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Related papers: Optical pump-probe studies of carrier dynamics in …

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Ultrafast pump-probe measurements of plasmonic nanostructures probe the non-equilibrium behavior of excited carriers, which involves several competing effects obscured in typical empirical analyses. Here we present pump-probe measurements…

We show that, in optical pump-probe experiments on bulk samples, the statistical distribution of the intensity of ultrashort light pulses after the interaction with a nonequilibrium complex material can be used to measure the time-dependent…

Strongly Correlated Electrons · Physics 2017-11-08 Francesco Randi , Martina Esposito , Francesca Giusti , Fulvio Parmigiani , Oleg Misochko , Daniele Fausti , Martin Eckstein

We developed a time-resolved force microscopy technique by integrating atomic force microscopy using a tuning-fork-type cantilever with the delay time modulation method for optical pump-probe light. We successfully measured the dynamics of…

We propose and demonstrate pump-probe spectroscopy of rubidium absorption which reveals the sub-Doppler hyperfine structure of the $^{5}$S$_{1/2} \leftrightarrow$ $^{5}$P$_{3/2}$ (D2) transitions. The counter propagating pump and probe…

Understanding and controlling the electronic as well as ro-vibrational motion and, thus, the entire chemical dynamics in molecules is the ultimate goal of ultrafast laser and imaging science. In photochemistry, laser-induced dissociation…

Spin preparation prior to a free-induction-decay (FID) measurement can be adversely affected by transverse bias fields, particularly in the geophysical field range. A strategy that enhances the spin polarization accumulated before readout…

We describe an ultrafast time resolved pump-probe spectroscopy setup aimed at studying the switching of nanophotonic structures. Both fs pump and probe pulses can be independently tuned over broad frequency range between 3850 and 21050…

Optics · Physics 2010-11-02 Tijmen G. Euser , Philip J. Harding , Willem L. Vos

The influence of the phase fluctuation of the pump laser on the phase-correlation between the signal and idler modes of the output fields from as non-degenerate optical parametric oscillator operating above oscillation threshold was…

Quantum Physics · Physics 2009-11-13 Dong Wang , Yana Shang , Zhihui Yan , Wenzhe Wang , Xiaojun Jia , Changde Xie , Kunchi Peng

We present a femtosecond time-resolved optical spectroscopy (TRS) as an experimental tool to probe the changes in the low energy electronic density of states as a result of short and long range charge density wave order. In these…

Strongly Correlated Electrons · Physics 2007-05-23 J. Demsar , D. Mihailovic , V. V. Kabanov , K. Biljakovic

We theoretically study dynamical excitonic condensates occurring in bilayers with an imposed chemical potential difference and in photodoped semiconductors. We show that optical spectroscopy can experimentally identify phase-trapped and…

Strongly Correlated Electrons · Physics 2024-10-30 Alexander Osterkorn , Yuta Murakami , Tatsuya Kaneko , Zhiyuan Sun , Andrew J. Millis , Denis Golež

We employ ultra-broadband terahertz-midinfrared probe pulses to characterize the optical response of photoinduced charge-carrier plasmas in high-resistivity silicon in a reflection geometry, over a wide range of excitation densities…

Materials Science · Physics 2015-02-11 Fanqi Meng , Mark D. Thomson , Bo E. Sernelius , Michael Jörger , Hartmut G. Roskos

Time-resolved measurements of quantum dynamics are based on the availability of controlled events (e.g. pump and probe pulses) that are shorter in duration than the typical evolution time scale of the dynamical processes to be observed.…

Femtosecond core-level transient absorption spectroscopy is utilized to investigate photoinduced dynamics of the charge density wave in 1T-TiSe2 at the Ti M2,3 edge (30-50 eV). Photoexcited carriers and phonons are found to primarily induce…

Materials Science · Physics 2022-11-08 Tobias Heinrich , Hung-Tzu Chang , Sergey Zayko , Kai Rossnagel , Murat Sivis , Claus Ropers

We have extended the range of the high-pressure optical spectroscopy to the far-infrared region keeping the accuracy of ambient-pressure experiments. The newly-developed method offers a powerful tool for the study of pressure-induced phase…

Strongly Correlated Electrons · Physics 2014-01-15 I. Kezsmarki , R. Gaal , C. C. Homes , B. Sipos , H. Berger , S. Bordacs , G. Mihaly , L. Forro

Nonlinear optical properties and carrier relaxation dynamics in graphene, suspended in three different solvents, are investigated using femtosecond (80 fs pulses) Z-scan and degenerate pumpprobe spectroscopy at 790 nm. The results…

Materials Science · Physics 2015-05-14 Sunil Kumar , M. Anija , N. Kamaraju , K. S. Vasu , K. S. Subrahmanyam , A. K. Sood , C. N. R. Rao

We use optical pump--THz probe spectroscopy at low temperatures to study the hot carrier response in thin Bi$_2$Se$_3$ films of several thicknesses, allowing us to separate the bulk from the surface transient response. We find that for…

Mesoscale and Nanoscale Physics · Physics 2015-06-23 R. Valdés Aguilar , J. Qi , M. Brahlek , N. Bansal , A. Azad , J. Bowlan , S. Oh , A. J. Taylor , R. P. Prasankumar , D. A. Yarotski

We analyze the optical pump-probe reflection and transmission coefficients when the photoinduced response depends nonlinearly on the incident pump intensity. Under these conditions, we expect the photoconductivity depth profile to change…

Strongly Correlated Electrons · Physics 2024-10-30 Leya Lopez , Derek G. Sahota , J. Steven Dodge

The dynamics of small perturbations against the stationary density matrix of a pumped polariton system with only one photon polarization is studied. Depending on the way the system is pumped and probed, decay times ranging from 30 to 5000…

Mesoscale and Nanoscale Physics · Physics 2015-04-28 Augusto Gonzalez

We present time-resolved scanning x-ray microscopy measurements with picosecond photo-excitation via a tailored infrared pump laser at a scanning transmission x-ray microscope. Specifically, we image the laser-induced demagnetization and…

Two dimensional nanomaterials like Molybdenum disulfide have been drawing a lot of interest due to their excellent nonlinear optical response. In this research we study thermal lens formation in MoS2 nanoflakes dispersion using mode…