Related papers: Non-linear spectroscopy of rubidium: An undergradu…
Optical nonlinearities typically require macroscopic media, thereby making their implementation at the quantum level an outstanding challenge. Here we demonstrate a nonlinearity for one atom enclosed by two highly reflecting mirrors. We…
We study theoretically the coherent nonlinear optical response of doped semiconductors with partially occupied subbands. When the Fermi energy of an occupied subband approaches the exciton level of an upper subband, the absorption spectrum…
Microfluidic NMR spectroscopy can probe chemical and bio-chemical processes non-invasively in a tightly controlled environment. We present a dual-channel modular probe assembly for high efficiency microfluidic NMR spectroscopy and imaging.…
Skimmed supersonic beams provide intense, cold, collision-free samples of atoms and molecules are one of the most widely used tools in atomic and molecular laser spectroscopy. High-resolution optical spectra are typically recorded in a…
The integration of cold atomic systems with optical nanofibres is an increasingly important experimental platform. Here, we report on the spectra observed during a strongly driven, single-frequency, two-photon excitation of cold rubidium…
Femtosecond dual-comb lasers have revolutionized linear Fourier-domain spectroscopy by offering a rapid motion-free, precise and accurate measurement mode with easy registration of the combs beat note in the RF domain. Extensions of this…
We experimentally demonstrate two-photon absorption (TPA) with broadband down-converted light (squeezed vacuum). Although incoherent and exhibiting the statistics of a thermal noise, broadband down-converted light can induce TPA with the…
Rydberg atomic electrometry leverages the extreme sensitivity of highly excited atoms for calibration-free electric field measurements. The technique uses a non-metallic vapor cell to link properties of an RF field to a spectroscopic…
We analyze theoretically and experimentally how nonlinear differential-transmission spectroscopy of a lambda-system medium can provide quantitative understanding of the optical dipole moments and transition energies. We focus on the…
We report a measurement of the hyperfine-structure constants of the $^{85}$Rb 4$D_{3/2}$ state using a two-photon 5$S_{1/2}\rightarrow$4$D_{3/2}$ transition. The hyperfine transitions are probed by measuring the transmission of the…
We investigate the Autler-Townes splitting for Rydberg atoms dressed with linearly polarized microwave radiation, resonant with generic $S_{1/2}\leftrightarrow{P}_{1/2}$ and $S_{1/2}\leftrightarrow{P}_{3/2}$ transitions. The splitting is…
Using resonant light absorption, random walk motions of rubidium atoms in nitrogen buffer gas are observed directly. The transmitted light intensity through atomic vapor is measured and its spectrum is obtained, down to orders of magnitude…
The possibility of spatially resolving the optical properties of atomically thin materials is especially appealing as they can be modulated at the micro- and nanoscale by reducing their thickness, changing the doping level or applying a…
We propose a new spectroscopic method for measuring weak transitions in cold and trapped atoms, which exploits the long interaction times and tight confinement offered by dark optical traps together with an electron shelving technique to…
In ponderomotive spectroscopy an amplitude-modulated optical standing wave is employed to probe Rydberg-atom transitions, utilizing a ponderomotive rather than a dipole-field interaction. Here, we engage nonlinearities in the modulation to…
Specific features of nonlinear interference processes at quantum transitions in near- and fully-resonant optically-dense Doppler-broadened medium are studied. The feasibility of overcoming of the fundamental limitation on a…
We calculated third order non-linear polarization to estimate the two-photon absorption of non-interacting two-level molecules in the transmission-type degenerate pump-probe geometry. The spectral intensity and the phase changes of the…
In this article, we present a simulation study of the linear and nonlinear spectroscopy of dense atomic vapors. Motivated by recent experiments, we focus on double quantum spectroscopy which directly probes dipole-dipole interactions. By…
We report on the observation of sub-Doppler resonances on the back-scattered light from a random porous glass medium with rubidium vapor filling its interstices. The sub-Doppler spectral lines are the consequence of saturated absorption…
We study the feasibility of nearly-degenerate two-photon rovibrational spectroscopy in ensembles of trapped, sympathetically cooled hydrogen molecular ions using a resonance-enhanced multiphoton dissociation (REMPD) scheme. Taking advantage…