Related papers: Non-linear spectroscopy of rubidium: An undergradu…
We extend the powerful frequency-domain analysis of femtosecond two-photon absorption to the intermediate-field regime, which involves both two- and four-photon transitions. Consequently, we find a broad family of shaped pulses that enhance…
We present an experimental approach to detect the saturated absorption spectroscopy different from conventional scheme. Using this approach, crossovers are removed to avoid their overlap with other peaks in the spectrum and sensitivity of…
Optical two-dimensional Fourier-transformed (2DFT) spectroscopy is used to study the coherent optical response of potassium vapor in a thin transmission cell. Rephasing and non-rephasing spectra of the D1 and D2 transitions are obtained and…
We report on the Doppler-free saturation spectroscopy of the nitrous oxide (N$_2$O) overtone transition at 1.28~$\mu$m. This measurement is performed by the noise-immune cavity-enhanced optical heterodyne molecular spectroscopy (NICE-OHMS)…
Non-linear effects in photoemission are shown to open a new access to the band structure of unoccupied states in solids, totally different from hitherto used photoemission spectroscopy. Despite its second-order nature, strong resonant…
The accuracy of quantitative absorption spectroscopy depends on correctly distinguishing molecular absorption signatures in a measured transmission spectrum from the varying intensity or "baseline" of the light source. Baseline correction…
Dual-comb spectroscopy is extended to the visible spectral range with a set-up based on two frequency-doubled femtosecond ytterbium-doped fiber lasers. The dense rovibronic spectrum of iodine around 19240 cm-1 is recorded within 12 ms at…
The dynamics of vibrational wave packets in triplet states of rubidium dimers (Rb2) formed on helium nanodroplets are studied using femtosecond pump-probe photoionization spectroscopy. Due to fast desorption of the excited Rb2 molecules off…
The nonlinear (NL) optical response of bulk lithium niobate (LiNbO$_3$) was investigated at 532 nm using the second harmonic of a Nd:YAG laser delivering pulses of 12 ps. The experiments were performed using the D4$\sigma$ method combined…
A theory of pump-probe spectroscopy is developed in which optical fields drive two-photon Raman transitions between ground states of an ensemble of three-level $\Lambda $ atoms. Effects related to the recoil the atoms undergo as a result of…
We predict a resonant enhancement of the nonlinear optical response of an interacting Rydberg gas under conditions of electromagnetically induced transparency. The enhancement originates from a two-photon process which resonantly couples…
A fiber taper waveguide is used to perform direct optical spectroscopy of a microdisk-quantum-dot system, exciting the system through the photonic (light) channel rather than the excitonic (matter) channel. Strong coupling, the regime of…
We utilize the recently demonstrated orders of magnitude enhancement of extremely nondegenerate two-photon absorption in direct-gap semiconductor photodiodes to perform scanned imaging of 3D structures using IR femtosecond illumination…
We present experiments on two-photon excitation of ${\rm ^{87}}$Rb atoms to Rydberg states. For this purpose, two continuous-wave (cw)-laser systems for both 780 nm and 480 nm have been set up. These systems are optimized to a small…
We present a theoretical study to investigate sub- and super-luminal light propagation in a rubidium atomic system consisting of a Rydberg state by using density matrix formalism. The analysis is performed in a 4-level vee+ladder system…
Spectroscopy has played the key role in revealing, and thereby understanding, the structure of atoms and molecules. A central drive in this field is the pursuit of higher precision and accuracy so that ever more subtle effects might be…
Doppler-free spectroscopy using two counter-propagating dual-frequency laser beams in alkali vapor cells has been demonstrated recently, providing the detection of high-contrast sign-reversed natural-linewidth sub-Doppler resonances.…
We report a precise measurement of the hyperfine interval in the ${2P}_{1/2}$ state of $^{7}$Li. The transition from the ground state ($D_1$ line) is accessed using a diode laser and the technique of saturated-absorption spectroscopy in hot…
Experimental insight into the elementary processes underlying charge transfer across interfaces has blossomed with the wide-spread availability of ultra-high vacuum set-ups that allow the preparation and characterization of solid surfaces…
Resonant nonlinear-optical interference processes in four-level Doppler-broadened media are studied. Specific features of amplification and optical switching of short-wavelength radiation in a strongly-absorbing resonant gas under coherent…