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Crystal structure and thermodynamic properties of Na$_2$SrCo(PO$_4$)$_2$, the chemical sibling of the triangular quantum spin-liquid candidate Na$_2$BaCo(PO$_4$)$_2$, are reported. From single crystal x-ray diffraction and high-resolution…

Strongly Correlated Electrons · Physics 2022-08-12 Vera P. Bader , Jan Langmann , Philipp Gegenwart , Alexander A. Tsirlin

It is shown that a k=0, A_{2u} distortion of the terbium tetrahedral network in Tb2Ti2O7 accounts for the apparent isolation of single tetrahedra as seen in neutron scattering studies. Single tetrahedron collective spin states, rather than…

Materials Science · Physics 2008-10-16 S. H. Curnoe

We study the low-temperature physics of the $SU(2)$-symmetric spin-$1/2$ Heisenberg antiferromagnet on a pyrochlore lattice and find fingerprint evidence for the thermal spin-ice state in this frustrated quantum magnet. Our conclusions are…

Strongly Correlated Electrons · Physics 2016-05-04 Yuan Huang , Kun Chen , Youjin Deng , Nikolay Prokof'ev , Boris Svistunov

We report low temperature specific heat and muon spin relaxation/rotation ($\mu$SR) measurements on both polycrystalline and single crystal samples of the pyrochlore magnet Yb$_2$Ti$_2$O$_7$. This system is believed to possess a spin…

Neutron scattering has been used to study the structure and spin dynamics of La$_{0.85}$Sr$_{0.15}$MnO$_3$. The magnetic structure of this system is ferromagnetic below T_C = 235 K. We see anomalies in the Bragg peak intensities and new…

Strongly Correlated Electrons · Physics 2009-10-31 L. Vasiliu-Doloc , J. W. Lynn , A. H. Moudden , A. M. de Leon-Guevara , A. Revcolevschi

Weak bond disorder disrupts the expected spin-liquid ground-state of the ideal $S$ = 1/2 Heisenberg pyrochlore antiferromagnet. Here we introduce a single crystal study of the structural and magnetic properties of the bond-disordered…

Strongly Correlated Electrons · Physics 2023-07-12 Andrej Kancko , Gerald Giester , Ross H. Colman

The pyrochlore Ho2Ge2O7 is a new highly correlated spin ice material. Physical property measurements including x-ray diffraction, dc susceptibility and ac susceptibility, confirm that it shares the distinctive characteristics of other known…

The SrCr$\_{9p}$Ga$\_{12-9p}$O$\_{19}$ and Ba$\_{2}$Sn$\_{2}$ZnGa$\_{10-7p}$Cr$\_{7p}$O$\_{22}$ compounds are two highly-frustrated magnets possessing a quasi-two-dimensional Kagom\'{e} bilayer of spin 3/2 chromium ions with…

Strongly Correlated Electrons · Physics 2007-05-23 David Bono , Laurent Limot , Philippe Mendels , Gaston Collin , Nicole Blanchard

Muon spin relaxation on Nd$_2$Ti$_2$O$_7$ (NTO) and NdLaTi$_2$O$_7$ (NLTO) compounds are presented. The time spectra for both compounds are as expected for the paramagnetic state at high temperatures, but deviate from the exponential…

Strongly Correlated Electrons · Physics 2014-10-21 Hanjie Guo , Hui Xing , Jun Tong , Qian Tao , Isao Watanabe , Zhu-an Xu

Rare-earth pyrochlores are known to exhibit exotic magnetic phenomena. We report a study of crystal growth and characterizations of a new rare-earth compound Er$_2$AlSbO$_7$, in which Al$^{3+}$ and Sb$^{5+}$ ions share the same positions…

We report on measurements of the sound velocity and attenuation in a single crystal of the candidate quantum- spin-ice material Yb$_2$Ti$_2$O$_7$ as a function of temperature and magnetic field. The acoustic modes couple to the spins…

We have studied spin relaxation in the spin ice compound Dy2Ti2O7 through measurements of the a.c. magnetic susceptibility. While the characteristic spin relaxation time is thermally activated at high temperatures, it becomes almost…

Materials Science · Physics 2009-11-10 J. Snyder , B. G. Ueland , J. S. Slusky , H. Karunadasa , R. J. Cava , Ari Mizel , P. Schiffer

Using neutron diffraction, 170Yb Mossbauer and muSR spectroscopies, we have examined the pyrochlore Yb2Ti2O7 where the Yb3+ S'=1/2 ground state has planar anisotropy. Below ~0.24K, the temperature of the known specific heat lambda…

A new pyrochlore compound, NaCaNi$_2$F$_7$, was recently synthesized and has a single magnetic site with spin-1 Ni$^{2+}$. We present zero field (ZF) and longitudinal field (LF) muon spin rotation ($\mu$SR) measurements on this pyrochlore.…

Strongly Correlated Electrons · Physics 2018-09-26 Y. Cai , M. N. Wilson , A. M. Hallas , L. Liu , B. A. Frandsen , S. R. Dunsiger , J. W. Krizan , R. J. Cava , Y. J. Uemura , O. Rubel , G. M. Luke

We have synthesized the novel material Na_2IrO_3 and studied its structure, transport, magnetic, and thermal properties using powder x-ray diffraction (PXRD), electrical resistivity, isothermal magnetization M versus magnetic field H,…

Strongly Correlated Electrons · Physics 2010-06-04 Yogesh Singh , P. Gegenwart

We report a structural and thermodynamic study of the "stuffed spin ice" material Ho2TiO5 (i.e., Ho2(Ti1.33Ho0.67)O6.67), comparing samples synthesized through two different routes. Neutron powder diffraction and electron diffraction reveal…

Materials Science · Physics 2009-11-13 G. C. Lau , B. G. Ueland , M. L. Dahlberg , R. S. Freitas , Q. Huang , H. W. Zandbergen , P. Schiffer , R. J. Cava

The interplay of spin-orbit interactions and electronic correlations dominates the physical properties of pyrochlore iridates, R2Ir2O7 (R = Y, rare earth element), which are typically magnetic insulators. We report an…

Strongly Correlated Electrons · Physics 2015-06-03 T. F. Qi , O. B. Korneta , Xiangang Wan , L. E. DeLong , P. Schlottmann , G. Cao

Crystal structure, magnetic susceptibility, and specific heat were measured in the normal cubic spinel compounds MnSc_2S_4 and FeSc_2S_4. Down to the lowest temperatures, both compounds remain cubic and reveal strong magnetic frustration.…

Strongly Correlated Electrons · Physics 2009-11-10 V. Fritsch , J. Hemberger , N. Buettgen , E. W. Scheidt , H. A. Krug von Nidda , A. Loidl , V. Tsurkan

A quantum spin liquid is a novel state of matter characterized by quantum entanglement and the absence of any broken symmetry. In condensed matter, the frustrated rare-earth pyrochlore magnets Ho$_2$Ti$_2$O$_7$ and Dy$_2$Ti$_2$O$_7$,…

Strongly Correlated Electrons · Physics 2017-04-05 E. Kermarrec , J. Gaudet , K. Fritsch , R. Khasanov , Z. Guguchia , C. Ritter , K. A. Ross , H. A. Dabkowska , B. D. Gaulin

Physical properties of a pyrohafnate compound Pr2Hf2O7 have been investigated by ac magnetic susceptibility \chi_ ac(T), dc magnetic susceptibility \chi(T), isothermal magnetization M(H) and heat capacity C_p(T) measurements on…

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