English

Metallic Spin Liquid-like Behavior of LiV$_2$O$_4$

Strongly Correlated Electrons 2019-01-23 v1

Abstract

LiV2_2O4_4 spinel is known to exhibit heavy fermion-like behavior below a characteristic temperature TK20T_K\simeq 20 K, while it preserves a paramagnetic state down to T102T\sim10^{-2} K due to geometrical frustration. Here, it is shown that the dynamical spin susceptibility χ(q,ω)\chi({\bf q},\omega) in LiV2_2O4_4 exhibits anomalous duality which is modeled as a sum of itinerant (χF\chi_{\rm F}) and local (χL\chi_{\rm L}) components,and that the local spin dynamics inferred from χL(q,ω)\chi_{\rm L}({\bf q},\omega) is qualitatively different from that expected from time-averaged bulk properties. The anomaly coexists with the marginal Fermi liquid behavior inferred from the lnT-\ln T dependence of the electronic specific heat over a wide temperature range below TKT_K. We argue that such unusual properties of LiV2_2O4_4 can be attributed to the putative metallic spin liquid state emerging near the quantum critical point between spin glass and Fermi liquid states.

Keywords

Cite

@article{arxiv.1812.05843,
  title  = {Metallic Spin Liquid-like Behavior of LiV$_2$O$_4$},
  author = {H. Okabe and M. Hiraishi and A. Koda and K. M. Kojima and S. Takeshita and I. Yamauchi and Y. Matsushita and Y. Kuramoto and R. Kadono},
  journal= {arXiv preprint arXiv:1812.05843},
  year   = {2019}
}

Comments

5 pages, 3 figures, Supplemental Material