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The spin-orbit coupling (SOC) interactions, electron correlation effects and Hund coupling cooperate and compete with each other, leading to novel properties, quantum phase and non-trivial topological electronic behavior in iridium oxides.…

Strongly Correlated Electrons · Physics 2018-12-19 Xing Ming , Xiangang Wan , Carmine Autieri , Jianfeng Wen , Xiaojun Zheng

Spin-orbit coupling (SOC) often gives rise to interesting electronic and magnetic phases in an otherwise ordinary pool of paramagnetic heavy metal oxides. In presence of strong SOC, assumed to be working in $j$-$j$ coupling regime, 5$d^4$…

The rich physics manifested by 5d oxides falls outside the Mott-Hubbard paradigm used to successfully explain the electronic and magnetic properties of 3d oxides. Much consideration has been given to the extent to which strong spin-orbit…

We employ first-principles density-functional theory, to perform a comparative investigation of the effect of the spin-orbit coupling (SOC) on the electronic and magnetic properties of three experimentally synthesized and characterized…

Strongly Correlated Electrons · Physics 2024-03-28 Roumita Roy , Sudipta Kanungo

Strong spin-orbit coupling (SOC) effects of heavy $d$-orbital elements have long been neglected in describing the ground states of their compounds thereby overlooking a variety of fascinating and yet unexplored magnetic and electronic…

In the context of correlated insulators, where electron-electron interactions (U) drive the localization of charge carriers, the metal-insulator transition (MIT) is described as either bandwidth (BC) or filling (FC) controlled. Motivated by…

Transition metal oxides exhibit various competing phases and exotic phenomena depending on how their reaction to the rich degeneracy of the $d$-orbital. Large spin-orbit coupling (SOC) reduces this degeneracy in a unique way by providing a…

$5d$ iridium oxides are of huge interest due to the potential for new quantum states driven by strong spin-orbit coupling. The strontium iridate Sr$_2$IrO$_4$ is particularly in the spotlight because of the so-called $j_\text{eff}=1/2$…

Iridates with the 5$d^4$ electronic configuration have attracted recent interest due to reports of magnetically-ordered ground states despite longstanding expectations that their strong spin-orbit coupling would generate a $J = 0$…

The combination of strong spin-orbit coupling and Coulomb interactions makes the $5d$ iridates a unique platform for realizing novel correlated electronic states. Here, utilizing infrared spectroscopy, we demonstrate that a robust Mott…

Strongly Correlated Electrons · Physics 2026-03-06 Kai Wang , Jun Yang , Chaoyang Kang , Weikang Wu , Wenka Zhu , Jianzhou Zhao , Yaomin Dai , Bing Xu

Analogs of the high-T$_c$ cuprates have been long sought after in transition metal oxides. Due to the strong spin-orbit coupling (SOC), the $5d$ perovskite iridates Sr$_2$IrO$_4$ exhibit a low-energy electronic structure remarkably similar…

Strongly Correlated Electrons · Physics 2017-10-26 Sen Zhou , Kun Jiang , Hua Chen , Ziqiang Wang

The Jeff=1/2 state is manifested in systems with large cubic crystal field splitting and spin-orbit coupling that are comparable to the on-site Coulomb interaction, U. 5d transition metal oxides host parameters in this regime and strong…

Strongly Correlated Electrons · Physics 2014-02-18 S. Calder , G. -X Cao , S. Okamoto , J. W. Kim , V. R. Cooper , Z. Gai , B. C. Sales , M. D. Lumsden , D. Mandrus , A. D. Christianson

Sr2IrO4 is a magnetic insulator driven by spin-orbit interaction (SOI) whereas the isoelectronic and isostructural Sr2RhO4 is a paramagnetic metal. The contrasting ground states have been shown to result from the critical role of the strong…

Strongly Correlated Electrons · Physics 2012-09-07 T. F. Qi , O. B. Korneta , L. Li , K. Butrouna , V. S. Cao , Xiangang Wan , P. Schlottmann , R. K. Kaul , G. Cao

We investigate the magnetic properties of the series Sr2Ir1-xRuxO4 with neutron, resonant x-ray and magnetization measurements. The results indicate an evolution and coexistence of magnetic structures via a spin flop transition from…

Investigation of elementary excitations has advanced our understanding of many-body physics governing most physical properties of matter. Recently spin-orbit excitons have drawn much attention, whose condensates near phase transitions…

Strongly Correlated Electrons · Physics 2019-07-24 A. Nag , S. Bhowal , M. Moretti Sala , A. Efimenko , I. Dasgupta , S. Ray

We have carried out a detailed first-principles study of a d$^{4.5}$ quaternary iridate Ba$_3$YIr$_2$O$_9$ both in its 6H-perovskite-type ambient pressure (AP) phase and also for the high pressure (HP) cubic phase. Our analysis reveals that…

Strongly Correlated Electrons · Physics 2015-11-11 S. K. Panda , S. Bhowal , Ying Li , S. Ganguly , Roser Valentí , L. L. Nordström , I. Dasgupta

To efficiently manipulate magnetism is a key physical issue for modern condensed matter physics, which is also crucial for magnetic functional applications. Most previous relevant studies rely on the tuning of spin texture, while the spin…

Strongly Correlated Electrons · Physics 2020-11-04 Yakui Weng , Xing'ao Li , Shuai Dong

The 5d iridates have been the subject of much recent attention due to the predictions of a large array of novel electronic phases driven by twisting strong spin-orbit coupling and Hubbard correlation. As a prototype, the single layered…

Materials Science · Physics 2015-03-10 Chengliang Lu , Shuai Dong , Andy Quindeau , Daniele Preziosi , Ni Hu , Marin Alexe

We study possible superconductivity in a carrier-doped iridium oxide insulator Sr$_{2}$IrO$_{4}$ based on an effective $t_{2g}$ three-orbital Hubbard model on the square lattice with a large spin-orbit coupling (SOC). Numerically solving…

Superconductivity · Physics 2019-09-02 Kazutaka Nishiguchi , Tomonori Shirakawa , Hiroshi Watanabe , Ryotaro Arita , Seiji Yunoki

We investigated electronic structure of 5d transition-metal oxide Sr2IrO4 using angle-resolved photoemission, optical conductivity, and x-ray absorption measurements and first-principles band calculations. The system was found to be well…

Strongly Correlated Electrons · Physics 2009-11-13 B. J. Kim , Hosub Jin , S. J. Moon , J. -Y. Kim , B. -G. Park , C. S. Leem , Jaeju Yu , T. W. Noh , C. Kim , S. -J. Oh , J. -H. Park , V. Durairaj , G. Cao , E. Rotenberg
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