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Muon spin relaxation measurements on some quantum spin ice candidate materials, the insulating pyrochlores Pr2B2O7 (B = Sn, Zr, Hf), have been performed for temperatures in the range 0.05-280 K. The results are indicative of a static…

Strongly Correlated Electrons · Physics 2015-06-22 F. R. Foronda , F. Lang , J. S. Möller , T. Lancaster , A. T. Boothroyd , F. L. Pratt , S. R. Giblin , D. Prabhakaran , S. J. Blundell

LiV$_2$O$_4$ spinel is known to exhibit heavy fermion-like behavior below a characteristic temperature $T_K\simeq 20$ K, while it preserves a paramagnetic state down to $T\sim10^{-2}$ K due to geometrical frustration. Here, it is shown that…

Strongly Correlated Electrons · Physics 2019-01-23 H. Okabe , M. Hiraishi , A. Koda , K. M. Kojima , S. Takeshita , I. Yamauchi , Y. Matsushita , Y. Kuramoto , R. Kadono

PbCuTe2O6 is a rare example of a spin liquid candidate featuring a three dimensional magnetic lattice. Strong geometric frustration arises from the dominant antiferromagnetic interaction which generates a hyperkagome network of Cu2+ ions…

Strongly Correlated Electrons · Physics 2016-03-14 P. Khuntia , F. Bert , P. Mendels , B. Koteswararao , A. V. Mahajan , M. Baenitz , F. C. Chou , C. Baines , A. Amato , Y. Furukawa

The insulating pyrochlore compound Nd2Sn2O7 has been shown to undergo a second order magnetic phase transition at Tc ~ 0.91 K to a noncoplanar all-in--all-out magnetic structure of the Nd3+ magnetic moments. An anomalously slow paramagnetic…

Strongly Correlated Electrons · Physics 2017-05-04 P. Dalmas de Reotier , A. Yaouanc , A. Maisuradze , A. Bertin , P. J. Baker , A. D. Hillier , A. Forget

In the garnet structure compound Yb3Ga5O12, the Yb3+ ions (ground state effective spin S' = 1/2) are situated on two interpenetrating corner sharing triangular sublattices such that frustrated magnetic interactions are possible. Previous…

Condensed Matter · Physics 2009-11-10 J. A. Hodges , P. Bonville , M. Rams , K. Krolas

NaCaNi$_2$F$_7$ is an insulating, frustrated A$_2$B$_2$F$_7$ pyrochlore with magnetic S = 1 Ni$^{2+}$ on the pyrochlore B site. Non-magnetic Na and Ca are disordered on the A-site. Magnetic susceptibility measurements made on an oriented…

Materials Science · Physics 2015-04-30 J. W. Krizan , R. J. Cava

A comprehensive study of the structural properties of the heavily investigated rare-earth A2Ir2O7 series under extreme conditions is presented. The series is covered by studying iridates with A = Pr, Sm, Dy-Lu. Temperature- and…

LuCuGaO4 has magnetic Cu2+ and diamagnetic Ga3+ ions distributed on a triangular bilayer and is suggested to undergo a spin-glass transition with T_g approximately 0.4 K. Using muSR and neutron scattering measurements, we show that at low…

Materials Science · Physics 2013-05-29 S Calder , SR Giblin , DR Parker , PP Deen , C Ritter , JR Stewart , S Rols , T Fennell

We report the first observation of two-dimensional incommensurate magnetic fluctuations in the layered metallic perovskite Sr3Ru2O7. The wavevectors where the magnetic fluctuations are strongest are different from those observed in the…

Strongly Correlated Electrons · Physics 2007-05-23 L. Capogna , E. M. Forgan , S. M. Hayden , A. Wildes , J. A. Duffy , A. P. Mackenzie , R. S. Perry , S. Ikeda , Y. Maeno , S. P. Brown

Perturbed angular correlation spectroscopy combined with $ab-initio$ electronic structure calculations is used to unravel the structural phase transition path from the low-temperature polar structure to the high-temperature structural phase…

We report on thermodynamic, magnetization, and muon spin relaxation measurements of the strong spin-orbit coupled iridate Ba$_3$IrTi$_2$O$_9$, which constitutes a new frustration motif made up a mixture of edge- and corner-sharing…

