Related papers: Molecular Orientation by Intense Single Cycle THz …
Direct imaging of molecular dynamics is a long-standing goal in physics and chemistry. As an emerging tool, high-harmonic spectroscopy (HHS) enables accessing molecular dynamics on femtosecond to attosecond time scales. However, decoding…
THz radiation allows for the controlled excitation of vibrational modes in molecules and crystals. We show that the circular motion of ions introduces inertial effects on electrons. In analogy to the classical Coriolis and centrifugal…
Terahertz (THz) emission by two-color, ultrashort optical pulses interacting with underdense helium gases at ultrahigh intensities ($> 10^{19}\,\mathrm{W/cm}^2$) is investigated by means of 3D particle-in-cell simulations. The THz field is…
Torque is ubiquitous in many molecular systems, including collisions, chemical reactions, vibrations, electronic excitations and especially rotor molecules. We present a straightforward theoretical method based on forces acting on atoms and…
Enantioselective orientation of chiral molecules excited by a shaped picosecond laser pulse and a delayed femtosecond pulse is considered. Using quantum mechanical simulations, we demonstrate a strong field-free enantioselective orientation…
We present a theoretical study of the mixed-field orientation of molecules without rotational symmetry. The time-dependent one-dimensional and three-dimensional orientation of a thermal ensemble of 6-chloropyridazine-3-carbonitrile…
Strong laser-induced magnetization of oxygen gas at room temperature and atmospheric pressure is achieved experimentally on the sub-nanosecond time scale. The method is based on controlling the electronic spin of paramagnetic molecules by…
We study the propagation effects of radio waves in a pulsar magnetosphere, composed of relativistic electron-positron pair plasmas streaming along the magnetic field lines and corotating with the pulsar. We critically examine the various…
We have performed terahertz (THz)-time domain spectroscopy in various geometries, for characterizing the directivity of THz waves emitted from groove-patterned InAs structures. First, we have distinguished the THz emission mechanisms as a…
The influence of large permanent dipoles on molecular orbital tomography via high-order harmonic generation (HHG) is investigated in this work. It is found that, owing to the modification of the angle-dependent ionization rate resulting…
A tilted-pulse-front pumped terahertz pulse source is proposed for the generation of extremely high field single-cycle terahertz pulses. The very simple and compact source consists of a single crystal slab having a blazed reflection grating…
A laser pulse composed of a fundamental and properly phased second harmonic exhibits an asymmetric electric field that can drive a time-dependent current of photoionized electrons. The current produces an ultrashort burst of terahertz (THz)…
We investigate the orientation dependence of Enhanced Ionization (EI) during strong-field-driven nuclear motion in acetylene (C$_2$H$_2$). Here, we both initiate and probe molecular dynamics in acetylene with intense 6-fs cross-polarized…
We study the strong-field interaction of a helical bi-chromatic pump with an anisotropic and inhomogeneous molecular system in the form of planar distribution of radially aligned molecular ensemble. This setting gives rise to macroscopic…
We study the orbital and spin dynamics of charge carriers induced by non-overlapping linearly polarized light pulses in semiconductor quantum wells (QWs). It is shown that such an optical excitation with coherent pulses leads to a spin…
Sub-cycle electromagnetic pulses in the Terahertz region are considered to be one of the best ways to orient molecules. The simplest option corresponds to half-cycles pulses in the sudden regime, for which the pulse duration is much shorter…
We demonstrate how dynamic Stark control (DSC) can be achieved on molecular photodissociation in the dipole limit, using single-cycle (FWHM) laser pulses in the terahertz (THz) regime. As the laser-molecule interaction follows the…
The field-free alignment and orientation of the linear molecule by the two-color trapezoidal laser pulses were theoretically investigated. The trapezoidal shape of a laser pulse allows to enhance the maximum alignment degree for the same…
Pumping n-type GaAs and InSb with ultrafast THz pulses having intensities higher than 150 MW/cm2 shows strong free carrier absorption saturation at temperatures of 300 K and 200 K respectively. If the energy imparted to the carriers exceeds…
We identify that both the dynamic core polarization and dynamic orbital deformation are important in the orientation-dependent high-harmonic generation of CO molecules subjected to intense few cycle laser fields. These polarization dynamics…