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To investigate excess-hydrolysis of titanium alkoxides, TiO2 powders were fabricated from titanium-tetra-isopropoxide using 6:1 and 100:1 H2O:Ti (r) ratios. Powders were dried and fired at a range of temperatures ( up to 800 C).…

Materials Science · Physics 2014-10-31 Dorian A. H. Hanaor , Ilkay Chironi , Inna Karatchevtseva , Gerry Triani , Charles C. Sorrell

The electrical transport properties of anodically grown TiO2 nanotubes was investigated. Amorphous nanotubes were anodically grown on titanium foil and transformed through annealing into the anatase phase. Amorphous and polycrystalline…

We report on the transient-enhanced shape transformation of nano-structured Si(001) surfaces upon in vacuo annealing at relatively low temperatures of 1175K - 1225K for a few minutes. We find dramatic surface mass transport concomitant with…

Materials Science · Physics 2009-11-10 H. Lichtenberger , M. Muehlberger , F. Schaffler

This work describes the elaboration of rutile titanium dioxide films with high refractive indices and low scattering by sol-gel process and controlled crystallization. The evolutions of the optical properties and crystalline structure of…

Anatase is a metastable polymorph of TiO$_2$. In contrast to the more widely-studied TiO$_2$ rutile, O vacancies (V$_\mathrm O$'s) are not stable at the anatase (101) surface. Low-temperature STM shows that surface V$_\mathrm O$'s, created…

Effect of uncompensated Ga-V co-doping on structural phase transition, grain growth process and optical properties of TiO2 is reported here. Inhibition of phase transition due to co-doping is confirmed by X-ray diffraction measurement.…

Thin TiO2 films on quartz substrates were prepared by spin coating of undoped and metal-ion-doped Sol Gel precursors. These films were characterised by Scanning Electron Microscopy, Laser Raman Microspectroscopy, Xray Diffraction and UV Vis…

Materials Science · Physics 2021-06-08 D. A. H. Hanaor , G. Triani , C. C. Sorrell

Titanium dioxide has been extensively studied in the rutile or anatase phases, while its high-pressure phases are less well understood, despite that many are thought to have interesting optical, mechanical and electrochemical properties.…

Materials Science · Physics 2022-03-14 Jacob G. Lee , Chris J. Pickard , Bingqing Cheng

Titanium dioxide, TiO$_2$, has multiple applications in catalysis, energy conversion and memristive devices because of its electronic structure. Most of these applications utilize the naturally existing phases: rutile, anatase and brookite.…

Materials Science · Physics 2016-11-28 Ye Luo , Anouar Benali , Luke Shulenburger , Jaron T. Krogel , Olle Heinonen , Paul R. C. Kent

Nanotubed titanic acid (H2Ti2O4(OH)2) was prepared from nanotubed sodium titanate (Na2Ti2O4(OH)2) by an ion exchange reaction in a pH=1 HCl solution. The effect of annealing temperature on the morphology, structure and photocatalytic…

Materials Science · Physics 2010-09-16 Min Zhang , Zhensheng Jin , Jingwei Zhang , Xinyong Guo , Jianjun Yang , Wei Li , Xiaodong Wang , Zhijun Zhang

The influence of the electric field and electric current on the behavior of oxygen vacancies (VOs) in TiO2 anatase was investigated with Scanning Tunneling Microscopy (STM). At the anatase (101) surface VOs are not stable; they migrate into…

Materials Science · Physics 2018-04-16 Martin Setvin , Michael Schmid , Ulrike Diebold

The optical properties of thermally annealed TiO2 samples depend on their preparation process, and the TiO2 thin films usually exist in the form of anatase or rutile or the mixture of the two phases. The electronic structures and optical…

Materials Science · Physics 2016-11-29 Li Jinping , Meng Songhe , Qin Liyuan , Hantao Lu

The recent identification of strongly bound excitons in room temperature anatase TiO$_2$ single crystals and nanoparticles underscores the importance of bulk many-body effects in samples used for applications. Here, for the first time, we…

Mesoscale and Nanoscale Physics · Physics 2018-01-16 Edoardo Baldini , Tania Palmieri , Enrico Pomarico , Gerald Auböck , Majed Chergui

We present a study on the crystallization process of undoped and Ta doped TiO2 amorphous thin films. In particular, the effect of ultra-fast annealing treatments in environments characterized by different oxygen concentrations is…

We investigate the effect of annealing temperature on the crystalline structure and physical properties of tantalum-pentoxide films grown by radio frequency magnetron sputtering. For this purpose, several tantalum films were deposited and…

Understanding the atomic-scale interaction mechanism of CO$_2$ and H$_2$O on TiO$_2$ surface is crucial to establish a correlation between the catalytic efficiency with its exposed facet. Here, with the aid of a three-state model, nudged…

Materials Science · Physics 2020-08-07 Shashi B. Mishra , B. R. K. Nanda

Ruthenium metal and its oxide stand out for their exceptional catalytic activity, stability in Oxygen Evolution Reactions (OER) and electrical conductivity, making them indispensable in electronics and electrocatalysis. In this study,…

Materials Science · Physics 2024-10-31 S. S. Nalawade , R. S. Kim , J. Mahl , S. Cherono , I. Chris-Okoro , V. Craciun , J. Yan , E. Crumlin , D. Kumar , S. Aravamudhan

Water absorption and dissociation processes on pristine low-index TiO$_2$ interfaces are important but poorly understood outside the well-studied anatase (101) and rutile (110). To understand these, we construct three sets of machine…

Materials Science · Physics 2023-03-15 Zezhu Zeng , Felix Wodaczek , Keyang Liu , Frederick Stein , Jürg Hutter , Ji Chen , Bingqing Cheng

Nanoporous anatase TiO2 rods and rutile TiO2 chrysanthemums were successfully synthesized via a simple ethylene glycol-mediated synthesis route. Their morphologies, phase compositions and components were characterized by SEM, TEM, Raman and…

Materials Science · Physics 2012-03-20 Quanjun Li , Bingbing Liu , Yingai Li , Ran Liu , Xianglin Li , Shidan Yu , Dedi Liu , Peng Wang , Bo Zou , Tian Cui , Guangtian Zou

We have found a remarkably large response of the transition temperature of CaFe2As2 single crystals grown out of excess FeAs to annealing / quenching temperature. Whereas crystals that are annealed at 400 C exhibit a first order phase…

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