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Evidence for quasi-two-dimensional superconductivity in infinite-layer nickelates

Superconductivity 2023-07-24 v1 Materials Science Strongly Correlated Electrons

Abstract

After being expected as a promising analogue to cuprates for decades, superconductivity was recently discovered in infinite-layer nickelates, providing new opportunities to explore mechanisms of high-temperature superconductivity. However, in sharp contrast to the single-band quasi-two-dimensional superconductivity in cuprates, nickelates exhibit a multi-band electronic structure and an unexpected isotropic superconductivity as reported recently, which challenges the cuprate-like picture in nickelates. Here, we show the superconductivity in nickelates is actually anisotropic and quasi-two-dimensional in nature, as that in cuprates. By synthesizing high-quality lanthanide nickelate films with enhanced crystallinity and superconductivity (TconsetT_{c}^{onset} = 18.8 K, TczeroT_{c}^{zero} = 16.5 K), strong anisotropic magnetotransport behaviors have been observed. The quasi-two-dimensional nature is further confirmed by the existence of a cusp-like peak of the angle-dependent TcT_{c}, and a Berezinskii-Kosterlitz-Thouless transition near TcT_{c}. Our work thus suggests a quasi-two-dimensional superconductivity in infinite-layer nickelates, implying a single-3dx2y2d_{x^2-y^2}-band cuprate-like picture may remain valid in these compounds.

Keywords

Cite

@article{arxiv.2204.13264,
  title  = {Evidence for quasi-two-dimensional superconductivity in infinite-layer nickelates},
  author = {Wenjie Sun and Yueying Li and Ruxin Liu and Jiangfeng Yang and Jiayi Li and Shengjun Yan and Haoying Sun and Wei Guo and Zhengbin Gu and Yu Deng and Xuefeng Wang and Yuefeng Nie},
  journal= {arXiv preprint arXiv:2204.13264},
  year   = {2023}
}

Comments

32 pages, 4 main figures, 6 extended data