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A scheme for decoupling and selectively recoupling large networks of dipolar-coupled spins is proposed. The scheme relies on a combination of broadband, decoupling pulse sequences applied to all the nuclear spins with a band-selective pulse…

The impact of control sequences on the environmental coupling of a quantum system can be described in terms of a filter. Here we analyze how the coherent evolution of two interacting spins subject to periodic control pulses, at the example…

量子物理 · 物理学 2015-08-20 Andreas Albrecht , Martin B. Plenio

We investigate numerically the time dependence of the multiple quantum coherences and entanglement in linear chains up to nine nuclear spins of 1/2 coupled by the dipole-dipole interactions. Two models are considered: (1) a spin chain with…

量子物理 · 物理学 2009-11-13 G. B. Furman , V. M. Meerovich , V. L. Sokolovsky

Dense spin ensembles in solids present a natural platform for studying quantum many-body dynamics. Multiple-pulse coherent control can be used to manipulate the magnetic dipolar interaction between the spins to engineer their dynamics.…

量子物理 · 物理学 2024-12-24 Linta Joseph , Wynter Alford , Chandrasekhar Ramanathan

We analyze the simultaneous time-optimal control of two-spin systems. The two non coupled spins which differ in the value of their chemical offsets are controlled by the same magnetic fields. Using an appropriate rotating frame, we restrict…

量子物理 · 物理学 2015-05-19 E. Assemat , M. Lapert , Y. Zhang , M. Braun , S. J. Glaser , D. Sugny

In the framework of nuclear magnetic resonance, we consider the general problem of the coherent control of a spin coupled to a bath by means of composite or continuous pulses of duration $\tau_\mathrm{p}$. We show explicity that it is…

量子物理 · 物理学 2010-03-16 S. Pasini , P. Karbach , C. Raas , G. S. Uhrig

We show how to divide a coupled multi-spin system into a small subset of ``active'' spins that evolve under chemical shift or scalar coupling operators, and a larger subset of ``spectator'' spins which are returned to their initial states,…

量子物理 · 物理学 2009-10-31 N Linden , H Barjat , RJ Carbajo , R Freeman

We demonstrate time reversal of nuclear spin dynamics in highly magnetized dilute liquid 3He-4He mixtures through effective inversion of long-range dipolar interactions. These experiments, which involve using magic sandwich NMR pulse…

其他凝聚态物理 · 物理学 2007-10-10 Michael E. Hayden , Emmanuel Baudin , Geneviève Tastevin , Pierre-Jean Nacher

We study the time evolution of a single spin coupled inhomogeneously to a spin environment. Such a system is realized by a single electron spin bound in a semiconductor nanostructure and interacting with surrounding nuclear spins. We find…

介观与纳米尺度物理 · 物理学 2009-11-07 John Schliemann , Alexander V. Khaetskii , Daniel Loss

The dominant source of decoherence for an electron spin in a quantum dot is the hyperfine interaction with the surrounding bath of nuclear spins. The decoherence process may be slowed down by subjecting the electron spin to suitable…

介观与纳米尺度物理 · 物理学 2017-08-23 Wenxian Zhang , V. V. Dobrovitski , Lea F. Santos , Lorenza Viola , B. N. Harmon

Nuclear spins of noble gases can maintain coherence for hours at ambient conditions owing to their extraordinary isolation by the enclosing, complete electronic shells. This isolation, however, impedes the ability to manipulate and control…

量子物理 · 物理学 2023-11-06 Roy Shaham , Or Katz , Ofer Firstenberg

Decoupling the interactions in a spin network governed by a pair-interaction Hamiltonian is a well-studied problem. Combinatorial schemes for decoupling and for manipulating the couplings of Hamiltonians have been developed which use…

量子物理 · 物理学 2023-11-27 Martin Roetteler

Time reversal in a macroscopic system is contradicting daily experience. It is practically impossible to restore a shattered cup to its original state by just time reversing the microscopic dynamics that led to its breakage. Yet, with the…

The polarisation dynamics of nuclear spins weakly coupled to an NV center is highly sensitive to the parameters of the microwave control and the nuclear Larmor frequency. What is commonly regarded as a challenge, we propose here as a…

量子物理 · 物理学 2018-10-24 Q. Chen , Z. -Y. Wang , B. Tratzmiller , I. Schwartz , M. B. Plenio

An exact general theory of heteronuclear decoupling is presented for spin-1/2 IS systems. RF irradiation applied to the I spins decouples the S spins by reversing the sign of antiphase magnetization. A one-to-one correspondence is…

化学物理 · 物理学 2015-06-19 Thomas E. Skinner

We study the decoherence of a single electron spin in an isolated quantum dot induced by hyperfine interaction with nuclei for times smaller than the nuclear spin relaxation time. The decay is caused by the spatial variation of the electron…

介观与纳米尺度物理 · 物理学 2016-08-31 Alexander Khaetskii , Daniel Loss , Leonid Glazman

We study the decay of multiple quantum (MQ) NMR coherences in systems with the large number of equivalent spins. As being created on the preparation period of MQ NMR experiment, they decay due to the dipole-dipole interactions (DDI) on the…

量子物理 · 物理学 2011-01-25 S. I. Doronin , E. B. Fel'dman , A. I. Zenchuk

We propose a new pulse sequence for dynamical averaging of the dipole-dipole interactions and inhomogeneities of the magnetic fields in the nuclear spin system. The sequence contains a short cycle of the periodic resonant pulse excitation…

量子物理 · 物理学 2015-03-05 S. A. Moiseev , V. A. Skrebnev

Non-equilibrium dynamics of many-body systems is important in many branches of science, such as condensed matter, quantum chemistry, and ultracold atoms. Here we report the experimental observation of a phase transition of the quantum…

量子物理 · 物理学 2015-09-24 Gonzalo A. Alvarez , Dieter Suter , Robin Kaiser

A nitrogen-vacancy (NV) center in a diamond enables the access to an electron spin, which is expected to present highly sensitive quantum sensors. Although exploiting a nitrogen nuclear spin improves the sensitivity, manipulating it using a…

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