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Scanning tunneling microscopy combined with molecular dynamics simulations reveal a dislocation-mediated island diffusion mechanism for Cu on Ag(111), a highly mismatched system. Cluster motion is tracked with atomic precision at multiple…

Materials Science · Physics 2015-05-14 A. W. Signor , Henry H. Wu , Dallas R. Trinkle

We consider the influence of realistic island diffusion rates to homoepitaxial growth on metallic surfaces using a recently developed rate equation model which describes growth in the submonolayer regime with hyperthermal deposition. To…

Materials Science · Physics 2015-06-25 M. O. Jahma , M. Rusanen , A. Karim , I. T. Koponen , T. Ala-Nissila , T. S. Rahman

Monte Carlo simulations of an atomistic solid-on-solid model are used to study the effect of lattice misfit on the distribution of two-dimensional islands sizes as a function of coverage $\Theta$ in the submonolayer aggregation regime of…

Condensed Matter · Physics 2009-10-22 C. Ratsch , A. Zangwill , P. Šmilauer

The diffusion of two dimensional adatom islands (up to 100 atoms) on Cu(111) has been studied, using the self-learning Kinetic Monte Carlo (SLKMC) method [1]. A variety of multiple- and single-atom processes are revealed in the simulations,…

Materials Science · Physics 2015-05-30 Altaf Karim , Abdelkader Kara , Oleg Trushin , Talat S. Rahman

Surface reconstructions can drastically modify growth kinetics during initial stages of epitaxial growth as well as during the process of surface equilibration after termination of growth. We investigate the effect of activation barriers…

Condensed Matter · Physics 2009-10-31 J. Myslivecek , T. Jarolimek , P. Smilauer , B. Voigtlaender , M. Kaestner

We present Monte Carlo simulations for the size and temperature dependence of the diffusion coefficient of adatom islands on the Cu(100) surface. We show that the scaling exponent for the size dependence is not a constant but a decreasing…

Materials Science · Physics 2009-10-31 J. Heinonen , I. Koponen , J. Merikoski , T. Ala-Nissila

Square lattice gas models for heteroepitaxial growth are studied by means of kinetic Monte Carlo simulations, in order to find a possible origin of anisotropic island shape observed in growth experiments of long organic molecules. When…

Materials Science · Physics 2009-11-13 Yukio Saito , Ryo Kawasaki

We describe a theoretical study of the role of adsorbate interactions in island nucleation and growth, using Ag/Pt(111) heteroepitaxy as an example. From density-functional theory, we obtain the substrate-mediated Ag adatom pair interaction…

Materials Science · Physics 2009-10-31 Kristen A. Fichthorn , Matthias Scheffler

Effect of an anisotropic detachment on a heteroepitaxial island shape is studied by means of a kinetic Monte Carlo simulation of a square lattice gas model. Only with molecular deposition followed by surface diffusion, islands grow in a…

Materials Science · Physics 2007-07-20 Yukio Saito , Ryo Kawasaki

We investigate the influence of intermixing on heteroepitaxial growth dynamics, using a two-dimensional point island model, expected to be a good approximation in the early stages of epitaxy. In this model, which we explore both…

Statistical Mechanics · Physics 2015-06-22 K. I. Mazzitello , L. M. Delgado , J. L. Iguain

Diffusion of small two dimensional Cu islands (containing up to 10 atoms) on Cu(111) has been studied using the newly developed self-learning Kinetic Monte Carlo SLKMC method. It is based on a database of diffusion processes and their…

The properties of a particle diffusing on a one-dimensional lattice where at each site a random barrier and a random trap act simultaneously on the particle are investigated by numerical and analytical techniques. The combined effect of…

Condensed Matter · Physics 2009-10-28 Achille Giacometti , K. P. N. Murthy

We study one-dimensional models of particle diffusion and attachment/detachment from islands where the detachment rates gamma(m) of particles at the cluster edges increase with cluster mass m. They are expected to mimic the effects of…

Statistical Mechanics · Physics 2009-11-13 R. B. Stinchcombe , F. D. A. Aarão Reis

We use atomistic simulations with an empirical potential (EAM) to study the elastic effects of heteroepitaxial islands on adatom diffusion. We measure the diffusion barrier on pure stressed substrate and near a misfit island, as well as the…

Materials Science · Physics 2007-05-23 E. Somfai , L. M. Sander

The decay of hexagonal Ag adatom islands on top of larger Ag adatom islands on a Ag(111) surface is followed by a fast scanning tunneling microscope. Islands do not always show the expected increase in decay rate with decreasing island…

Other Condensed Matter · Physics 2009-11-11 Karina Morgenstern , Erik Lae gsgaard , Flemming Besenbacher

We simulated the growth of 2D islands with 2 kinds of diffusion atoms using the kinetic Monte- Carlo (kMC) method. As a result, we found that the slow atoms tend to create nuclei and determine the island volume distribution, along with…

Atomic and Molecular Clusters · Physics 2015-03-17 R. Yamauchi , X. M. Lu , M. Koyama , H. Sasakura , Y. Nakata , S. Muto

The steering effect on the growth of islands is investigated by combining molecular dynamics (MD) and kinetic Monte Carlo (KMC) simulations. Dynamics of depositing atoms and kinetics of atoms on a substrate are realized by MD and KMC,…

Materials Science · Physics 2009-11-07 Jikeun Seo , S. -M. Kwon , H. -Y. Kim , J. -S. Kim

We investigate island formation during heteroepitaxial growth using an atomistic model that incorporates deposition, activated diffusion and stress relaxation. For high misfit the system naturally evolves into a state characterized by a…

Statistical Mechanics · Physics 2009-10-30 Albert-László Barabási

A model for diffusion on a cubic lattice with a random distribution of traps is developed. The traps are redistributed at certain time intervals. Such models are useful for describing systems showing dynamic disorder, such as ion-conducting…

Condensed Matter · Physics 2009-10-31 S. Mandal , R. Dasgupta

A model that describes self diffusion, island nucleation and film growth on FCC(001) metal substrates is presented. The parameters of the model are optimized to describe Cu diffusion on Cu(001), by comparing activation energy barriers to a…

Materials Science · Physics 2008-02-03 O. Biham , I. Furman , M. Karimi , G. Vidali , R. Kennett , H. Zeng
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