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Within the Coulomb blockade regime, our study delves into the charge, spin, and thermoelectric transport characteristics in a benzene-based molecular nano-junction using the Pauli master equation and linear response theory. The charge- and…

Mesoscale and Nanoscale Physics · Physics 2024-01-17 Parbati Senapati , Prakash Parida

Redox molecular junctions are molecular conduction junctions that involve more than one oxidation state of the molecular bridge. This property is derived from the ability of the molecule to transiently localize transmitting electrons,…

Mesoscale and Nanoscale Physics · Physics 2013-06-21 Agostino Migliore , Abraham Nitzan

We investigate the dimerization and fusion of C60 molecules to form various C60 dimers when pushed against each other at several inter-molecular distances. We study the stability of this dimerized C60 molecule based on its binding strength…

Materials Science · Physics 2009-11-13 Narinder Kaur , K. Dharamvir , V. K. Jindal

We theoretically examine the effect of the coupling of the transport electrons to a vibrational mode of the molecule on the ac linear-response conductance of molecular junctions. Representing the molecule by a single electronic state, we…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 A. Ueda , O. Entin-Wohlman , A. Aharony

The present paper gives an elaborate theoretical description of a new molecular charge transport mechanism applying to a single molecule trapped between two macroscopic electrodes in a solid state device. It is shown by a Hubbard type model…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Per Hedegard , Thomas Bjornholm

Understanding electron transport processes in molecular wires connected between contacts is a central focus in the field of molecular electronics. Especially, the dephasing effect causing tunneling-to-hopping transition has great importance…

Mesoscale and Nanoscale Physics · Physics 2012-06-26 Daijiro Nozaki , Claudia Gomes da Rocha , Horacio M. Pastawski , Gianaurelio Cuniberti

We calculate the zero temperature conductance and characteristic correlation functions of a molecule with a center of mass (CM) motion which modulates couplings to the leads. In the first model studied, the CM vibrational mode is…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 J. Mravlje , A. Ramsak , T. Rejec

In the present work we theoretically study the length dependence of thermopower of a single-molecule junction with a chain-like molecular bridge of an arbitrary length using a tight-binding model. We analyze conditions bringing a nonlinear…

Mesoscale and Nanoscale Physics · Physics 2017-03-20 Natalya A. Zimbovskaya

We induce superconductivity by proximity effect in thin layers of gold and study the number of conduction channels which contribute to the current in one-atom contacts and atomic wires. The atomic contacts and wires are fabricated with a…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 G. Rubio-Bollinger , C. de las Heras , E. Bascones , N. Agrait , F. Guinea , S. Vieira

Routinely, experiments on tunneling molecular junctions report values of conductances ($G_{RT}$) and currents ($I_{RT}$) measured at room temperature. On the other side, theoretical approaches based on simplified models provide analytic…

Mesoscale and Nanoscale Physics · Physics 2023-05-17 Ioan Baldea

We present results of spin-unrestricted first-principles quantum transport for a gated C$_{60}$ molecule weakly contacted to Al electrodes, making emphasis on the role played by the electronic localization and the spin degree of freedom. As…

Materials Science · Physics 2007-05-23 J. J. Palacios

Transistors, regardless of their size, rely on electrical gates to control the conductance between source and drain contacts. In atomic-scale transistors, this conductance is exquisitely sensitive to single electrons hopping via individual…

In the present work we theoretically analyze thermoelectric transport in single-molecule junctions (SMJ) characterized by strong interactions between electrons on the molecular linkers and phonons in their nuclear environments where…

Mesoscale and Nanoscale Physics · Physics 2024-01-17 Natalya A. Zimbovskaya

Electron transport properties through single conjugated molecules sandwiched between two non-superconducting electrodes are studied by the use of Green's function technique. Based on the tight-binding model, we do parametric calculations to…

Mesoscale and Nanoscale Physics · Physics 2009-11-06 Santanu K. Maiti

We study the thermopower of a quantum dot weakly coupled to two reservoirs by tunnel junctions. At low temperatures the transport through the dot is suppressed by charging effects (Coulomb blockade). As a result the thermopower shows an…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 M. Turek , K. A. Matveev

Recently Smit et al. [Nature 419, 906 (2002)] have reported that a single hydrogen molecule can form a bridge between Pt electrodes, which has a conductance close to one quantum unit, carried by a single channel. We present density…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 J. Heurich , F. Pauly , J. C. Cuevas , W. Wenzel , Gerd Schoen

Electrically connected and plasmonically enhanced molecular junctions combine the optical functionalities of high field confinement and enhancement (cavity function), and of high radiative efficiency (antenna function) with the electrical…

We report low-temperature measurements of the electrical transport properties of few-atom contacts of the superconducting metal zinc, arranged with lithographically fabricated mechanically controllable breakjunctions (MCB). The conductance…

Mesoscale and Nanoscale Physics · Physics 2016-08-31 A. Mayer-Gindner , H. v. Löhneysen , E. Scheer

Structural disorder is present in almost all experimental measurements of electronic transport through single molecules or molecular wires. To assess its influence on the conductance is computationally demanding, because a large number of…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 R. Maul , W. Wenzel

We study the variation of electron transmission through Au-S-benzene-S-Au junctions and related systems as a function of the structure of the Au:S contacts. For junctions with semi-infinite flat Au(111) electrodes, the highly coordinated…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 A. Grigoriev , J. Skoeldberg , G. Wendin , Z. Crljen