English

Correlation effects and hidden spin-orbit entangled electronic order in parent and electron-doped iridates Sr$_2$IrO$_4$

Strongly Correlated Electrons 2017-10-26 v4

Abstract

Analogs of the high-Tc_c cuprates have been long sought after in transition metal oxides. Due to the strong spin-orbit coupling (SOC), the 5d5d perovskite iridates Sr2_2IrO4_4 exhibit a low-energy electronic structure remarkably similar to the cuprates. Whether a superconducting state exists as in the cuprates requires understanding the correlated spin-orbit entangled electronic states. Recent experiments discovered hidden order in the parent and electron doped iridates, some with striking analogies to the cuprates, including Fermi surface pockets, Fermi arcs, and pseudogap. Here, we study the correlation and disorder effects in a five-orbital model derived from the band theory. We find that the experimental observations are consistent with a dd-wave spin-orbit density wave order that breaks the symmetry of a joint two-fold spin-orbital rotation followed by a lattice translation. There is a Berry phase and a plaquette spin flux due to spin procession as electrons hop between Ir atoms, akin to the intersite SOC in quantum spin Hall insulators. The associated staggered circulating Jeff=1/2J_\text{eff}=1/2 spin current can be probed by advanced techniques of spin-current detection in spintronics. This electronic order can emerge spontaneously from the intersite Coulomb interactions between the spatially extended iridium 5d5d orbitals, turning the metallic state into an electron doped quasi-2D Dirac semimetal with important implications on the possible superconducting state suggested by recent experiments.

Keywords

Cite

@article{arxiv.1702.07070,
  title  = {Correlation effects and hidden spin-orbit entangled electronic order in parent and electron-doped iridates Sr$_2$IrO$_4$},
  author = {Sen Zhou and Kun Jiang and Hua Chen and Ziqiang Wang},
  journal= {arXiv preprint arXiv:1702.07070},
  year   = {2017}
}

Comments

8 pages, 4 figures + supplementary material (4 pages with 3 figures), published version