Related papers: Non-linear spectroscopy of rubidium: An undergradu…
We develop a theoretical treatment of polarization spectroscopy and use it to make predictions about the general form of polarization spectra in the alkali atoms. Using our model, we generate theoretical spectra for the D2 transitions in…
We demonstrate background-free imaging and sideband cooling of a single 133Cs atom via the narrow-line 6S1/2 to 5D5/2 electric quadrupole transition in a 1064 nm optical tweezer. The 5D5/2 state decays through the 6P3/2 state to the ground…
The common approach for producing Rydberg atoms in warm vapor cells is with lasers arranged in a counter-propagating, collinear configuration. Doppler effects in these configurations reduce the efficiency of excitation to the Rydberg state…
We demonstrate the phenomenon of blockade in two-photon excitations to the Rydberg state in thermal vapor. A technique based on optical heterodyne is used to measure the dispersion of a probe beam far off resonant to the D2 line of rubidium…
Nonlinear transmission of 80 and 140 femtosecond pulsed light with $0.79 \mu m$ wavelength through single walled carbon nanotubes suspended in water containing sodium dodecyl sulphate is studied. Pulse-width independent saturation…
Numerical ab initio variational calculations of the transition probabilities and ac Stark shifts in two-photon transitions of antiprotonic helium atoms driven by two counter-propagating laser beams are presented. We found that sub-Doppler…
We present a detailed study of the absolute Doppler-broadened absorption of a probe beam scanned across the potassium D lines in a thermal vapour. Spectra using a weak probe were measured on the 4S $\rightarrow$ 4P transition and compared…
A multichannel dual-comb spectroscopy (DCS) approach for high-resolution, broadband spectral measurements is presented, demonstrating its effectiveness in studying complex atomic systems. By implementing a photodetector array, we enhance…
We introduce an all-optical quantum-enhanced diagnostic for electric fields in low-temperature plasmas. Trace amounts of rubidium vapor, added to argon plasma, allow us to produce spectrally narrow electric field-sensitive optical…
Recent studies have shown that the nonlinear optical response of crystalline systems is fundamentally a quantum geometric property. In this work, we propose two-dimensional coherent spectroscopy (2DCS), which measures the nonlinear…
We show that a combination of linear absorption spectroscopy, hyper-Rayleigh scattering, and a theoretical analysis using sum rules to reduce the size of the parameter space leads to a prediction of the two-photon absorption cross-section…
Although diamond photonics has driven considerable interest and useful applications, as shown in frequency generation devices and single photon emitters, fundamental studies on the third-order optical nonlinearities of diamond are still…
Attosecond nonlinear Fourier transform (NFT) pump probe spectroscopy is an experimental technique which allows investigation of the electronic excitation, ionization, and unimolecular dissociation processes. The NFT spectroscopy utilizes…
We demonstrate two ways of obtaining sub-natural linewidth for probe absorption through room-temperature Rb vapor. Both techniques use a control laser that drives the transition from a different ground state. The coherent drive splits the…
We have carried out theoretical research on ultra-high resolution spectroscopy of atoms (or molecules) in the suggested cell with a series of plane-parallel thin gas layers between spatially separated gas regions of this cell for optical…
We develop a model to calculate nonlinear polarization in a nondegenerate four-wave mixing in diamond configuration which includes the effects of hyperfine structure and Doppler broadening. We verify the model against the experiment with…
Here we report on measurements of the absolute absorption spectra of dense rubidium vapour on the D1 line in the weak-probe regime for temperatures up to 170 C and number densities up to 3 \times 10^14 cm^-3. In such vapours, modifications…
The atomic spectra and structure of the open d- and f-shell elements are extremely complex, where tens of thousands of transitions between fine structure energy levels can be observed as spectral lines across the infrared and UV per…
Vibrational spectroscopy, comprised of infrared absorption and Raman scattering spectroscopy, is widely used for label-free optical sensing and imaging in various scientific and industrial fields. The group theory states that the two…
An optical frequency comb generated with an electro-optic phase modulator and a chirped radiofrequency waveform is used to perform saturation and pump-probe spectroscopy on the $D_1$ and $D_2$ transitions of atomic potassium. With a comb…