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Perovskite solid solutions PbHfO3-PbSnO3 offer valuable opportunities for studying the formation mechsnisms of incommensurate phases, owing to the presence of an intermediate (between cubic and incommensurate) phase, which is stabilized in…

We study the interplay of structural and polar distortions in hexagonal YMnO3 and short-period PbTiO3/SrTiO3 superlattices by means of first-principles calculations at constrained electric displacement field D. We find that in YMnO3 the…

Materials Science · Physics 2015-06-05 Massimiliano Stengel , Craig J. Fennie , Philippe Ghosez

Multiferroic hexagonal RMnO3 (R=rare earths) crystals exhibit dense networks of vortex lines at which six domain walls merge. While the domain walls can be readily moved with an applied electric field, the vortex cores were so far…

Materials Science · Physics 2015-06-19 Xueyun Wang , Maxim Mostovoy , Myung-Geun Han , Yoichi Horibe , T. Aoki , Yimei Zhu , Sang-Wook Cheong

The resistivity $\rho_{dc}$ of manganites is studied using a random-resistor-network, based on phase-separation between metallic and insulating domains. When percolation occurs, both as chemical composition and temperature vary, results in…

Strongly Correlated Electrons · Physics 2009-10-31 Matthias Mayr , Adriana Moreo , Jose A. Verges , Jeanette Arispe , Adrian Feiguin , Elbio Dagotto

Domain walls (DWs) in ferroic materials, across which the order parameter abruptly changes its orientation, can host emergent properties that are absent in the bulk domains. Using a broadband ($10^6-10^{10}$ Hz) scanning impedance…

Mesoscale and Nanoscale Physics · Physics 2018-03-30 Xiaoyu Wu , Urko Petralanda , Lu Zheng , Yuan Ren , Rongwei Hu , Sang-Wook Cheong , Sergey Artyukhin , Keji Lai

Ferroelectric domain walls are boundaries between regions with different polarization orientations in a ferroelectric material. Using first principles calculations, we characterize all different types of domain walls forming on…

Materials Science · Physics 2020-04-16 Đorđe Dangić , Éamonn D. Murray , Stephen Fahy , Ivana Savić

Nanostructured ferroelectrics display exotic multidomain configurations resulting from the electrostatic and elastic boundary conditions they are subject to. While the ferroelectric domains appear frozen in experimental images, atomistic…

Controlling the ferroelectricity and magnetism in multiferroic materials has been an important research topic. We report the formation of a highly polarized state in multiferroic DyMnO3 single crystals which develops well above the magnetic…

Materials Science · Physics 2014-09-05 Tao Zou , Zhiling Dun , Huibo Cao , Mengze Zhu , Daniel Coulter , Haidong Zhou , Xianglin Ke

Ferroelectrics are characterized by domain structures as are other ferroics. At the nanoscale though, ferroelectrics may exhibit non-trivial or exotic polarization configurations under proper electrostatic and elastic conditions. These…

Materials Science · Physics 2019-11-15 Saul Estandia , Florencio Sanchez , Matthew F. Chisholm , Jaume Gazquez

This work investigates the magnetically driven ferroelectricity in orthorhombic manganites RMnO3 (R=Gd, Dy or Tb) from the point of view of the symmetry. The method adopted generalizes the one used to characterize the polar properties of…

Materials Science · Physics 2009-11-13 J. L. Ribeiro

Ferroelectric domains are mesoscale structures that mediate between synchronized atomic-scale ion displacements and switchable macroscopic polarization. Here, we evaluated the randomness of the domain distribution at the onset of…

Materials Science · Physics 2024-02-06 Asaf Hershkovitz , Elangovan Hemaprabha , Doaa Khorshid , Liyang Ma , Shi Liu , Shai Cohen , Yachin Ivry

Improper ferroelectrics are described by two order parameters: a primary one, driving a transition to long-range distortive, magnetic or otherwise non-electric order, and the electric polarization, which is induced by the primary order…

The candidate magnetoelectric Pb3Mn7O15 has a structure consisting of 1/3 filled Kagome layers linked by ribbons of edge-sharing octahedra in the stacking direction. Previous reports have indicated a complex hexagonal-orthorhombic…

Strongly Correlated Electrons · Physics 2012-04-18 Simon A. J. Kimber

The lattice dynamics of the $\rm YMnO_3$ magneto-electric compound has been investigated using density functional calculations, both in the ferroelectric and the paraelectric phases. The coherence between the computed and experimental data…

Materials Science · Physics 2012-03-09 Julien Varignon , Sébastien Petit , Marie-Bernadette Lepetit

A detailed study of the electric field gradient (EFG) across the Pr1-xCaxMnO3 phase diagram and its temperature dependence is given. Clearly, distinct EFG behaviours for samples outside/inside the charge order (CO) region are observed. The…

Strongly Correlated Electrons · Physics 2009-11-13 A. M. L. Lopes , J. P. Araujo , V. S. Amaral , J. G. Correia , Y. Tomioka , Y. Tokura

The ferroelectric phase of the multiferroic hexagonal manganites (h-ReMnO3) has been reported to undergo a series of magnetic transitions involving long-range ordering/reorientation of 4fRe3+ and/or 3dMn3+ spins below room temperature.…

Hexagonal manganese oxides RMnO$_3$ show intriguing topological ferroelectric-domain walls with variable conductivity, leading to domain wall engineering. Despite the numerous experimental studies on the polar nanoscale structures,…

The commensurate and incommensurate magnetic structures of the magnetoelectric system YMn$_{2}$O$_{5}$, as determined from neutron diffraction, were found to be spin-density waves lacking a global center of symmetry. We propose a model,…

Materials Science · Physics 2009-11-11 L. C. Chapon , P. G. Radaelli , G. R. Blake , S. Park , S-W. Cheong

We show that the transition in AMnO3 from the orthorhombic perovskite phase to the hexagonal phase is promoted by inducing disorder on the A-site. The gap between the orthorhombic and the hexagonal phase is widened for disordered, mixed…

Strongly Correlated Electrons · Physics 2007-05-23 Jan-Willem Bos , Bas B. van Aken , Thomas T. M. Palstra

We demonstrate the formation of ferroelectric domain-wall polarons in a minimal two-dimensional lattice model of electrons interacting with rotating dipoles. Along the domain-wall, the rotors polarize in opposite directions, causing the…

Mesoscale and Nanoscale Physics · Physics 2025-03-20 Florian Kluibenschedl , Georgios M. Koutentakis , Ragheed Alhyder , Mikhail Lemeshko