English

Probing embedded topological modes in bulk-like GeTe-Sb$_2$Te$_3$ heterostructures

Mesoscale and Nanoscale Physics 2021-09-07 v2 Materials Science

Abstract

The interface between topological and normal insulators hosts metallic states that appear due to the change in band topology. While these topological states at a surface, i.e., a topological insulator-air/vacuum interface, have been studied intensely, topological states at a solid-solid interface have been less explored. Here we combine experiment and theory to study such \textit{embedded} topological states (ETSs) in heterostructures of GeTe (normal insulator) and Sb2_2Te3_3 (topological insulator). We analyse their dependence on the interface and their confinement characteristics. To characterise the heterostructures, we evaluate the GeTe-Sb2_2Te3_3 band offset using X-ray photoemission spectroscopy, and chart the elemental composition using atom probe tomography. We then use first-principles to independently calculate the band offset and also parametrise the band structure within a four-band continuum model. Our analysis reveals, strikingly, that under realistic conditions, the interfacial topological modes are delocalised over many lattice spacings. Interestingly, the first-principles calculations indicate that the ETSs are relatively robust to disorder and this may have practical ramifications. Our study provides insights into how to manipulate topological modes in heterostructures and also provides a basis for recent experimental findings [Nguyen \textit{et al.}, Sci. Rep. \textbf{6}, 27716 (2016)] where ETSs were seen to couple over large distances.

Keywords

Cite

@article{arxiv.1912.11167,
  title  = {Probing embedded topological modes in bulk-like GeTe-Sb$_2$Te$_3$ heterostructures},
  author = {Hisao Nakamura and Johannes Hofmann and Nobuki Inoue and Sebastian Koelling and Paul M. Koenraad and Gregor Mussler and Detlev Grützmacher and Vijay Narayan},
  journal= {arXiv preprint arXiv:1912.11167},
  year   = {2021}
}
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