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In atoms spin-orbit coupling (SOC) cannot raise the angular momentum above a maximum value or lower it below a minimum. Here we show that this need not be the case in materials built from nanoscale structures including multi-nuclear…

Strongly Correlated Electrons · Physics 2017-03-15 A. L. Khosla , A. C. Jacko , J. Merino , B. J. Powell

We present measurements of magnetic tunnel junctions made using a self-assembled-monolayer molecular barrier. Ni/octanethiol/Ni samples were fabricated in a nanopore geometry. The devices exhibit significant changes in resistance as the…

Mesoscale and Nanoscale Physics · Physics 2010-10-05 J. R. Petta , S. K. Slater , D. C. Ralph

Spin-orbit coupling in crystals is known to lead to unusual direction dependent exchange interactions, however understanding of the consequeces of such effects in molecular crystals is incomplete. Here we perform four component relativistic…

Strongly Correlated Electrons · Physics 2017-04-19 A. C. Jacko , A. L. Khosla , J. Merino , B. J. Powell

We report on scanning tunneling microscopy (STM) topographs of individual metal phthalocyanines (MPc) on a thin salt (NaCl) film on a gold substrate, at tunneling energies within the molecule's electronic transport gap. Theoretical models…

Mesoscale and Nanoscale Physics · Physics 2023-10-24 Abhishek Grewal , Christopher C. Leon , Klaus Kuhnke , Klaus Kern , Olle Gunnarsson

We report the emergence of adsorption-induced magnetism from heterohelicene molecules on a non-magnetic Cu(100) surface. Spin-polarized low-energy electron microscopy (SP-LEEM) measurements reveal spin-dependent electron reflectivity for…

Understanding the fundamental mechanisms of optoelectronic excitation and relaxation pathways on the single-molecule level has only recently been started by combining scanning tunneling microscopy (STM) and spectroscopy (STS) with…

Quantum sensing is a key component of quantum technology, enabling highly sensitive magnetometry. We combined a nickelocene molecule with scanning tunneling microscopy to perform versatile spin sensing of magnetic surfaces, namely of model…

Mesoscale and Nanoscale Physics · Physics 2023-11-27 A. Fétida , O. Bengone , M. Romeo , F. Scheurer , R. Robles , N. Lorente , L. Limot

In recent years inelastic spin-flip spectroscopy using a lowtemperature scanning tunneling microscope has been a very successful tool for studying not only individual spins but also complex coupled systems. When these systems interact with…

Mesoscale and Nanoscale Physics · Physics 2015-10-21 Markus Ternes

A theory of resonant spin-dependent tunneling has been developed for symmetrical double-barrier structures grown of non-centrosymmetrical semiconductors. The dependence of the tunneling transparency on the spin orientation and the wave…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 M. M. Glazov , P. S. Alekseev , M. A. Odnoblyudov , V. M. Chistyakov , S. A. Tarasenko , I. N. Yassievich

Spin-orbit coupling (SOC) is a relativistic effect, where an electron moving in an electric field experiences an effective magnetic field in its rest frame. In crystals without inversion symmetry, it lifts the spin degeneracy and leads to…

Molecular bridges covalently bonded to two ferromagnetic electrodes can transform ferromagnetic materials and produce intriguing spin transport characteristics. This paper discusses the impact of molecule induced strong coupling on spin…

Materials Science · Physics 2019-12-04 Pawan Tyagi , Edward Friebe

We study theoretically spin relaxation during phonon-assisted tunneling of a single electron in self-assembled InAs/GaAs quantum-dot molecules formed by vertically stacked dots. We find that the spin-flip tunneling rate may be as high as 1%…

Mesoscale and Nanoscale Physics · Physics 2021-06-23 Michał Gawełczyk , Krzysztof Gawarecki

Characterization of the structural and electron transport properties of single chiral molecules provides critical insights into the interplay between their electronic structure and electrochemical environments, providing broader…

Chemical Physics · Physics 2024-09-26 Yueqing Shi , Liya Bi , Zihao Wang , Kangkai Liang , Ji-Kun Li , Xiao-Ye Wang , Wan-Lu Li , Shaowei Li

This article presents a review on the theoretical and the experimental developments on macroscopic quantum tunneling and phase transition of the escape rate in spin systems. We present the basic ideas with simplified calculations so that it…

Other Condensed Matter · Physics 2014-12-18 S. A. Owerre , M. B. Paranjape

Controlling electronic transport through a single-molecule junction is crucial for molecular electronics or spintronics. In magnetic molecular devices, the spin degree-of-freedom can be used to this end since the magnetic properties of the…

The spin-dependent transport of the electrons tunneling through a resonant tunneling structure with ferromagnetic multi-terminal under dc and ac fields is explored by means of the nonequilibrium Green function technique. A general…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Zhen-Gang Zhu , Gang Su , Qing-Rong Zheng , Biao Jin

A proper theoretical description of electronic structure of the 3d orbitals in the metal centers of functional metalorganics is a challenging problem. In this letter, we apply density functional theory and an exact diagonalization method in…

We consider spin-dependent tunneling through a gallium arsenide barrier, a material which has no inversion symmetry. We are dealing with free electrons, with one effective mass and a spin-splitting in the barrier material. When we take into…

Mesoscale and Nanoscale Physics · Physics 2009-09-29 T. L. Hoai Nguyen , Henri-Jean Drouhin , Jean-Eric Wegrowe , Guy Fishman

To explore the strength, isospin dependence, and density dependence of the in-medium spin-orbit coupling that is poorly known but relevant for understanding the structure of rare isotopes, the nucleon spin up-down differential transverse…

Nuclear Theory · Physics 2014-06-19 Yin Xia , Jun Xu , Bao-An Li , Wen-Qing Shen

We theoretically investigate inelastic transport through anisotropic magnetic molecules weakly coupled to one ferromagnetic and one nonmagnetic lead. We find that the current is suppressed over wide voltage ranges due to spin blockade. In…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 Florian Elste , Carsten Timm
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