Strongly Correlated Electrons · Physics 2017-09-13 W. -J. Lee , S. -H. Do , Sungwon Yoon , S. Lee , Y. S. Choi , D. J. Jang , M. Brando , M. Lee , E. S. Choi , S. Ji , Z. H. Jang , B. J. Suh , K. -Y. Choi

By means of neutron scattering techniques we have investigated the frustrated pyrochlore magnet Ho_2Sn_2O_7, which was found to show a ferromagnetic spin-ice behavior below T \simeq 1.4 K by susceptibility measurements. High-resolution…

Disordered Systems and Neural Networks · Physics 2007-05-23 Hiroaki Kadowaki , Yoshinobu Ishii , Kazuyuki Matsuhira , Yukio Hinatsu

We have studied the spin liquid Tb$\_2$Sn$\_2$O$\_7$ by neutron diffraction and specific heat measurements. Below about 2 K, the magnetic correlations change from antiferromagnetic to ferromagnetic. Magnetic order settles in two steps, with…

Strongly Correlated Electrons · Physics 2009-11-11 I. Mirebeau , A. Apeteri , J. Rodriguez-Carvajal , P. Bonville , A. Forget , D. Colson , V. Glazkov , J. P. Sanchez , O. Isnard , E. Suard

In this work, we show that the zero field excitation spectra in the quantum spin ice candidate pyrochlore compound \ybti\ is a continuum characterized by a very broad and almost flat dynamical response which extends up to $1-1.5$ meV,…

Strongly Correlated Electrons · Physics 2015-09-30 J. Robert , E. Lhotel , G. Remenyi , S. Sahling , I. Mirebeau , C. Decorse , B. Canals , S. Petit

We investigated the temperature dependence of the superlattice intensity and thermal diffuse scattering intensity of BaAl2O4, which has a network structure with corner-sharing AlO4 tetrahedra, via synchrotron X-ray diffraction experiments.…

Materials Science · Physics 2016-04-27 Y. Ishii , S. Mori , Y. Nakahira , C. Moriyoshi , H. Taniguchi , H. Moriwake , Y. Kuroiwa

We explore orbital dynamics in the spin liquid candidate Ba3CuSb2O9 using multi-frequency electron spin resonance. We prepared two high quality single crystals. The crystal with a slight copper deficiency shows a structural phase transition…

Strongly Correlated Electrons · Physics 2015-12-09 Yibo Han , Masayuki Hagiwara , Takehito Nakano , Yasuo Nozue , Kenta Kimura , Mario Halim , Satoru Nakatsuji

The geometrically-frustrated spin glass Y2Mo2O7 has been considered widely to be crystallographically ordered with a unique nearest neighbor magnetic exchange interaction, J. To test this assertion, we present x-ray-absorption…

Statistical Mechanics · Physics 2009-10-31 C. H. Booth , J. S. Gardner , G. H. Kwei , R. H. Heffner , F. Bridges , M. A. Subramanian

Structure with orbital degeneracy is unstable toward spontaneous distortion. Such orbital correlation usually has a much higher energy scale than spins, and therefore, magnetic transition takes place at a much lower temperature, almost…

Strongly Correlated Electrons · Physics 2018-10-11 Huiyuan Man , Mario Halim , Hiroshi Sawa , Masayuki Hagiwara , Yusuke Wakabayashi , Satoru Nakatsuji

Using inelastic x-ray scattering we have investigated lattice vibrations in a geometric frustrated system CdCr2O4 that upon cooling undergoes a spin-Peierls phase transition at TN = 7.8 K from a cubic and paramagnetic to a tetragonal and…

Strongly Correlated Electrons · Physics 2015-05-28 J. -H. Kim , M. Matsuda , H. Ueda , Y. Ueda , J. -H. Chung , S. Tsutsui , A. Baron , S. -H. Lee

Slow spin fluctuations ($\nu < 10^{12}$ s$^-1$) observed by the muon spin relaxation technique in Y$_{1-x}$Sc$_x$Mn$_2$ exhibits a power law dependence on temperature ($\nu \propto T^\alpha$), where the power converges asymptotically to…

Strongly Correlated Electrons · Physics 2011-06-13 M. Miyazaki , R. Kadono , M. Hiraishi , T. Masuda , A. Koda , K. M. Kojima , T. Yamazaki , Y. Tabata , H. Nakamura