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Strong field ionization by circularly polarized laser fields from initial states with internal orbital momentum has interesting propensity rule: electrons counter-rotating with respect to the laser field can be liberated more easily than…

Atomic Physics · Physics 2015-12-16 Jivesh Kaushal , Felipe Morales , Olga Smirnova

In ultrafast experiments with gas phase molecules, the alignment of the molecular axis relative to the polarization of the interacting laser pulses plays a crucial role in determining the dynamics following this light-matter interaction.…

Chemical Physics · Physics 2025-04-14 Shashank Kumar , Eric Liu , Liang Z. Tan , Varun Makhija , Niranjan Shivaram

We theoretically demonstrate the possibility to tune the temporal waveform of optical unipolar pulses upon their coherent interaction with a multi-level resonant medium. This is achieved through the coherent control of the response of a…

We numerically investigate the use of strong THz radiation in assisting single attosecond pulse generation by few-cycle, 800 nm laser pulses. We optimize focusing conditions to generate short and powerful single attosecond pulses of…

Optics · Physics 2014-02-14 Emeric Balogh , Katalin Kovács , Valer Tosa , Katalin Varjú

High-order harmonic generation by few-cycle 800 nm laser pulses in neon gas in the presence of a strong terahertz (THz) field is investigated numerically with propagation effects taken into account. Our calculations show that the…

Intense attosecond magnetic field pulses are predicted to be produced by intense few cycle circularly polarized UV pulses. Numerical solutions of the time dependent Schr\"{o}dinger equation for H$_2^+$ are used to study the dynamical…

Optics · Physics 2013-07-24 Kai-Jun Yuan , Andre D. Bandrauk

We present high resolution two-photon excitation microscopy studies combining two-photon fluorescence (TPF) and second harmonic generation (SHG) in order to probe orientational distributions of molecular ensembles at room temperature. A…

Soft Condensed Matter · Physics 2007-05-23 Veronique Le Floc'h , Sophie Brasselet , Jean-Francois Roch , Joseph Zyss

Recent experiments on convection in binary mixtures have shown that the interaction between localized waves (pulses) can be repulsive as well as {\it attractive} and depends strongly on the relative {\it orientation} of the pulses. It is…

patt-sol · Physics 2009-10-28 Hermann Riecke

Measuring terahertz waveforms in terahertz spectroscopy often relies on electrooptic sampling employing a ZnTe crystal. Although the nonlinearities in such zincblende semiconductors induced by intense terahertz pulses have been studied at…

In Terahertz (THz) technology, one of the long-standing challenges has been the formation of intense pulses covering the hard-to-access frequency range of 1-15 THz (so-called THz gap). This frequency band, lying between the electronically…

Optics · Physics 2014-07-29 C. Vicario , B. Monoszlai , M. Jazbinsek , S. -H Lee , O. -P. Kwon , C. P. Hauri

A strong inhomogeneous static electric field is used to spatially disperse a supersonic beam of polar molecules, according to their quantum state. We show that the molecules residing in the lowest-lying rotational states can be selected and…

The spatial and spectral distributions of terahertz (THz) pulses emitted by two-color air plasmas are theoretically investigated for focused laser pulses and in the filamentation regime. We derive a so-called ''augmented'' conical emission…

Plasma Physics · Physics 2024-12-18 Alexandre Stathopulos , Stefan Skupin , Binbin Zhou , Peter U. Jepsen , Luc Bergé

Alignment and orientation of molecules by intense, ultrashort laser fields are crucial for a variety of applications in physics and chemistry. These include control of high harmonics generation, molecular orbitals tomography, control of…

We show, both classically and quantum mechanically, enantioselective orientation of gas phase chiral molecules excited by laser fields with twisted polarization. Counterintuitively, the induced orientation, whose direction is laser…

Chemical Physics · Physics 2019-10-16 Ilia Tutunnikov , Johannes Floß , Erez Gershnabel , Paul Brumer , Ilya Sh. Averbukh

We show that a 450 fs nonresonant, moderately intense, linearly polarized laser pulse can induce field-free molecular axis alignment of methyliodide molecules dissolved in a helium nanodroplet. Time-resolved measurements reveal rotational…

Chemical Physics · Physics 2015-06-12 Dominik Pentlehner , Jens H. Nielsen , Alkwin Slenczka , Klaus Mølmer , Henrik Stapelfeldt

We investigate rotational state changes in a single collision of diatomic molecular ions, polar or apolar, with an atomic ion. Rotational state changes may occur since the angular degree of freedom of the molecular ions interacts with the…

Quantum Physics · Physics 2026-04-20 J. Martin Berglund , Michael Drewsen , Christiane P. Koch

A moderately intense $450$ fs laser pulse is used to create rotational wave packets in gas phase $\rm{I_2}$ molecules. The ensuing time-dependent alignment, measured by Coulomb explosion imaging with a delayed probe pulse, exhibits the…

The availability of few-cycle optical pulses opens a window to physical phenomena occurring on the attosecond time scale. In order to take full advantage of such pulses, it is crucial to measure and stabilise their carrier-envelope (CE)…

Experimental results of direct measurement of resonant monochromatic terahertz emission optically excited in InGaAs transistor channels are presented. The emission is attributed to two-dimensional plasma waves excited by photogeneration of…

Mesoscale and Nanoscale Physics · Physics 2011-07-22 P. Nouvel , J. Torres , H. Marinchio , T. Laurent , C. Palermo , L. Varani , P. Shiktorov , E. Starikov , V. Gruzinskis , F. Teppe

Terahertz (THz)-based electron acceleration and manipulation has recently been shown to be feasible and to hold tremendous promise as a technology for the development of next-generation, compact electron sources. Previous work has…