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相关论文: Theory of x-ray absorption by laser-dressed atoms

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We devise a theory of x-ray absorption by symmetric-top molecules which are aligned by an intense optical laser. Initially, the density matrix of the system is composed of the electronic ground state of the molecules and a thermal ensemble…

化学物理 · 物理学 2008-02-23 Christian Buth , Robin Santra

X-ray refraction and absorption by neon atoms under the influence of an 800 nm laser with an intensity of 10^13 W/cm^2 is investigated. For this purpose, we use an ab initio theory suitable for optical strong-field problems. Its results are…

原子物理 · 物理学 2013-03-25 Christian Buth , Robin Santra , Linda Young

We devise a theoretical description for the response of nitrogen molecules (N2) to ultrashort and intense x rays from the free electron laser (FEL) Linac Coherent Light Source (LCLS). We set out from a rate-equation description for the…

Photoabsorption of atomic oxygen in the energy region below the $\rm 1s^{-1}$ threshold in x-ray spectroscopy from {\it Chandra} and {\it XMM-Newton} is observed in a variety of x-ray binary spectra. Photoabsorption cross sections…

高能天体物理现象 · 物理学 2015-06-16 B. M. McLaughlin , C. P. Ballance , K. P. Bowen , D. J. Gardenghi , W. C. Stolte

We investigated the complex index of refraction in the x-ray regime of atoms in laser light. The laser (intensity up to 10^13 W/cm^2, wavelength 800nm) modifies the atomic states but, by assumption, does not excite or ionize the atoms in…

原子物理 · 物理学 2008-11-18 Christian Buth , Robin Santra

When treating the absorption of light, one focuses on the absorption coefficient, related to the probability of photons to survive while traversing a layer of material. From the point of view of particles doing the absorption, however, the…

高能天体物理现象 · 物理学 2018-09-26 Nicola Locatelli , Gabriele Ghisellini

We present a new theoretical approach to attosecond laser-assisted photo- and Compton ionization. Attosecond x-ray absorption and scattering are described by $\hat{\mathrsfs{S}}^{(1,2)}$-matrices, which are coherent superpositions of…

原子物理 · 物理学 2010-12-24 G. L. Yudin , D. I. Bondar , S. Patchkovskii , P. B. Corkum , A. D. Bandrauk

Within the framework of the second-order non-relativistic quantum perturbation theory, the methods of the theory of irreducible tensor operators, and nonorthogonal orbitals, the absolute values and shape of the generalized cross-sections of…

原子物理 · 物理学 2025-12-30 A. N. Hopersky , A. M. Nadolinsky , S. A. Novikov , R. V. Koneev

We theoretically study orbital alignment in x-ray-ionized atoms and ions, based on improved electronic-structure calculations starting from the Hartree-Fock-Slater model. We employ first-order many-body perturbation theory to improve the…

原子物理 · 物理学 2023-01-03 Laura Budewig , Sang-Kil Son , Robin Santra

Exploration of a new ultrafast-ultrasmall frontier in atomic and molecular physics has begun. Not only is is possible to control outer-shell electron dynamics with intense ultrafast optical lasers, but now control of inner-shell processes…

We present a non-Hermitian theory of atomic and molecular absorption, which enables computing the absorption spectrum of multi-electron atoms and molecules without using any fitting parameters. We propose a method for optically inducing…

化学物理 · 物理学 2019-04-02 Adi Pick , Petra Ruth Kaprálová-Žďánská , Nimrod Moiseyev

We consider the elastic scattering of electrons by hydrogen atoms in the presence of a two-color circularly polarized laser field in the domain of moderate intensities below $10^{13}$ W/cm$^2$ and high projectile energies. A hybrid approach…

原子物理 · 物理学 2023-06-16 Gabriela Buica

I classify multiphoton absorption into separable, linked, and simultaneous processes. The first and second types can be distinguished when the rate-equation approximation is valid whereas the third type refers to the case when the full…

原子物理 · 物理学 2017-09-14 Christian Buth

We investigate the process of photon absorption by atoms or molecules shortly interacting with a laser beam in the dipole approximation. Assuming that the interaction time $\tau$ is much smaller than the lifetime of the corresponding…

We derive a time-dependent density functional theory appropriate for calculating the near-edge X-ray absorption spectrum in molecules and condensed matter. The basic assumption is to increase the space of many-body wave functions from one…

强关联电子 · 物理学 2015-06-16 G. F. Bertsch , A. Lee

Formulas to describe the photoabsorption and the photon scattering by a plasma or a liquid metal are derived in a unified manner with each other. It is shown how the nuclear motion, the free-electron motion and the core-electron behaviour…

材料科学 · 物理学 2009-10-31 Junzo Chihara

We have studied the Stark effect in the soft x-ray region for various small molecules by calculating the field-dependent x-ray absorption spectra. This effect is explained in terms of the response of molecular orbitals (core and valence),…

化学物理 · 物理学 2025-03-26 Avdhoot Datar , Catherine Wright , Devin A. Matthews

Photoabsorption cross sections for 235 stable nuclei, ranging from $^{40}$Ca to $^{209}$Bi, were investigated by the quasiparticle finite amplitude method (QFAM) based on the axially deformed relativistic Hartree-Bogoliubov (RHB) approach…

核理论 · 物理学 2025-06-25 C. Chen , Y. F. Niu , R. Xu , Y. Tian

The effect of the absorption of hard X-ray photons on the solid-state dynamics, at energies below the defect creation threshold, is considered. First, it is shown that due to the sensitivity to parameter choices, the present state of the…

材料科学 · 物理学 2015-10-08 Michael Leitner , Markus Stana , Manuel Ross , Bogdan Sepiol

We present a method to calculate the natural line width and energy dependent line shape due to fluorescence decay of core excited atoms within a full relativistic multi-reference configuration interaction theory. The atomic absorption lines…

原子物理 · 物理学 2023-07-27 Marc Merstorf , Martin Braß , Maurits W. Haverkort
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