LiV2O4 spinel is known to exhibit heavy fermion-like behavior below a characteristic temperature TK≃20 K, while it preserves a paramagnetic state down to T∼10−2 K due to geometrical frustration. Here, it is shown that the dynamical spin susceptibility χ(q,ω) in LiV2O4 exhibits anomalous duality which is modeled as a sum of itinerant (χF) and local (χL) components,and that the local spin dynamics inferred from χL(q,ω) is qualitatively different from that expected from time-averaged bulk properties. The anomaly coexists with the marginal Fermi liquid behavior inferred from the −lnT dependence of the electronic specific heat over a wide temperature range below TK. We argue that such unusual properties of LiV2O4 can be attributed to the putative metallic spin liquid state emerging near the quantum critical point between spin glass and Fermi liquid states.
@article{arxiv.1812.05843,
title = {Metallic Spin Liquid-like Behavior of LiV$_2$O$_4$},
author = {H. Okabe and M. Hiraishi and A. Koda and K. M. Kojima and S. Takeshita and I. Yamauchi and Y. Matsushita and Y. Kuramoto and R. Kadono},
journal= {arXiv preprint arXiv:1812.05843},
year = {2019}
}