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Single crystals of a novel ruthenate, Ca2Ru2O7, were obtained. An X-ray diffraction study on a single crystal revealed that this material crystallizes in a pyrochlore structure with a lattice parameter, a = 10.197 Angstroms. The magnetic…

Materials Science · Physics 2009-11-11 Taiya Munenaka , Hirohiko Sato

We report the growth of large high quality crystals of the frustrated magnet, Pr2Zr2O7 by the floating zone technique. Several crystals have been produced starting with varying levels of excess of Pr6O11 to compensate for the loss of Pr2O3…

Materials Science · Physics 2016-11-09 M. Ciomaga Hatnean , C. Decorse , M. R. Lees , O. A. Petrenko , D. S. Keeble , G. Balakrishnan

We have investigated the spin fluctuations in the langasite compound Ba3NbFe3Si2O14 in both the ordered state and as a function of temperature. The low temperature magnetic structure is defined by a spiral phase characterized by magnetic…

Strongly Correlated Electrons · Physics 2015-05-19 C. Stock , L. C. Chapon , A. Schneidewind , Y. Su , P. G. Radaelli , D. F. McMorrow , A. Bombardi , N. Lee , S. -W. Cheong

We report measurements of the ac susceptibility of the cooperative paramagnet Tb2Ti2O7 in a strong magnetic field. Our data show the expected saturation maximum in chi(T) and also an unexpected low frequency dependence (< 1 Hz) of this…

Statistical Mechanics · Physics 2011-11-09 B. G. Ueland , G. C. Lau , R. J. Cava , J. R. OBrien , P. Schiffer

Pyrochlore materials are characterized by their hallmark network of corner-sharing rare-earth tetrahedra, which can produce a wide array of complex magnetic ground states. Ferromagnetic Ising pyrochlores often obey the "two-in-two-out" spin…

Quantum spin liquids are highly entangled ground states of quantum systems with emergent gauge structure, fractionalized spinon excitations, and other unusual properties. While these features clearly distinguish quantum spin liquids from…

Strongly Correlated Electrons · Physics 2013-06-18 Lucile Savary , Leon Balents

The antiferromagnetic pyrochlore material NaCaCo$_2$F$_7$ is a thermal spin liquid over a broad temperature range (~ 140 K down to $T_F = 2.4 $K), in which magnetic correlations between Co$^{2+}$ dipole moments explore a continuous manifold…

Strongly Correlated Electrons · Physics 2017-04-26 K. A. Ross , J. M. Brown , R. J. Cava , J. W. Krizan , S. E. Nagler , J. A. Rodriguez-Rivera , M. B. Stone

We study the finite-temperature transition in a model XY antiferromagnet on a pyrochlore lattice, which describes the pyrochlore material Er2Ti2O7. The ordered magnetic structure selected by thermal fluctuations is six-fold degenerate.…

Strongly Correlated Electrons · Physics 2014-04-15 M. E. Zhitomirsky , P. C. W. Holdsworth , R. Moessner

Strontium titanate is a classic quantum paraelectric oxide material that has been widely studied in bulk and thin films. It exhibits a well-known cubic-to-tetragonal antiferrodistortive phase transition at 105 K, characterized by the…

A single crystal of lead-zirconate-titanate (PZT), composition Pb(Zr0.80Ti0.20)O3, was studied by polarized-Raman scattering as a function of temperature. Raman spectra reveal that the local structure deviates from the average structure in…

Materials Science · Physics 2015-06-23 J. Frantti , Y. Fujioka , A. Puretzky , Y. Xie , Z. -G. Ye , C. Parish , A. M. Glazer

We apply the finite-temperature variational cluster approach to a strongly correlated and spin-orbit coupled model for four electrons (i.e. two holes) in the $t_{2g}$ subshell. We focus on parameters suitable for antiferromagnetic Mott…

Strongly Correlated Electrons · Physics 2021-07-21 Jan Lotze , Maria Daghofer

The ferrimagnetic spinel $\mathrm{CoV_2O_4}$ has been a topic of intense recent interest, both as a frustrated insulator with unquenched orbital degeneracy and as a near-itinerant magnet which can be driven metallic with moderate applied…

Strongly Correlated Electrons · Physics 2016-02-03 D. Reig-i-Plessis , D. Casavant , V. O. Garlea , A. A. Aczel , M. Feygenson , J. Neuefeind , H. D. Zhou , S. E. Nagler , G. J. MacDougall

Geometrical frustration among interacting spins combined with strong quantum fluctuations destabilize long-range magnetic order in favour of more exotic states such as spin liquids. By following this guiding principle, a number of spin…

Pyrochlores offer an ideal playground to investigate the magnetic ground state of frustrated magnetic systems. In this class of materials, competition between various magnetic interactions remains frustrated and prevents an ordered magnetic…

Strongly Correlated Electrons · Physics 2022-10-06 Karan Singh , Dheeraj Ranaut , G. Sharma , K. Mukherjee

Sc$_{2}$Ga$_{2}$CuO$_{7}$ (SGCO) crystallizes in a hexagonal structure (space group: $P$$6$$_{3}/mmc$),\textcolor{black}{{} which can be seen as an alternating stacking of single and double triangular layers. Combining neutron, x-ray, and…

Strongly Correlated Electrons · Physics 2015-11-25 R. Kumar , P. Khuntia , D. Sheptyakov , P. G. Freeman , H. M. Rønnow , B. Koteswararao , M. Baenitz , M. Jeong , A. V. Mahajan

We have investigated the spin dynamics in the bilayered perovskite Sr3Ru2O7 as a function of magnetic field and temperature using 17O-NMR. This system sits close to a metamagnetic quantum critical point (MMQCP) for the field perpendicular…

Strongly Correlated Electrons · Physics 2007-05-23 Kentaro Kitagawa , Kenji Ishida , Robin S. Perry , Takashi Tayama , Toshiro Sakakibara , Yoshiteru Maeno

We report the observation of spin glass state in the double perovskite oxide Sr$_{2}$FeCoO$_{6}$ prepared through sol-gel technique. Initial structural studies using x rays reveal that the compound crystallizes in tetragonal $I 4/m$…

The magnetization (both dc and ac) of pyrochlore Eu2Ti2O7 have been investigated. Ac susceptibility measurements reveal a new unusual spin freezing below 35K for pure Eu2Ti2O7. Frequency dependence of these ac peak positions indicate slow…

Materials Science · Physics 2018-05-23 Arkadeb Pal , Abhishek Singh , Prajyoti Singh , A. K. Ghosh , Sandip Chatterjee

Magnetic and magnetoelastic properties of terbium titanate pyrochlore in paramagnetic phase are simulated. The magnetic field and temperature dependences of magnetization and forced magnetostriction in Tb2Ti2O7 single crystals and…

Strongly Correlated Electrons · Physics 2011-10-27 V. V. Klekovkina , A. R. Zakirov , B. Z. Malkin , L. A. Kasatkina

The magnetic pyrochlore oxide materials of general chemical formula R2Ti2O7 and R2Sn2O7 (R = rare earth) display a host of interesting physical behaviours depending on the flavour of rare earth ion. These properties depend on the value of…

Statistical Mechanics · Physics 2015-06-24 Adrian G. Del Maestro , Michel J. P. Gingras
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