相关论文: Orientation of molecules via laser-induced anti-al…
We study the influence of laser radiation on the electron transport through a molecular wire weakly coupled to two leads. In the absence of a generalized parity symmetry, the molecule rectifies the laser induced current, resulting in…
We investigate the full control over the orientation of a non-symmetric molecule by using moderate and weak electric fields. Quantum Optimal Control techniques allow us to orient any axis of 6-chloropyridazine-3-carbonitrile, which is taken…
A comprehensive theoretical approach to describe the electron-ion radiative recombination in the presence of intense, short laser pulses, which accounts for nondipole corrections is presented. It is based on the relativistic Coulomb-Volkov…
Study on a rectified current induced by active particles has received a great attention due to its possible application to a microscopic motor in biological environments. Insertion of an {\em asymmetric} passive object amid many active…
We consider the use of pulse-shaped broadband femtosecond lasers to optically cool rotational and vibrational degrees of freedom of molecules. Since this approach relies on cooling rotational and vibrational quanta by exciting an electronic…
A long laser beam propagating through an underdense plasma produces a positively charged ion channel by expelling plasma electrons in the transverse direction. We consider the dynamics of a test electron in a resulting two-dimensional…
The multiphoton ionization rate of molecules depends on the alignment of the molecular axis with respect to the ionizing laser polarization. By studying molecular frame photo-electron angular distributions from N$_2$, O$_2$ and benzene, we…
We apply a time-dependent perturbation theory based on unitary transformations combined with averaging techniques, on molecular orientation dynamics by ultrashort pulses. We test the validity and the accuracy of this approach on LiCl…
Measuring and controlling the ionization dynamics by intense laser fields has recently led to important breakthroughs, from the investigation of tunneling time delays to attosecond molecular imaging by electron holography. In these…
We show that a topological investigation of the phase space of a Semiconductor Ring Laser can be used to devise switching schemes which are alternative to optical pulse injection of counter-propagating light. To provide physical insight in…
Ultrashort pulsed mode-locked lasers enable research at new time-scales and revolutionary technologies from bioimaging to materials processing. In general, the performance of these lasers is determined by the degree to which the pulses of a…
We study optical response of a resonant medium possessing nonlinear coupling to external field driven by a few-cycle pump pulse sequence. We demonstrate the possibility to directly produce unipolar half-cycle pulses from the medium…
Using a three-dimensional quasiclassical technique we explore molecular double ionization by a linearly polarized, infrared (800 nm) and ultrashort (6 fs) laser pulse. We first focus on intensities corresponding to the tunneling regime and…
Supersonic beams of polar molecules are deflected using inhomogeneous electric fields. The quantum-state selectivity of the deflection is used to spatially separate molecules according to their quantum state. A detailed analysis of the…
Experimental results, supported by precise modelling, demonstrate optimisation of a plasma-based injector with intermediate laser pulse energy ($<1$ J), corresponding to a normalised vector potential $a_0 = 2.15$, using ionisation injection…
The simultaneous laser-driven acceleration and angular manipulation of the fast electron beam is experimentally demonstrated. The bunch of multi-MeV energy charged particles is generated during the propagation of the femtosecond laser pulse…
The generation of ultrashort pulses hinges on the careful management of dispersion. Traditionally, this has exclusively involved second-order dispersion, while higher-order dispersion was treated as a nuisance to be minimized. Here we show…
We present a theoretical study of the mixed-field-orientation of asymmetric top molecules in tilted static electric field and non-resonant linearly polarized laser pulse by solving the time-dependent Schr\"odinger equation. Within this…
The strong coupling between intense laser fields and valence electrons in molecules causes a distortion of the potential energy hypersurfaces which determine the motion of nuclei in a molecule and influences possible reaction pathways. The…
Combining the features of molecular wires and femtosecond laser pulses gives the unique opportunity to optically switch electron currents in molecular devices with very high speed. Based on a weak-coupling approximation between wire and…