Related papers: Non-linear spectroscopy of rubidium: An undergradu…
We present a simple, analytic model for pump-probe spectroscopy in dilute atomic gases. Our model treats multilevel atoms, takes several broadening mechanisms into account and, with no free parameters, shows excellent agreement with…
Quantum spectroscopy seeks to probe chemical systems using nonclassical light, which has properties that are qualitatively and quantitatively different than conventional light sources. One promising technique uses intensity-correlated twin…
Spectroscopy of alkali-buffer gas mixtures at high pressures from single-digit to several 100 bars in the regime of substantial collisional broadening is relevant in a wide range of fields, ranging from collisional redistribution cooling to…
We present an experimental and theoretical investigation of two-photon direct frequency-comb spectroscopy performed through velocity-selective excitation. In particular, we explore the effect of repetition rate on the…
A cascade of two-level superconducting artificial atoms -- a source and a probe -- strongly coupled to a semi-infinite waveguide is a promising tool for observing nontrivial phenomena in quantum nonlinear optics. The probe atom can scatter…
We report on Doppler-free continuous-wave optical UV-spectroscopy resolving the hyperfine structure of the $\mathrm{A}\,^2\Sigma^+ \leftarrow \mathrm{X}\,^2\Pi_{3/2}$ transition in nitric oxide for total angular momenta $J_X=1.5-19.5$ on…
Accurate parameters of molecular hot-band transitions, i.e., those starting from vibrationally excited levels, are needed to accurately model high-temperature spectra in astrophysics and combustion, yet laboratory spectra measured at high…
We propose the new method of essential decrease of transit-time broadening of Doppler-free absorption resonances on transitions between long-lived quantum levels of atoms (or molecules) of a rarefied gas medium. This method is based on…
Applicability and accuracy of traditional scanned-wavelength direct absorption spectroscopy (SDAS) diagnostic method is largely affected by combustion state such as temperature and pressure. To resolve this problem, an innovative…
In this paper, we introduce an all-fibered dual-comb spectrometer based on a new design of highly nonlinear fiber to efficiently convert frequency combs from 1.55 micron to 2 micron We show that our spectrometer can be used to measure…
The analysis of nonlinear spectroscopy, widely used to study the dynamics and structures of condensed-phase matter, typically employs a perturbative approach noticing the weak interaction between the laser and the matter of interest.…
We study resonance redistribution mechanisms inside a hot vapor cell. This is achieved by pumping atoms on the first cesium resonance, 6S1/2-->6P1/2, and subsequently probing the velocity distribution of the 6P1/2 population by a linear…
We present femtosecond pump-probe measurements of the nondegenerate (1960$\,$nm excitation and 1176--1326$\,$nm probe) two-photon absorption spectra of 8 $\,$nm GaAs/12$\,$nm Al$_{0.32}$Ga$_{0.68}$As quantum well waveguides. Experiments…
We present a simple and inexpensive means to measure background-free photoinduced absorption spectra by implementing a dual optical modulation scheme. Our objective is to measure quasi-steady-state absorption spectra of long-lived…
We report the experimental observation of strong two-color optical nonlinearity in an ultracold gas of $^{85}\mathrm{Rb}$-$^{87}\mathrm{Rb}$ atom mixture. By simultaneously coupling two probe transitions of $^{85}$Rb and $^{87}$Rb atoms to…
Using a mid-infrared quantum cascade laser and wavelength modulation absorption spectroscopy, we measure the frequencies of ro-vibrational transitions of N$_2$O in the 17 $\mu$m region with uncertainties below 5 MHz. These lines,…
Coherent two-dimensional spectroscopy in IR or visible region is very effective for studying correlations, energy relaxation/transfer pathways in complex multi-chromophore or multi-mode systems. However it is usually restricted up to…
We demonstrate dual-frequency absorption spectroscopy (DFAS) using laser-cooled 87Rb and 85Rb atoms. Doppler-free resonances with high-contrast are produced, which suggest the suitability of using dual-frequency absorption spectroscopy…
Selective reflection is a high-resolution spectroscopic method that allows the probing of atomic and molecular gases in the near field of dielectric cell windows. It is a sensitive technique for measuring interactions between excited atoms…
We demonstrate a technique for spatially resolved temperature measurement utilizing Rydberg Doppler broadening thermometry. This method employs two focused laser beams arranged perpendicularly to excite laser-cooled atoms from the ground…