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Magnetic multilayers of $(SrRuO_3)_m(SrMnO_3)_n$ were grown artificially using the pulsed laser deposition technique on (001)-oriented $SrTiO_3$ substrates. The state of strain at the interfaces and the structural coherency are studied in…

Strongly Correlated Electrons · Physics 2016-08-31 P. Padhan , W. Prellier , B. Mercey

Transition metal oxides display a great variety of quantum electronic behaviours where correlations often play an important role. The achievement of high quality epitaxial interfaces involving such materials gives a unique opportunity to…

The evolution of the atomic structure of LaAlO3 grown on SrTiO3 was investigated using surface x-ray diffraction in conjunction with model-independent, phase-retrieval algorithms between two and five monolayers film thickness. A…

Oxide heterointerfaces constitute a rich platform for realizing novel functionalities in condensed matter. A key aspect is the strong link between structural and electronic properties, which can be modified by interfacing materials with…

Materials Science · Physics 2021-07-09 T. C. van Thiel , J. Fowlie , C. Autieri , N. Manca , M. Šiškins , D. Afanasiev , S. Gariglio , A. D. Caviglia

We propose to insert TiO layers to perovskite ATiO$_{3}$ to form a superlattice and use first-principles calculations to investigate its basic properties. Our computational analysis shows that the structure, which consists of repeated…

Materials Science · Physics 2020-02-11 S. Raza , R. Zhang , N. Zhang , Z. Li , L. Liu , F. Zhang , D. Wang , C. -L. Jia

Diluted oxide interface of LaAl1-xMnxO/SrTiO3 (LAMO/STO) provides a new way of tuning the ground states of the interface between the two band insulators of LAO and STO from metallic/superconducting to highly insulating. Increasing the Mn…

Strongly Correlated Electrons · Physics 2019-10-02 Yulin Gan , Yu Zhang , Dennis V. Christensen , Nini Pryds , Yunzhong Chen

A two-dimensional electron gas (2DEG) forms at the interface of complex oxides like $SrTiO_{3}$ (STO) and $LaTiO_{3}$ (LTO), despite each material having a low native conductivity, as a band and a Mott insulator, respectively. The interface…

Controlling the coupling between localized spins and itinerant electrons can lead to exotic magnetic states. A novel system featuring local magnetic moments and extended 2D electrons is the interface between LaAlO3 and SrTiO3. The magnetism…

Strongly Correlated Electrons · Physics 2013-06-19 Arjun Joshua , J. Ruhman , S. Pecker , E. Altman , S. Ilani

Cuprate high temperature superconductors consist of two quasi-two-dimensional (2D) substructures: CuO2 superconducting layers and charge reservoir layers. The superconductivity is realized by charge transfer from the charge reservoir layers…

Superconductivity · Physics 2016-10-13 Lili Wang , Xucun Ma , Qi-Kun Xue

By employing first-principles electronic structure calculations we investigate nickelate superlattices [LaNiO$_3$]$_1$/[LaAlO$_3$]$_1$ and [LaNiO$_3$]$_1$/[SrTiO$_3$]$_1$ with (001) orientation under epitaxial tensile strain. Within density…

Strongly Correlated Electrons · Physics 2023-04-12 Heung-Sik Kim , Sang Hyeon Park , Myung Joon Han

Using {\it ab initio} density functional theory we explore the behavior of thin layers of metallic $d^4$ SrFeO$_3$ confined between the $d^0$ dielectric SrTiO$_3$ in a superlattice geometry. We find the presence of insulating SrTiO$_3$…

Materials Science · Physics 2010-02-24 James M. Rondinelli , Nicola A. Spaldin

Two-dimensional electron gas due to semiconductor interfaces can have high mobility and exhibits superconductivity, magnetism, and other exotic properties that are unexpected in constituent bulk materials. We study crystal structures,…

Materials Science · Physics 2019-06-13 Xue-Jing Zhang , Bang-Gui Liu

A fundamental understanding of the interplay between lattice structure, polarization and electrons is pivotal to the optical control of ferroelectrics. The interaction between light and matter enables the remote and wireless control of the…

LaNiO$_3$ (LNO) is an intriguing member of the rare-earth nickelates in exhibiting a metal-insulator transition for a critical film thickness of about 4 unit cells [Son et al., Appl. Phys. Lett. 96, 062114 (2010)]; however, such thin films…

First principles calculations reveal that adding a metallic overlayer on LaAlO3/SrTiO3(001) eliminates the electric field within the polar LaAlO3 film and thus suppresses the thickness-dependent insulator-to-metal transition observed in…

Materials Science · Physics 2012-03-23 V. G. Ruiz López , R. Arras , W. E. Pickett , R. Pentcheva

Driven quantum materials with on demand properties controlled by external stimuli are critical for emergent quantum technology. In optically tunable superconducting heterostructures, the lattice responses at the buried interface may hold…

Catalytic conversion of CO$_2$ into useful chemicals is an attractive alternative to expensive physical carbon sequestration methods. However, this approach is challenging because current chemical conversion methods employ high temperatures…

Chemical Physics · Physics 2015-07-30 Babatunde Alawode , Alexie Kolpak

The interface between the insulators LaAlO$_3$ and SrTiO$_3$ accommodates a two-dimensional electron liquid (2DEL) -- a high mobility electron system exhibiting superconductivity as well as indications of magnetism and correlations. While…

Strongly Correlated Electrons · Physics 2021-06-24 R. J. Green , V. Zabolotnyy , M. Zwiebler , Z. Liao , S. Macke , R. Sutarto , F. He , M. Huijben , G. Rijnders , G. Koster , J. Geck , V. Hinkov , G. A. Sawatzky

The emerging field of complex oxide interfaces is generically built on one of the most celebrated substrates - strontium titanate (SrTiO3). This material hosts a range of phenomena, including ferroelasticity, incipient ferroelectricity, and…

Mesoscale and Nanoscale Physics · Physics 2013-12-13 Maayan Honig , Joseph A. Sulpizio , Jonathan Drori , Arjun Joshua , Eli Zeldov , Shahal Ilani

The atomic-level control achievable in artificially-structured oxide superlattices provides a unique opportunity to explore interface phases of matter including high-density 2D electron gases. Electronic-structure calculations show that the…

Materials Science · Physics 2007-05-23 D. R. Hamann , D. A. Muller , H. Y. Hwang
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