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相关论文: Ab-initio path integral techniques for molecules

200 篇论文

An expression for the Green function G(E;x_1,x_2) of the Schroedinger equation is obtained through the approximations of the path integral by n-fold multiple integrals. The approximations to Re{G(E;x,x)} on the real E-axis have peaks near…

计算物理 · 物理学 2007-05-23 S. I. Blinnikov , N. V. Nikitin

Ab initio Monte Carlo simulations have been performed to determine the equilibrium properties of liquid lithium and lithium clusters at different temperatures. First-principles density-functional methods were employed to calculate the…

材料科学 · 物理学 2007-05-23 Sanwu Wang , Steven J. Mitchell , Per Arne Rikvold

The density matrix quantum Monte Carlo (DMQMC) set of methods stochastically samples the exact $N$-body density matrix for interacting electrons at finite temperature. We introduce a simple modification to the interaction picture DMQMC…

化学物理 · 物理学 2022-05-25 William Van Benschoten , James J. Shepherd

Time derivatives of scalar fields occur quadratically in textbook actions. A simple Legendre transformation turns the lagrangian into a hamiltonian that is quadratic in the momenta. The path integral over the momenta is gaussian. Mean…

高能物理 - 理论 · 物理学 2017-04-19 David Amdahl , Kevin Cahill

In this paper it is shown how the generating functional for Green's functions in relativistic quantum field theory and in thermal field theory can be evaluated in terms of a standard quantum mechanical path integral. With this calculational…

高能物理 - 理论 · 物理学 2011-07-19 D. G. C. McKeon , A. Rebhan

We investigate the thermal expansion of crystalline SiO$_2$ in the $\beta$-- cristobalite and the $\beta$-quartz structure with path integral Monte Carlo (PIMC) techniques. This simulation method allows to treat low-temperature quantum…

统计力学 · 物理学 2009-10-31 Chr. Rickwardt , P. Nielaba , M. H. Müser , K. Binder

The energies of $^{3}H$, $^{3}He$, and $^{4}He$ ground states, the ${\frac{3}{2}}^{-}$ and ${\frac{1}{2}}^{-}$ scattering states of $^{5}He$, the ground states of $^{6}He$, $^{6}Li$, and $^{6}Be$ and the $3^{+}$ and $0^{+}$ excited states…

核理论 · 物理学 2016-09-08 B. S. Pudliner , V. R. Pandharipande , J. Carlson , R. B. Wiringa

We derive equations of motion for Green's functions of the multi-orbital Anderson impurity model by differentiating symmetrically with respect to all time arguments. The resulting equations relate the one- and two-particle Green's function…

强关联电子 · 物理学 2019-08-14 Josef Kaufmann , Patrik Gunacker , Alexander Kowalski , Giorgio Sangiovanni , Karsten Held

Learning the Green's function using deep learning models enables to solve different classes of partial differential equations. A practical limitation of using deep learning for the Green's function is the repeated computationally expensive…

机器学习 · 计算机科学 2023-08-02 Kishan Wimalawarne , Taiji Suzuki , Sophie Langer

We present an algorithm for the computation of unbiased Green functions and self-energies for quantum lattice models, free from systematic errors and valid in the thermodynamic limit. The method combines direct lattice simulations using the…

强关联电子 · 物理学 2015-10-28 D. Rost , N. Blümer

The possibility is discussed of using straight-line paths of integration in computing the integral representation of the three-body Coulomb Green's function. In our numerical examples two different integration contours are considered. It is…

数学物理 · 物理学 2015-05-14 S. A. Zaytsev

Within the imaginary-time theory for nonequilibrium in quantum dot systems the calculation of dynamical quantities like Green's functions is possible via a suitable quantum Monte-Carlo algorithm. The challenging task is to analytically…

强关联电子 · 物理学 2013-07-04 Andreas Dirks , Jong E. Han , Mark Jarrell , Thomas Pruschke

Correlated fermions are of high interest in condensed matter (Fermi liquids, Wigner molecules), cold atomic gases and dense plasmas. Here we propose a novel approach to path integral Monte Carlo (PIMC) simulations of strongly degenerate…

量子气体 · 物理学 2016-01-15 Tobias Dornheim , Simon Groth , Alexey Filinov , Michael Bonitz

In this work we develop tools that enable the study of non-adiabatic effects with variational and diffusion Monte Carlo methods. We introduce a highly accurate wave function ansatz for electron-ion systems that can involve a combination of…

化学物理 · 物理学 2014-10-29 Norm M. Tubman , Ilkka Kylänpää , Sharon Hammes-Schiffer , David M. Ceperley

Including finite-temperature effects from the electronic degrees of freedom in electronic structure calculations of semiconductors and metals is desired; however, in practice it remains exceedingly difficult when using zero-temperature…

化学物理 · 物理学 2016-11-24 Alicia Rae Welden , Alexander A. Rusakov , Dominika Zgid

In this work we calculate the thermodynamic properties of hydrogen-helium plasmas with different mass fractions of helium by the direct path integral Monte Carlo method. To avoid unphysical approximations we use the path integral…

等离子体物理 · 物理学 2009-11-11 P. R. Levashov , V. S. Filinov , M. Bonitz , V. E. Fortov

The use of ensemble Monte Carlo (EMC) methods for the simulation of transport in semiconductor devices has become extensive over the past few decades. This method allows for simulation utilizing particles while addressing the full physics…

其他凝聚态物理 · 物理学 2023-04-04 David K. Ferry

Inspired by the recent proposed Legendre orthogonal polynomial representation of imaginary-time Green's functions, we develop an alternate representation for the Green's functions of quantum impurity models and combine it with the…

强关联电子 · 物理学 2016-12-08 Li Huang , Liang Du

The path integral formulation of quantum mechanics, i.e., the idea that the evolution of a quantum system is determined as a sum over all the possible trajectories that would take the system from the initial to its final state of its…

量子物理 · 物理学 2024-06-12 Charles W. Robson , Yaraslau Tamashevich , Tapio T. Rantala , Marco Ornigotti

We present a method to compute real-time path integrals numerically, by Monte-Carlo sampling on near-Lefschetz thimbles. We present a collection of tools based on the Lefschetz thimble methods, which together provide an alternative to…

高能物理 - 格点 · 物理学 2025-02-28 Zong-Gang Mou , Paul M. Saffin , Anders Tranberg