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The effect of magnetic STM-tip on electronic, magnetic and electronic transport properties through the molecule junction STM-tip-Co/CoPc/Co(111), has been investigated by mean of ab initio electronic structure calculations. The spin…

Quantum Physics · Physics 2025-02-25 Ali Jaafar , Tarek Khalil

The low temperature spin dynamics of a Fe8 Single-Molecule Magnet was studied under circularly polarized electromagnetic radiation allowing us to establish clearly photon-assisted tunneling. This effect, while linear at low power, becomes…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 L. Sorace , W. Wernsdorfer , C. Thirion , A. -L. Barra , M. Pacchioni , D. Mailly , B. Barbara

Single chlorophyll-a molecules, a vital resource for the sustenance of life on Earth, have been investigated by using scanning-tunneling-microscope manipulation and spectroscopy on a gold substrate at 4.6 K. The chlorophyll-a binds on…

Soft Condensed Matter · Physics 2009-11-11 Violeta Iancu , Saw-Wai Hla

Molecular spintronics hinges on the detailed understanding of electronic and magnetic properties of molecules interfaced with various materials. Here we demonstrate with ab-initio simulations that the prototypical Co-phthalocyanine (CoPc)…

Mesoscale and Nanoscale Physics · Physics 2021-05-26 Ana M. Montero , Filipe S. M. Guimarães , Samir Lounis

We clarify the macroscopic symmetry and microscopic model-parameter conditions for emergence of spin-split electronic band structure in collinear antiferromagnets without atomic spin-orbit coupling. By using the microscopic multipole…

Strongly Correlated Electrons · Physics 2019-11-12 Satoru Hayami , Yuki Yanagi , Hiroaki Kusunose

A simple double-decker molecule with magnetic anisotropy, nickelocene, is attached to the metallic tip of a low-temperature scanning tunneling microscope. In the presence of a Cu(100) surface, the conductance around the Fermi energy is…

Strongly Correlated Electrons · Physics 2017-05-18 M. Ormaza , P. Abufager , B. Verlhac , N. Bachellier , M. -L. Bocquet , N. Lorente , L. Limot

We consider theoretically transport in a spinfull one-channel interacting quantum wire placed in an external magnetic field. For the case of two point-like impurities embedded in the wire, under a small voltage bias the spin-polarized…

Strongly Correlated Electrons · Physics 2010-02-17 Zoran Ristivojevic , George I. Japaridze , Thomas Nattermann

The spin-crossover in organometallic molecules constitutes one of the most promising routes towards the realization of molecular spintronic devices. In this article, we explore the hybridization-induced spin-crossover in metal-organic…

Mesoscale and Nanoscale Physics · Physics 2020-01-08 Jakob Steinbauer , Silke Biermann , Sumanta Bhandary

Molecular nanomagnets show clear signatures of coherent behavior and have a wide variety of effective low-energy spin Hamiltonians suitable for encoding qubits and implementing spin-based quantum information processing. At the nanoscale,…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 Mircea Trif , Filippo Troiani , Dimitrije Stepanenko , Daniel Loss

We show that in the presence of ferromagnetic electronic reservoirs and spin-dependent tunnel couplings, molecular vibrations in nonmagnetic single molecular transistors induce an effective intramolecular exchange magnetic field. It…

Mesoscale and Nanoscale Physics · Physics 2015-07-29 S. Weiss , J. Brüggemann , M. Thorwart

Recent observations of considerable spin polarization in photoemission from metal surfaces through monolayers of chiral molecules were followed by several efforts to rationalize the results as the effect of spin-orbit interaction that…

Mesoscale and Nanoscale Physics · Physics 2015-06-16 Joel Gersten , Kristen Kaasbjerg , Abraham Nitzan

Tunneling of electrons through rotor-stator anthracene aldehyde molecular interfaces is studied with a combined ab initio and model approach. Molecular electronic structure calculated from first principles is utilized to model different…

Chemical Physics · Physics 2016-05-27 Irina Petreska , Vladimir Ohanesjan , Ljupco Pejov , Ljupco Kocarev

Spin-polarized scanning tunneling microscopy is used to investigate the magnetic state of the Fe monolayer on Re(0001). Two coexisting atomic-scale non-collinear spin textures are observed with a sharp transition between them on the order…

Strongly Correlated Electrons · Physics 2017-02-01 Alexandra Palacio-Morales , André Kubetzka , Kirsten von Bergmann , Roland Wiesendanger

We consider transport through a single-molecule magnet strongly coupled to metallic electrodes. We demonstrate that for half-integer spin of the molecule electron- and spin-tunneling \emph{cooperate} to produce both quantum tunneling of the…

Strongly Correlated Electrons · Physics 2009-11-11 C. Romeike , M. R. Wegewijs , W. Hofstetter , H. Schoeller

We study the model of a molecular switch comprised of a molecule with a soft vibrational degree of freedom coupled to metallic leads. In the presence of strong electron-ion interaction, different charge states of the molecule correspond to…

Mesoscale and Nanoscale Physics · Physics 2008-12-18 Fabio Pistolesi , Yaroslav M. Blanter , Ivar Martin

Spin-electronic devices are poised to become part of mainstream microelectronic technology .Downsizing them, however, faces the intrinsic difficulty that as ferromagnets become smaller, it becomes more difficult to stabilize their magnetic…

Control over quantum systems is typically achieved by time-dependent electric or magnetic fields. Alternatively, electronic spins can be controlled by spin-polarized currents. Here we demonstrate coherent driving of a single spin by a…

Mesoscale and Nanoscale Physics · Physics 2024-06-26 Stepan Kovarik , Richard Schlitz , Aishwarya Vishwakarma , Dominic Ruckert , Pietro Gambardella , Sebastian Stepanow

We coincidently measure the molecular frame photoelectron angular distribution and the ion sum-momentum distribution of single and double ionization of CO molecules by using circularly and elliptically polarized femtosecond laser pulses,…

Atomic Physics · Physics 2015-06-04 J. Wu , L. Ph. H. Schmidt , M. Kunitski , M. Meckel , S. Voss , H. Sann , H. Kim , T. Jahnke , A. Czasch , R. Dörner

In this paper we investigate the spin-resolved thermoelectric properties of strongly correlated molecular junctions in the linear response regime. The magnetic molecule is modeled by a single orbital level to which the molecular core spin…

Mesoscale and Nanoscale Physics · Physics 2021-05-25 Anand Manaparambil , Ireneusz Weymann

We present a general formulation of spin-dependent transport through a clean one-dimensional interacting quantum wire or carbon nanotube, connected to non-collinear ferromagnets via tunnel junctions. We show that the low energy description…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Leon Balents , Reinhold Egger