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We report two examples of transport phenomena based on sharp features in the effective density of states of molecular-scale transistors: Kondo physics in C$_{60}$-based devices, and gate-modulated negative differential resistance (NDR) in…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 L. H. Yu , D. Natelson

Recent experiments have shown that transport properties of molecular-scale devices can be reversibly altered by the surrounding solvent. Here, we use a combination of first-principles calculations and experiment to explain this change in…

Mesoscale and Nanoscale Physics · Physics 2015-09-03 Michele Kotiuga , Pierre Darancet , Carlos R. Arroyo , Latha Venkataraman , Jeffrey B. Neaton

We investigate the thermopower of a metal-molecule-metal junction taking into account thermal effects on the junction. Based on analytical expressions and numerical simulations we show that the thermoelectric potential reveals valuable…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Dvira Segal

Proper design and manufacturing thermal bridges based on molecular junctions at the contact between graphene platelets or other thermally conductive nanoparticles would provide a fascinating way to produce efficient heat transport networks…

Materials Science · Physics 2017-11-07 Alessandro Di Pierro , Guido Saracco , Alberto Fina

For defining the conductance of single molecule junctions with a redox functionality in an electrochemical cell, two conceptually different electron transport mechanisms, namely coherent tunnelling and vibrationally induced hopping compete…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 Georg Kastlunger , Robert Stadler

Atomic and single-molecule junctions represent the ultimate limit to the miniaturization of electrical circuits. They are also ideal platforms to test quantum transport theories that are required to describe charge and energy transfer in…

Mesoscale and Nanoscale Physics · Physics 2013-08-01 Woochul Lee , Kyeongtae Kim , Wonho Jeong , Linda Angela Zotti , Fabian Pauly , Juan Carlos Cuevas , Pramod Reddy

We present an atomistic theory of electronic transport through single organic molecules that reproduces the important features of the current-voltage characteristics observed in recent experiments. We trace these features to their origin in…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 J. Heurich , J. C. Cuevas , W. Wenzel , G. Schoen

We study charge transport of a topological superconductor connected to different electromagnetic environments using a low-energy description where only the Majorana bound states in the superconductor are included. Extending earlier findings…

Mesoscale and Nanoscale Physics · Physics 2015-12-01 Konrad Wölms , Karsten Flensberg

This article reviews recent advances in low-temperature electronic thermal transport properties of thermally biased superconductor heterostructures focusing on the two-terminal transport. Since the last decade, ferromagnetism has been…

Superconductivity · Physics 2025-04-01 Paramita Dutta

We consider a model of a molecular junction made of BDT (benzene dithiol) molecule trapped between two Au(100) leads. Using the ab initio approach implemented in the SIESTA package we look for the optimal configuration of the molecule as a…

Materials Science · Physics 2015-06-25 Victor M. Garcia-Suarez , Tomasz Kostyrko , Steven Bailey , Colin Lambert , Bogdan R. Bulka

Metal-string complexes in the quasi-1D framework may play an important role in molecular electronics by serving not only as nanoscale interconnects but also as active functional elements for nanoelectronic devices. However, because of the…

Mesoscale and Nanoscale Physics · Physics 2020-01-03 Talem Rebeda Roy , Arijit Sen

Measurements of the thermal conductance of single-molecule junctions have recently been reported for the first time. It is presently unclear, how much the heat transport can be controlled through molecule-internal effects. The search for…

Mesoscale and Nanoscale Physics · Physics 2025-10-01 Matthias Blaschke , Fabian Pauly

We investigate phonon thermal transport of fullerene-based single-molecule junctions by employing classical molecular dynamics simulations. The thermal conductances of fullerene monomers, dimers, and trimers are computed through three…

Mesoscale and Nanoscale Physics · Physics 2024-02-12 Joanna Li , Jonathan J. Wang , Dvira Segal

We demonstrate a technique for creating high quality, large area tunnel junction barriers for normal-insulating- superconducting or superconducting-insulating-superconducting tunnel junctions. We use atomic layer depo- sition and an…

Superconductivity · Physics 2013-03-28 Stephanie M. Moyerman , Guangyuan Feng , Lisa Krayer , Nathan Stebor , Brian G. Keating

Microtubule-based molecular motors often work in small groups to transport cargos in cells. A key question in understanding transport (and its regulation in vivo) is to identify the sensitivity of multiple-motor-based motion to various…

Biomolecules · Quantitative Biology 2016-10-06 Jing Xu , Zhanyong Shu , Stephen J. King , Steven P. Gross

A single molecule break junction device serves as a tunable model system for probing the many body Kondo state. The low-energy properties of this state are commonly described in terms of a Kondo model, where the response of the system to…

Strongly Correlated Electrons · Physics 2013-06-28 Gavin D. Scott , Douglas Natelson , Stefan Kirchner , Enrique Muñoz

Ambipolar charge carrier transport in Copper phthalocyanine (CuPc) is studied experimentally in field-effect transistors and metal-insulator-semiconductor diodes at various temperatures. The electronic structure and the transport properties…

Mesoscale and Nanoscale Physics · Physics 2015-03-13 C. Schuster , M. Kraus , A. Opitz , W. Brütting , U. Eckern

Atomic-sized lead (Pb) contacts are deposited and dissolved in an electrochemical environment, and their transport properties are measured. Due to the electrochemical fabrication process, we obtain mechanically unstrained contacts and…

Mesoscale and Nanoscale Physics · Physics 2010-09-21 F. -Q. Xie , F. Hüser , F. Pauly , Ch. Obermair , G. Schön , Th. Schimmel

Ab initio calculations of phenyl dithiol connected to Au, Ag, Pd, and Pt electrodes are performed using non-equilibrium Green's functions and density functional theory. For each metal, the properties of the molecular junction are considered…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 John W. Lawson , Charles W. Bauschlicher

We have investigated charge transport in ZnTPPdT-Pyr molecular junctions using the lithographic MCBJ technique at room temperature and cryogenic temperature (6K). We combined low-bias statistical measurements with spectroscopy of the…