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Interface effects on the ferroelectric behavior of PbTiO$_3$ ultrathin films deposited on SrTiO$_3$ substrate are investigated using an interatomic potential approach with parameters fitted to first-principles calculations. We find that the…

Materials Science · Physics 2009-11-11 M Sepliarsky , M. G. Stachiotti , R. L. Migoni

Above-bandgap femtosecond optical excitation of a ferroelectric/dielectric BaTiO3/CaTiO3 superlattice leads to structural responses that are a consequence of the screening of the strong electrostatic coupling between the component layers.…

Polarized neutron reflectivity measurements of a ferromagnetic [(LaMnO$_3$)$_{11.8}$/(SrMnO$_3$)$_{4.4}$]$_6$ superlattice reveal a modulated magnetic structure with an enhanced magnetization at the interfaces where LaMnO$_3$ was deposited…

Charge transfer in superlattices consisting of SrIrO$_3$ and SrMnO$_3$ is investigated using density functional theory. Despite the nearly identical work function and non-polar interfaces between SrIrO$_3$ and SrMnO$_3$, rather large charge…

Materials Science · Physics 2017-09-25 Satoshi Okamoto , John Nichols , Changhee Sohn , Soy Yeun Kim , Tae Won Noh , Ho Nyung Lee

The polar discontinuity at the SrTiO3/LaAlO3 interface (STO/LAO) can in principle sustain an electron density of 3.3E14 cm-2 (0.5 electrons per unit cell). However, experimentally observed densities are more than an order of magnitude…

Materials Science · Physics 2015-06-12 A. Janotti , L. Bjaalie , L. Gordon , C. G. Van de Walle

The recent observation of superconductivity at the interfaces between KTaO3 and EuO (or LaAlO3) offers a new example of emergent phenomena at oxide interfaces. This superconductivity exhibits an unusual strong dependence on the crystalline…

Superconductivity · Physics 2022-08-25 Tianshuang Ren , Miaocong Li , Xikang Sun , Lele Ju , Yuan Liu , Siyuan Hong , Yanqiu Sun , Qian Tao , Yi Zhou , Zhu-An Xu , Yanwu Xie

Quantum confinement at complex oxide interfaces establishes an intricate hierarchy of the strongly correlated $d$-orbitals which is widely recognized as a source of emergent physics. The most prominent example is the (001)…

Strongly Correlated Electrons · Physics 2019-05-15 A. M. R. V. L. Monteiro , M. Vivek , D. J. Groenendijk , P. Bruneel , I. Leermakers , U. Zeitler , M. Gabay , A. D. Caviglia

In oxide heterostructures, different materials are integrated into a single artificial crystal, resulting in a breaking of inversion-symmetry across the heterointerfaces. A notable example is the interface between polar and non-polar…

The interface between graphene and the ferroelectric superlattice $\mathrm{PbTiO_3/SrTiO_3}$ (PTO/STO) is studied. Tuning the transition temperature through the PTO/STO volume fraction minimizes the adsorbates at the graphene-ferroelectric…

Mesoscale and Nanoscale Physics · Physics 2014-08-27 Mohammed Humed Yusuf , Bent Nielsen , Matthew Dawber , Xu Du

Despite its simple structure and low degree of electronic correlation, SrTiO$_3$ (STO) features collective phenomena linked to charge transport and, ultimately, superconductivity, that are not yet fully explained. Thus, a better insight in…

Employing a first-principles and model Hamiltonian approach, we work out the electronic properties of polar-polar LaVO$_3$/KTaO$_3$ (LVO/KTO, 001) heterostrctures, with up to six layers of KTO and five layers of LVO. Our analyses indicate…

Materials Science · Physics 2024-08-02 Shubham Patel , Narayan Mohanta , Snehasish Nandy , Subhendra D. Mahanti , A Taraphder

In ABO3 perovskites, oxygen octahedron rotations are common structural distortions that can promote large ferroelectricity in BiFeO3 with an R3c structure [1], but suppress ferroelectricity in CaTiO3 with a Pbnm symmetry [2]. For many…

Materials Science · Physics 2016-04-05 Hongwei Wang , Jianguo Wen , Dean J. Miller , Qibin Zhou , Mohan Chen , Ho Nyung Lee , Karin M. Rabe , Xifan Wu

A combination of spectroscopic probes was used to develop a detailed experimental description of the transport and magnetic properties of superlattices composed of the paramagnetic metal CaRuO$_3$ and the antiferromagnetic insulator…

Strongly Correlated Electrons · Physics 2015-05-13 J. W. Freeland , J. Chakhalian , A. V. Boris , J. -M. Tonnerre , J. J. Kavich , P. Yordanov , S. Grenier , P. Popovich , H. N. Lee , B. Keimer

We report the emergence of a transverse dielectric response in PbTiO$_{3}$/SrTiO$_{3}$ superlattices hosting polar vortex structures. Using second-principles simulations, we find that an electric field applied along one direction induces…

Materials Science · Physics 2025-05-30 Fernando Gómez-Ortiz , Ramamoorthy Ramesh , Javier Junquera

Under various conditions of the growth process, when the presumably unconventional superconductor Sr$_2$RuO$_4$ (SRO) contains micro-inclusions of Ru metal, the superconducting critical temperature increases significantly. An STEM study…

Materials Science · Physics 2017-11-15 Soham S. Ghosh , Yan Xin , Zhiqiang Mao , Efstratios Manousakis

We report on the growth and properties of high quality bicolor oxide superlattices, composed of two perovskites out of BaTiO3, CaTiO3, and SrTiO3. The artificially grown superlattices are structurally unique and have a macroscopically…

Polar compensation can play an important role in the determination of interfacial electronic and magnetic properties in oxide heterostructures. Using x-ray absorption spectroscopy, x-ray magnetic circular dichroism, bulk magnetometry, and…

Using first-principles density functional theory calculations, we find a strong position and thickness dependence of the formation energy of oxygen vacancies in LaAlO3|SrTiO3 (LAO|STO) multilayers and interpret this with an analytical…

Materials Science · Physics 2010-11-01 Zhicheng Zhong , P. X. Xu , Paul J. Kelly

The possibility of controlling the interfacial properties of artificial oxide heterostructures is still attracting researchers in the field of materials engineering. Here, we used surface sensitive techniques and high-resolution…

Materials Science · Physics 2018-02-14 Santiago J. Carreira , Myriam H. Aguirre , Javier Briatico , Eugen Weschke , Laura B. Steren

Depositing disordered Al on top of SrTiO$_3$ is a cheap and easy way to create a two-dimensional electron system in the SrTiO$_3$ surface layers. To facilitate future device applications we passivate the heterostructure by a disordered…