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Molecules with unpaired spins (radicals) offer promising alternatives to closed-shell molecules as they are less limited regarding the spin statistics in their electroluminescence. Here, we combine scanning tunneling microscopy induced…

Mesoscale and Nanoscale Physics · Physics 2026-02-09 Vibhuti N. Rai , Christof Holzer , Carsten Rockstuhl , Wulf Wulfhekel , Lukas Gerhard

We consider electrical transport through molecules with Heisenberg-coupled spins arranged in a ring structure in the presence of an easy-axis anisotropy. The molecules are coupled to two metallic leads and a gate. In the charged state of…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Jörg Lehmann , Daniel Loss

Using Density functional theory and non-equilibrium Green's function formalism, spin dependent electron transport in Fe/Mo$_x$Cr$_{1-x}$S$_2$/Fe magnetic tunnel junction is studied. Spin transport for different thicknesses (1, 3, 5, and 7…

Materials Science · Physics 2026-01-06 Aloka Ranjan Sahoo , Sharat Chandra

Realization of spin crossover (SCO) based applications requires studying of spin state switching characteristics of SCO complex molecules at nanostructured environments especially on-surface. Except for a very few cases, the SCO of a…

An important consequence of the discovery of giant magnetoresistance in metallic magnetic multilayers is a broad interest in spin dependent effects in electronic transport through magnetic nanostructures. An example of such systems are…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 J. Barnas , I. Weymann

Using first-principles calculations, we show that the magnetic properties of a two-dimensional antiferromagnetic transition-metal surface are modified on the atomic scale by the adsorption of small organic molecules. We consider benzene…

Materials Science · Physics 2015-06-16 Nuala M. Caffrey , Paolo Ferriani , Simone Marocchi , Stefan Heinze

The ability to make electrical contact to single molecules creates opportunities to examine fundamental processes governing electron flow on the smallest possible length scales. We report experiments in which we controllably stretch…

Metallorganic molecules have been proposed as excellent spin filters in molecular spintronics because of the large spin-polarization of their electronic structure. However, most of the studies involving spin transport, have disregarded…

Mesoscale and Nanoscale Physics · Physics 2015-04-29 P. N. Abufager , R. Robles , N. Lorente

The excitation of the spin degrees of freedom of an adsorbed atom by tunneling electrons is computed using a strong coupling theory. The excitation process is shown to be a sudden switch between the initial state determined by the…

Mesoscale and Nanoscale Physics · Physics 2009-04-29 Nicolás Lorente Jean-Pierre Gauyacq

Spin dependent single electron tunneling in a ferromagnetic double junction is investigated theoretically in the limit of incoherent sequential tunneling. The junction consists of a small nonmagnetic metallic grain with discrete energy…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 G. Michalek , J. Martinek , J. Barnas , B. R. Bulka

The advent of two-dimensional (2D) crystals has led to numerous scientific breakthroughs. Conventional 2D systems have in-plane covalent bonds and a weak out-of-plane van-der-Waals bond. Here we report a new type of 2D material composed of…

Advances in molecular spintronics rely on the in-depth characterization of the molecular building blocks in terms of their electronic and, more importantly, magnetic properties. For this purpose, inert substrates that interact only weakly…

Applied Physics · Physics 2019-11-06 Emil Sierda , Micha Elsebach , Roland Wiesendanger , Maciej Bazarnik

We demonstrate spin polarized tunneling from Fe through a SiO2 tunnel barrier into a Si n-i-p heterostructure. Transport measurements indicate that single step tunneling is the dominant transport mechanism. The circular polarization, Pcirc,…

Materials Science · Physics 2015-05-14 C. H. Li , G. Kioseoglou , O. M. J. van t Erve , P. E. Thompson , B. T. Jonker

Quantum-well (QW) states in {\it nonmagnetic} metal layers contained in magnetic multilayers are known to be important in spin-dependent transport, but the role of QW states in {\it magnetic} layers remains elusive. Here we identify the…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Zhong-Yi Lu , X. -G. Zhang , Sokrates T. Pantelides

Spin-crossover (SCO) molecules are versatile magnetic switches with applications in molecular electronics and spintronics. Downscaling devices to the single-molecule level remains, however, a challenging task since the switching mechanism…

Spin properties of organic molecules have attracted great interest for their potential applications in spintronic devices and quantum computing. Fe-tetraphenyl porphyrin (FeTPP) is of particular interest for its robust magnetic properties…

Mesoscale and Nanoscale Physics · Physics 2022-10-19 Mingjun Zhong , Qimeng Wu , Liang Ma , Jie Li , Yifan Wang , Yansong Wang , Xin Li , Yajie Zhang , Jingtao Lü , Yongfeng Wang

We investigate transport and thermoelectric properties of hybrid systems based on a single-level quantum dot and one superconducting lead. The other lead is generally normal-metallic ferromagnet. In the latter case single-particle transport…

Mesoscale and Nanoscale Physics · Physics 2017-05-03 Piotr Trocha , Józef Barnaś

The inelastic portion of the tunnel current through an individual magnetic atom grants unique access to read out and change the atom's spin state, but it also provides a path for spontaneous relaxation and decoherence. Controlled closure of…

Mesoscale and Nanoscale Physics · Physics 2016-01-05 B. Bryant , R. Toskovic , A. Ferrón , J. L. Lado , A. Spinelli , J. Fernández-Rossier , A. F. Otte

Understanding the spin-texture behavior of boundary modes in ultrathin topological insulator films is critically essential for the design and fabrication of functional nano-devices. Here by using spin-resolved photoemission spectroscopy…

We present a systematic investigation of molecule-metal interactions for transition-metal phthalocyanines (TMPc, with TM = Fe, Co, Ni, Cu) adsorbed on Ag(100). Scanning tunneling spectroscopy and density functional theory provide insight…

Materials Science · Physics 2012-04-20 A. Mugarza , R. Robles , C. Krull , R. Korytar , N. Lorente , P. Gambardella