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Recent experiments indicate that Na$_4$Ir$_3$O$_8$, a material in which s=1/2 iridium local moments form a three dimensional network of corner-sharing triangles, may have a quantum spin liquid ground state with gapless spin excitations.…

Strongly Correlated Electrons · Physics 2009-11-13 Michael Lawler , Arun Paramekanti , Yong Baek Kim , Leon Balents

We report gapless quantum spin liquid behavior in the layered triangular Sr$_{3}$CuSb$_{2}$O$_{9}$ (SCSO) system. X-ray diffraction shows superlattice reflections associated with atomic site ordering into triangular Cu planes well-separated…

The existence of a quantum spin liquid (QSL) in which quantum fluctuations of spins are sufficiently strong to preclude spin ordering down to zero temperature was originally proposed theoretically more than 40 years ago, but its…

Systematic pressure- and temperature-dependent infrared studies on the two-dimensional organic quantum spin-liquid $\beta^{\prime}$-EtMe$_3$Sb[Pd(dmit)$_2$]$_2$ disclose the electronic and lattice evolution across the Mott insulator-metal…

Strongly Correlated Electrons · Physics 2019-03-27 Weiwu Li , Andrej Pustogow , Reizo Kato , Martin Dressel

Quantum fluctuations originating phase competition or geometrical frustration of spins lead to novel states such as a quantum critical point and a quantum spin liquid where the strong quantum fluctuations suppress any ordered states even at…

Strongly Correlated Electrons · Physics 2019-11-28 Y. Saito , H. Nakamura , M. Sawada , T. Yamazaki , S. Fukuoka , N. Matsunaga , K. Nomura , M. Dressel , A. Kawamoto

We study the doping of a Mott insulator in the presence of quenched frustrating disorder in the magnetic exchange. A low doping regime $\delta<J/t$ is found, in which the quasiparticle coherent scale is low : $\epsilon_F^* = J…

Strongly Correlated Electrons · Physics 2016-08-31 Olivier Parcollet , Antoine Georges

A phenomenological description for confinement of fractionalized excitations is proposed in the gauge theory approach for doped Mott insulators. Introducing the Polyakov-loop parameter into an SU(2) gauge theory for the t-J model, we show…

Strongly Correlated Electrons · Physics 2009-12-11 Ki-Seok Kim , Hyun-Chul Kim

In this paper, we study the non-magnetic insulator state near Mott transition of 2D pi-flux Hubbard model on square lattice and find that such non-magnetic insulator state is quantum spin liquid state with nodal fermionic excitations -…

Strongly Correlated Electrons · Physics 2015-03-13 Su-Peng Kou , Lan-Feng Liu , Jing He , Ya-Jie Wu

It has long been believed that doped quantum spin liquids (QSLs) can give rise to fascinating quantum phases, including the possibility of high-temperature superconductivity (SC) as proposed by P. W. Anderson's resonating valence bond (RVB)…

Strongly Correlated Electrons · Physics 2024-04-09 Zheng-Tao Xu , Zheng-Cheng Gu , Shuo Yang

Inelastic neutron scattering is used to study the low-energy magnetic excitations in the spin-1 triangular lattice of the 6H-B phase of Ba$_3$NiSb$_2$O$_9$. We study two powder samples: Ba$_3$NiSb$_2$O$_9$ synthesized under high pressure…

Strongly Correlated Electrons · Physics 2017-02-08 B. Fak , S. Bieri , E. Canevet , L. Messio , C. Payen , M. Viaud , C. Guillot-Deudon , C. Darie , J. Ollivier , P. Mendels

We study the Mott transition from a metal to cluster Mott insulators in the 1/4- and 1/8-filled pyrochlore lattice systems. It is shown that such Mott transitions can arise due to charge localization in clusters or in tetrahedron units,…

Strongly Correlated Electrons · Physics 2014-11-11 Gang Chen , Hae-Young Kee , Yong Baek Kim

Discovery of novel spin-orbital entangled quantum ground states paves an important avenue for controllable quantum materials via unique couplings to the lattice and other external perturbations. In this work, motivated by recent experiments…

Strongly Correlated Electrons · Physics 2020-03-11 Adarsh S. Patri , Ilia Khait , Yong Baek Kim

In this article, we review some recent theoretical developments on potential high-temperature superconductors and unconventional metallic states that can arise from doping a spin-one Mott insulator in the $d^{8}$ valence. These studies are…

Strongly Correlated Electrons · Physics 2025-09-04 Hanbit Oh , Hui Yang , Ya-Hui Zhang

By using a high pressure, high temperature (HPHT) technique, the antiferromagnetically ordered ($T_N$ = 13.5 K) 6H-A phase of Ba$_3$NiSb$_2$O$_9$ was transformed into two new gapless quantum spin liquid(QSL) candidates with S=1 (Ni$^{2+}$)…

Strongly Correlated Electrons · Physics 2011-11-08 J. G. Cheng , G. Li , L. Balicas , J. S. Zhou , J. B. Goodenough , Cenke Xu , H. D. Zhou

Using tensor network states to unravel the physics of quantum spin liquids in minimal, yet generic microscopic spin or electronic models remains notoriously challenging. A prominent open question concerns the nature of the insulating ground…

Strongly Correlated Electrons · Physics 2020-10-22 Amir M Aghaei , Bela Bauer , Kirill Shtengel , Ryan V. Mishmash

The metal-organic-framework (MOF) compound Cu$_3$(HOTP)$_2$, a.k.a. Cu$_3$(HHTP)$_2$, is a small-gap semiconductor containing a kagome lattice of antiferromagnetically coupled $S$=1/2 Cu$^\mathrm{II}$ spins with intra-layer nearest-neighbor…

Strongly Correlated Electrons · Physics 2024-11-28 F. L. Pratt , D. Lopez-Alcala , V. Garcia-Lopez , M. Clemente-Leon , J. J. Baldovi , E. Coronado

We study the energetics of Gutzwiller projected BCS states of various symmetries for the triangular lattice antiferromagnet with a four particle ring exchange using variational Monte Carlo methods. In a range of parameters the energetically…

Strongly Correlated Electrons · Physics 2011-01-04 Tarun Grover , N. Trivedi , T. Senthil , Patrick A. Lee

Pressure-temperature phase diagram of the organic Mott insulator $\kappa$-(ET)$_2$Cu$_2$(CN)$_3$, a model system of the spin liquid on triangular lattice, has been investigated by $^1$H NMR and resistivity measurements. The spin-liquid…

Strongly Correlated Electrons · Physics 2007-05-23 Y. Kurosaki , Y. Shimizu , K. Miyagawa , K. Kanoda , G. Saito

The static and dynamic local spin susceptibility of the organic Mott insulator $\kappa$-(ET)$_2$Cu$_2$(CN)$_3$, a model material of the spin- 1/2 triangular lattice, is studied by $^{13}$C NMR spectroscopy from room temperature down to 20…

Strongly Correlated Electrons · Physics 2007-05-23 Yasuhiro Shimizu , Kazuya Miyagawa , Kazushi Kanoda , Maesato Mitsuhiko , Gunzi Saito

Quantum spin liquids are highly fascinating quantum liquids in which the spin degrees of freedom fractionalize. An interesting class of spin liquids are the exactly solvable, three-dimensional Kitaev spin liquids. Their fractionalized…

Strongly Correlated Electrons · Physics 2018-06-22 Stephanie Matern , Maria Hermanns