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Thermoelectricity evidence for quantum criticality in clean infinite-layer nickelate films

Superconductivity 2025-08-19 v1 Materials Science Strongly Correlated Electrons

Abstract

We investigate the Seebeck coefficient (SS) in infinite-layer nickelate films with different disorder levels. The disordered NdNiO2_{2} film exhibits a flat S/TS/T curve, whereas cleaner samples display a logarithmic divergence with decreasing temperature, followed by a pronounced ``hump'' near 25 K. These distinct behaviors reveal a disorder-driven transition from band-structure-dominated transport to quantum-critical-dominated transport. Below the ``hump'' temperature, four-fold symmetry breaking is observed in the in-plane angular magnetoresistance, indicating the presence of short-range antiferromagnetic order in parent infinite-layer nickelate films. Furthermore, the logarithmic divergence in S/TS/T is also observed in a clean superconducting Sm0.73_{0.73}Ca0.05_{0.05}Eu0.22_{0.22}NiO2_{2} film, where it coexists with linear-in-temperature resistivity over the same temperature range. These findings demonstrate the existence of quantum criticality over a wide doping range in clean infinite-layer nickelate films, similar to cuprates, which highlights the central role of antiferromagnetic spin correlations in their superconducting pairing mechanisms.

Keywords

Cite

@article{arxiv.2508.12974,
  title  = {Thermoelectricity evidence for quantum criticality in clean infinite-layer nickelate films},
  author = {Xu Zhang and Chihao Li and Mingwei Yang and Yan Zhao and Zhitong An and Danfeng Li and Liang Qiao and Haichao Xu and Rui Peng and Donglai Feng and Shiyan Li},
  journal= {arXiv preprint arXiv:2508.12974},
  year   = {2025}
}

Comments

8 pages, 4 figures