English

Doping a spin-one Mott insulator: possible application to bilayer nickelate

Strongly Correlated Electrons 2025-09-04 v1 Superconductivity

Abstract

In this article, we review some recent theoretical developments on potential high-temperature superconductors and unconventional metallic states that can arise from doping a spin-one Mott insulator in the d8d^{8} valence. These studies are particularly relevant-though not limited-to the recently discovered bilayer nickelate superconductor La3_3Ni2_2O7_7. We focus on a ferromagnetic (FM) Kondo lattice model with mobile electrons in the dx2y2d_{x^2-y^2} orbital coupled to the localized spin moments in dz2d_{z^2} orbital through a large Hund's coupling JHJ_H. In the large JHJ_H limit, the model reduces to the type II t-J model with a mixture of spin-half singlon states and spin-one doublon states. We summarize DMRG results on the Luther-Emery liquid in one dimensional chain and two-leg ladder. Then we mainly focus on bilayer square lattice and show that a large inter-layer coupling JJ_\perp of dz2d_{z^2} orbital can induce strong inter-layer pairing of dx2y2d_{x^2-y^2} orbital. In the strong JJ_\perp limit, a kinetic-energy driven high TcT_c superconductivity is demonstrated in an ideal model with only a single hopping term. Furthermore, the model predicts a symmetric pseudogap metal-dubbed `second Fermi liquid"-in the underdoped regime, yielding a phase diagram analogous to that of hole-doped cuprates. The bilayer Kondo model therefore, presents a promising platform for both realizing higher-Tc superconductors and exploring non-Fermi liquid physics. We also comment on the possible limitations of the current models for the bilayer nickelate material and point out some future directions.

Keywords

Cite

@article{arxiv.2509.02673,
  title  = {Doping a spin-one Mott insulator: possible application to bilayer nickelate},
  author = {Hanbit Oh and Hui Yang and Ya-Hui Zhang},
  journal= {arXiv preprint arXiv:2509.02673},
  year   = {2025}
}

Comments

Review paper submitted to Focus Issue in New Journal of Physics (https://iopscience.iop.org/collections/njp-241206-740); 17 pages, 10 figures

R2 v1 2026-07-01T05:18:00.790Z