相关论文: Photonic mode density effects on single-molecule f…
Single molecule localization microscopy relies on the precise quantification of the position of single dye emitters in a sample. This precision is improved by the number of photons that can be detected from each molecule. It is therefore…
Two-dimensional molecular aggregate (2DMA), a thin sheet of strongly interacting dipole molecules self-assembled at close distance on an ordered lattice, is a fascinating fluorescent material. It is distinctively different from the single…
Interfacial electron transfer (IET) dynamics in 1,1'-dioctadecyl-3, 3, 3', 3'-tetramethylindodicarbocyanine (DiD) dye molecules / indium tin oxide (ITO) film system have been probed at the ensemble and single-molecule level by recording the…
We report fluorescence blinking statistics measured from single CdSe nanorods (NRs) of seven different sizes with aspect ratio ranging from 3 to 11. This study included core/shell CdSe/ZnSe NRs and core NRs with two different surface…
Luminescence properties of colloidal quantum dots have found applications in imaging, light-sources, and displays. Despite wide interest, several experimental observations from these quantum dots, such as the short lifetime on the scale of…
We calculate the intensity of photon emission from a trion in a single quantum dot, as a function of energy and gate voltage, using the impurity Anderson model and variational wave functions. Assuming a flat density of conduction states and…
We theoretically investigate signatures of stimulated emission at the single photon level for a two-level atom interacting with a one-dimensional light field. We consider the transient regime where the atom is initially excited, and the…
The demand for high-efficiency and miniaturized on-chip light sources drives continuous innovation in photonic crystal (PhC) microcavity lasers. The presence of slow-light effects in PhC microcavities leads to the mode competition between…
Resonance fluorescence from atomic systems consists of a single spectral peak that evolves into a Mollow triplet for a strong excitation field. Photons from different peaks of the triplet show distinct photon correlation that make the…
Abrupt fluorescence intermittency or blinking is long recognized to be characteristic of single nano-emitters. Extended quantum-confined nanostructures also undergo spatially heterogeneous blinking, however, there is no such precedence in…
Fluorescence lifetime experiments are a standard approach for measuring excited state dynamics and local environment effects. Here, we show that entangled photon pairs produced from a continuous-wave (CW) laser diode can replicate pulsed…
We consider an ensemble of diatomic molecules resonantly coupled to an optical cavity under strong coupling conditions at normal incidence. Photodissociation dynamics is examined via direct numerical integration of the coupled…
The ability to control chemical reactions by coupling organic molecules to confined light in a cavity has recently attracted much attention. While most previous studies have focused on single-mode photonic or plasmonic cavities, here we…
In this paper we experimentally study the statistical properties of a bright squeezed vacuum state containing up to 10^13 photons per mode (10 uJ per pulse), produced via high gain parametric down conversion (PDC). The effects of bunching…
We present measurements of how multimode fiber focal-ratio degradation (FRD) and throughput vary with levels of fiber surface polish from 60 to 0.5 micron grit. Measurements used full-beam and laser injection methods at wavelengths between…
At the exit surface of a photonic crystal, the intensity of the diffracted wave can be periodically modulated, showing a maximum in the "positive" (forward diffracted) or in the "negative" (diffracted) direction, depending on the slab…
Charged magneto-excitons X- in a dilute 2D electron gas in narrow and symmetric quantum wells are studied using exact diagonalization techniques. An excited triplet X- state with a binding energy of about 1 meV is found. This state and the…
Open quantum systems can host dark or subradiant states whose decay is highly suppressed. While these states have been extensively studied in the few-excitation regime, their impact on the many-body dynamics remains largely unexplored.…
Single photon emitters are core building blocks of quantum technologies, with established and emerging applications ranging from quantum computing and communication to metrology and sensing. Regardless of their nature, quantum emitters…
We study the collective photon decay of multiple quantum emitters embedded in a thin high-index dielectric layer such as hexagonal boron nitride (hBN), with and without a metal substrate. We first explore the significant role that guided…