zhang , Wan-Su Bao , Chu Guo

We report on the development and application of a parametrized crystal-field model for both C$_{1}$ symmetry centers in trivalent erbium-doped Y$_{2}$SiO$_{5}$. High resolution Zeeman and temperature dependent absorption spectroscopy was…

Materials Science · Physics 2022-06-22 N. L. Jobbitt , J. -P. R. Wells , M. F. Reid , S. P. Horvath , P. Goldner , A. Ferrier

X-ray diffraction experiments were performed on polycrystalline and single-crystal specimens of Ce$_{2}$Fe$_{17}$ at temperatures between 10 K and 300 K. Below $T_{\mathrm{t}}$ = 118$\pm$2 K, additional weak superstructure reflections were…

Thallium monofluoride (TlF) is a prime candidate molecule for precision measurements aimed at discovering new physics. Optical cycling on the B $\leftarrow$ X transition around 271 nm enhances this potential. Hyperfine resolved ultraviolet…

Chemical Physics · Physics 2024-09-09 Gerard Meijer , Boris G. Sartakov

We report spectroscopic results of the \(X^2\Sigma^+(v=2) \rightarrow A^2\Pi_{1/2}(v=1)\) transition in magnesium monofluoride (MgF). Using Doppler-free Laser-Induced Fluorescence (LIF) spectroscopy on the \(X^2\Sigma^+(v=2) \rightarrow…

Atomic Physics · Physics 2026-04-01 Youngju Cho , Yongwoong Lee , Kikyeong Kwon , Seunghwan Roh , Giseok Lee , Eunmi Chae

The vibrational branching ratios of SrOH for radiative decay to the ground electronic state, $X^{2}\Sigma^{+}$, from the first two electronically excited states, $A^{2}\Pi$ and $B^{2}\Sigma^{+}$, are determined experimentally at the…

Atomic Physics · Physics 2022-08-17 Zack Lasner , Annika Lunstad , Chaoqun Zhang , Lan Cheng , John M. Doyle

Supersonic beams of polar molecules are deflected using inhomogeneous electric fields. The quantum-state selectivity of the deflection is used to spatially separate molecules according to their quantum state. A detailed analysis of the…

We study the dynamics of polarizable particles coupled to a lossy cavity mode that are transversally driven by a laser. Our analysis is performed in the regime where the cavity linewidth exceeds the recoil frequency by several orders of…

Quantum Physics · Physics 2025-03-20 Simon B. Jäger

Radium compounds have attracted recently considerable attention due to both development of experimental techniques for high-precision laser spectroscopy of molecules with short-lived nuclei and amenability of certain radium compounds for…

We examine the prospects for utilizing the optical bichromatic force (BCF) to greatly enhance laser deceleration and cooling for near-cycling transitions in small molecules. We discuss the expected behavior of the BCF in near-cycling…

Atomic Physics · Physics 2015-05-30 M. A. Chieda , E. E. Eyler

By means of one-step model calculations the strong in-plane anisotropy seen in angle-resolved photoemission of the well-known iron pnictide prototype compounds BaFe$_2$As$_2$ and Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ in their low-temperature…

Superconductivity · Physics 2016-04-27 Gerald Derondeau , Jürgen Braun , Hubert Ebert , Ján Minár