English

Quantum criticality at the end of a pseudogap phase in superconducting infinite-layer nickelates

Strongly Correlated Electrons 2025-10-15 v1 Superconductivity

Abstract

In many unconventional superconductors, the strange-metal regime is thought to emerge from quantum criticality, yet in cuprates this link is obscured by the enigmatic pseudogap. Superconducting infinite-layer nickelates provide a new arena to test this paradigm but are constrained to thin films, precluding calorimetry. We use the Seebeck coefficient as a low-temperature proxy for entropy per carrier and uncover a clear quantum-critical thermodynamic signature: in La1x_{1-x}Srx_xNiO2_2 at the onset of TT-linear resistivity (x=0.20x=0.20), S/TS/T diverges logarithmically upon cooling, S/TlogTS/T \propto \log T. Boltzmann transport based on ARPES-derived band structure reproduces the high-temperature magnitude and sign of S/TS/T and reveals a threefold mass renormalization at the Fermi level. To identify the terminating phase, we analyze Hall data across Nd1x_{1-x}Srx_xNiO2_2 and show that its temperature evolution is quantitatively captured by a minimal two-band model in which a strongly correlated Ni-dx2y2d_{x^2-y^2} Fermi surface exhibits Planckian TT-linear scattering while the rare-earth Nd-ss pocket remains Fermi-liquid-like. Inverting the zero-temperature Hall response reveals a collapse of the Ni-dx2y2d_{x^2-y^2} band carrier density from 1+p1+p to pp holes across the critical doping, without long-range magnetic order -- mirroring the cuprate pseudogap transition in cuprates. These results establish a quantum critical point at the end of a pseudogap-like phase in infinite-layer nickelates and unify the broader paradigm among correlated superconductors that strange metal behaviour is intimately linked to quantum criticality.

Keywords

Cite

@article{arxiv.2510.12786,
  title  = {Quantum criticality at the end of a pseudogap phase in superconducting infinite-layer nickelates},
  author = {C. Iorio-Duval and E. Beauchesne-Blanchet and F. Perreault and J. L. Santana González and W. Sun and Y. F. Nie and A. Gourgout and G. Grissonnanche},
  journal= {arXiv preprint arXiv:2510.12786},
  year   = {2025}
}

Comments

8 pages, 3 figures