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Sr2IrO4 is a prototype of the class of Mott insulators in the strong spin-orbit interaction (SOI) limit described by a $J_{\mathrm{eff}}=1/2$ ground state. In Sr2IrO4, the strong SOI is predicted to manifest itself in the slaving of the…

Strongly Correlated Electrons · Physics 2013-09-30 S. Boseggia , H. C. Walker , J. Vale , R. Springell , Z. Feng , M. Moretti Sala , H. M. Rønnow , S. P. Collins , D. F. McMorrow

Sr2IrO4 is an archetypal spin-orbit-coupled Mott insulator with an antiferromagnetic state below 240 K. Here we report results of our study on single crystals of Sr2Ir1-xFexO4 (0<x<0.32) and Sr2Ir1-xCoxO4 (0<x<0.22). Fe doping retains the…

Strongly Correlated Electrons · Physics 2020-12-21 Bing Hu , Hengdi Zhao , Yu Zhang , Pedro Schlottmann , Feng Ye , Gang Cao

We report a single-crystal neutron diffraction study of the layered $\rm Sr_2IrO_4$. This work unambiguously determines the magnetic structure of the system and reveals that the spin orientation rigidly tracks the staggered rotation of the…

Strongly Correlated Electrons · Physics 2013-04-23 Feng Ye , Songxue Chi , Bryan C. Chakoumakos , Jaime A. Fernandez-Baca , Tongfei Qi , G. Cao

We show how an accurate first-principles treatment of the canted-antiferromagnetic ground state of Sr$_2$IrO$_4$, a prototypical $5d$ correlated spin-orbit coupled material, can be obtained without invoking any free parameters such as the…

Strongly Correlated Electrons · Physics 2020-04-13 Christopher Lane , Yubo Zhang , James W. Furness , Robert S. Markiewicz , Bernardo Barbiellini , Jianwei Sun , Arun Bansil

We report study of magnetization, resistivity, magnetoresistance and specific heat of the pyrochlore Iridate (Eu1-xNdx)2Ir2O7 with x=0.0, 0.5 and 1.0, where spin orbit coupling, electronic correlation, magnetic frustration and Kondo…

Strongly Correlated Electrons · Physics 2020-12-02 Sampad Mondal , M. Modak , B. Maji , M. K. Ray , S. Mandal , Swapan K. Mandal , M. Sardar , S. Banerjee

Muon-spin relaxation results on the pyrochlore iridate Nd$_2$Ir$_2$O$_7$ are reported. Spontaneous coherent muon-spin precession below the metal-insulator transition (MIT) temperature of about 33 K is observed, indicating the appearance of…

Strongly Correlated Electrons · Physics 2013-09-03 Hanjie Guo , Kazuyuki Matsuhira , Ikuto Kawasaki , Makoto Wakeshima , Yukio Hinatsu , Isao Watanabe , Zhu-an Xu

A new iridium containing layered cuprate material, IrSr_2Sm_{1.15}Ce_{0.85}Cu_{2.175}O_{10, has been synthesized by conventional ambient-pressure solid-state techniques. The material's structure has been fully characterized by Rietveld…

Materials Science · Physics 2012-09-22 R. H. Colman , A. C. Mclaughlin

We used resonant inelastic x-ray scattering to reveal the nature of magnetic interactions in Sr2IrO4, a 5d transition-metal oxide with a spin-orbit entangled ground state and Jeff=1/2 magnetic momemts, referred to as 'isospins'. The magnon…

It has recently been proposed that Na4Ir3O8 is a weak Mott insulator at ambient pressure, supporting a three-dimensional spin liquid phase with a spinon Fermi surface. This proposal is consistent with recent experimental findings that the…

Strongly Correlated Electrons · Physics 2013-05-29 Daniel Podolsky , Yong Baek Kim

We report an unusual magnetic ground state in single-crystal, double-perovskite Ba2YIrO6 and Sr doped Ba2YIrO6 with Ir5+(5d4) ions. Long-range magnetic order below 1.7 K is confirmed by DC magnetization, AC magnetic susceptibility and heat…

Strongly Correlated Electrons · Physics 2017-09-01 J. Terizc , H. Zheng , Feng Ye , H. D. Zhao , P. Schlottmann , L. De Long , G. Cao

In the pyrochlore iridates, \textit{R}$_{2}$Ir$_{2}$O$_{7}$ (\textit{R} = Lanthanide, Y), determination of the magnetic structure of the iridium moments remains an outstanding problem despite the role this is expected to play in the…

Strongly Correlated Electrons · Physics 2014-06-23 Steven M. Disseler

Using density functional theory and LDA+U method, we investigate magnetic and electronic structure of Y$_{2}$Ir$_{2}$O$_{7}$ and rare-earth based pyrochlore iridates. Our study reveals that the ground state is a non-collinear magnetic…

Materials Science · Physics 2010-03-18 Xiangang Wan , Jinming Dong , Sergey Y. Savrasov

Sr$_{3}$ZnIrO$_{6}$ is an effective spin one-half Mott insulating iridate belonging to a family of magnets which includes a number of quasi-one dimensional systems as well as materials exhibiting three dimensional order. Here we present the…

Strongly Correlated Electrons · Physics 2020-05-19 P. A. McClarty , A. D. Hillier , D. T. Adroja D. D. Khalyavin , S. Rayaprol , P. Manuel , W. Kockelmann , E. V. Sampathkumaran

Recent years have seen many examples of how the strong spin-orbit coupling (SOC) present in iridates can stabilize new emergent states that are difficult or impossible to realize in more conventional materials. In this review we outline a…

Strongly Correlated Electrons · Physics 2019-06-10 Lin Hao , D. Meyers , M. P. M. Dean , Jian Liu

Quantum magnets with significant bond-directional Ising interactions, so-called Kitaev materials, have attracted tremendous attention recently in the search for exotic spin liquid states. Here we present a comprehensive set of measurements…

We employ first-principles density-functional theory, to perform a comparative investigation of the effect of the spin-orbit coupling (SOC) on the electronic and magnetic properties of three experimentally synthesized and characterized…

Strongly Correlated Electrons · Physics 2024-03-28 Roumita Roy , Sudipta Kanungo

The intertwined charge, spin, orbital, and lattice degrees of freedom could endow 5d compounds with exotic properties. Current interest is focused on electromagnetic interactions in these materials, whereas the important role of lattice…

Spin-orbit coupling in heavy 5$d$ metal oxides, in particular, iridates have received tremendous interest in recent years due to the realization of exotic electronic and magnetic phases. Here, we report the synthesis, structural, magnetic,…

Strongly Correlated Electrons · Physics 2022-10-26 Harish Kumar , M. Köpf , A. Ullrich , M. Klinger , A. Jesche , C. A. Kuntscher

The 5d iridates have been the subject of much recent attention due to the predictions of a large array of novel electronic phases driven by twisting strong spin-orbit coupling and Hubbard correlation. As a prototype, the single layered…

Materials Science · Physics 2015-03-10 Chengliang Lu , Shuai Dong , Andy Quindeau , Daniele Preziosi , Ni Hu , Marin Alexe

We report the structural, magnetic and thermodynamic properties of the double perovskite compound La2CuIrO6 from X-ray, neutron diffraction, neutron depolarization, dc magnetization, ac susceptibility, specific heat, muon-spin-relaxation…